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Properties of complex oxide thin films can be tuned over a range of values as a function of mismatch, composition, orientation, and structure. Here, we report a strategy for growing structured epitaxial thermoelectric thin films leading to…

Materials Science · Physics 2013-10-08 D. Pravarthana , O. I. Lebedev , D. Chateigner , S. Hebert , P. A. Salvador , W. Prellier

Thin films of the electron-doped infinite-layer cuprate superconductor Sr$_{1-x}$La$_x$CuO$_2$ (SLCO) with doping $x \approx 0.15$ were grown by means of pulsed laser deposition. (001)-oriented KTaO$_3$ and SrTiO$_3$ single crystals were…

Detailed analysis of transport, magnetism and x-ray absorption spectroscopy measurements on ultrathin La0.7Sr0.3MnO3 films with thicknesses from 3 to 70 unit cells resulted in the identification of a lower critical thickness for a…

Strongly Correlated Electrons · Physics 2009-11-13 M. Huijben , L. W. Martin , Y. -H. Chu , M. B. Holcomb , P. Yu , G. Rijnders , D. H. A. Blank , R. Ramesh

Bi$_2$Se$_3$ is a widely studied 3D topological insulator having potential applications in optics, electronics, and spintronics. When the thickness of these films decrease to less than approximately 6 nm, the top and bottom surface states…

Materials Science · Physics 2024-06-19 Saadia Nasir , Walter J. Smith , Thomas E. Beechem , Stephanie Law

Reversible and irreversible discontinuities at around 573 K and 823 K in the electric conductivity of a strained 175 nm thin film of (La0.8Sr0.2)0.95Ni0.2Fe0.8O3-{\delta} grown by pulsed laser deposition on SrTiO3 (110) are reflected by…

Strongly Correlated Electrons · Physics 2011-06-07 A. Braun , X. Zhang , Y. Sun , U. Müller , Z. Liu , S. Erat , M. Ari , H. Grimmer , S. S. Mao , T. Graule

We have grown La$_{0.3}$Sr$_{0.7}$CoO$_{3-{\delta}}$ thin films by pulsed laser deposition on (LaAlO$_3$)$_{0.3}$(Sr$_2$TaAlO$_3$)$_{0.7}$ substrates with and without a protective LaAlO$_3$ capping layer and investigated their structural…

Materials Science · Physics 2022-09-28 M. Kiaba , O. Caha , F. Abadizaman , A. Dubroka

(111)NiO epitaxial layers are grown on c-sapphire substrates by pulsed laser deposition (PLD) technique. Structural and morphological properties of the films are studied using in-plane as well as out-of-plane high resolution X-ray…

Materials Science · Physics 2021-05-26 Santosh Kumar Yadav , Subhabrata Dhar

Pulsed-laser deposition has been used to grow epitaxial thin films of the giant-dielectric-constant material CaCu_3Ti_4O_{12} on LaAlO_3 and SrTiO_3 substrates with or without various conducting buffer layers. The latter include…

Materials Science · Physics 2009-11-07 W. Si , E. M. Cruz , P. D. Johnson , P. W. Barnes , P. Woodward , A. P. Ramirez

Ferroelectric BaTiO3 films with large polarization have been integrated with Si(001) by pulsed laser deposition. High quality c-oriented epitaxial films are obtained in a substrate temperature range of about 300 deg C wide. The deposition…

Materials Science · Physics 2018-01-25 Jike Lyu , Ignasi Fina , Raul Solanas , Josep Fontcuberta , Florencio Sanchez

In this paper we report the deposition of epitaxial thin films of Nd1-xSrxCoO3 with x=0, 0.2 and 0.5 on single crystalline substrates (SrTiO3 and LaAlO3) carried out by means of rf-magnetron sputtering. The deposited films are all…

The interrelation between the epitaxial strain and oxygen deficiency in La0.7Ca0.3MnO3-{\delta} thin films was studied in terms of structural and functional properties. The films with a thickness of 1000{\AA} were prepared using a PLD…

Materials Science · Physics 2015-06-23 K. Kawashima , G. Logvenov , G. Christiani , H. -U. Habermeier

Understanding and manipulating properties emerging at a surface or an interface require a thorough knowledge of structure-property relationships. We report a study of a prototype oxide system, La2/3Sr1/3MnO3 grown on SrTiO3(001), by…

Strongly Correlated Electrons · Physics 2019-04-11 Lina Chen , Zhen Wang , Gaomin Wang , Hangwen Guo , Mohammad Saghayezhian , Zhaoliang Liao , Yimei Zhu , E. W. Plummer , Jiandi Zhang

Transition metal oxide thin films show versatile electrical, magnetic, and thermal properties which can be tailored by deliberately introducing macroscopic grain boundaries via polycrystalline solids. In this study, we focus on the…

We have synthesized epitaxial Ba2IrO4 (BIO) thin-films on SrTiO3 (001) substrates by pulsed laser deposition and studied their electronic structure by dc-transport and optical spectroscopic experiments. We have observed that BIO thin-films…

Strongly Correlated Electrons · Physics 2014-04-08 J. Nichols , O. B. Korneta , J. Terzic , G. Cao , J. W. Brill , S. S. A. Seo

We investigate nanoscale domain engineering via epitaxial coupling in a set of SrRuO$_3$/PbTiO$_3$/SrRuO$_3$ heterostructures epitaxially grown on (110)$_o$-oriented DyScO$_3$ substrates. The SrRuO$_3$ layer thickness is kept at 55 unit…

We have investigated a method for substituting oxygen with nitrogen in EuO thin films, which is based on molecular beam epitaxy distillation with NO gas as the oxidizer. By varying the NO gas pressure, we produce crystalline, epitaxial…

Materials Science · Physics 2012-05-23 R. Wicks , S. G. Altendorf , C. Caspers , H. Kierspel , R. Sutarto , L. H. Tjeng , A. Damascelli

LaFeAsO1-xFx thin films were deposited successfully on (001)-oriented LaAlO3 and MgO substrates from stoichiometric LaFeAsO1-xFx polycrystalline targets with fluorine concentrations up to x = 0.25 by PLD. Room temperature deposition and…

Superconductivity · Physics 2009-11-13 E. Backen , S. Haindl , T. Niemeier , T. Freudenberg , J. Werner , G. Behr , L. Schultz , B. Holzapfel

The sequence of ground states for SrTiO3 film subjected to epitaxial strain as well as to mechanical stress along the [001] and [110] axes is calculated from first principles within the density functional theory. Under the fixed-strain…

Materials Science · Physics 2016-07-11 Alexander I. Lebedev

We report on the observation of metallic behavior in thin films of oxygen-deficient SrTiO$_3$ - down to 9 unit cells - when coherently strained on (001) SrTiO$_3$ or DyScO$_3$-buffered (001) SrTiO$_3$ substrates. These films have carrier…

Materials Science · Physics 2016-06-06 Purnima P. Balakrishnan , Urusa S. Alaan , Matthew T. Gray , Yuri Suzuki

Using molecular beam epitaxy (MBE) to grow multi-elemental oxides (MEO) is generally challenging, partly due to difficulty in stoichiometry control. Occasionally, if one of the elements is volatile at the growth temperature, stoichiometry…

Materials Science · Physics 2022-11-08 Gaurab Rimal , Alessandro R. Mazza , Matthew Brahlek , Seongshik Oh