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Several methods of extrapolating the virial coefficients, including those proposed in this work, are discussed. The methods are demonstrated on predicting higher virial coefficients of one-component hard spheres. Estimated values of the…

Statistical Mechanics · Physics 2012-07-16 M. Oncák , A. Malijevský , J. Kolafa , S. Labík

We propose a new semi empirical expression of the virial coefficients for a hard sphere fluid which is valid in the disordered phase over the whole density range. The results are in good agreement with the numerical data and better than…

Statistical Mechanics · Physics 2016-03-15 Richard Bonneville

We evaluate the virial coefficients B_k for k<=10 for hard spheres in dimensions D=2,...,8. Virial coefficients with k even are found to be negative when D>=5. This provides strong evidence that the leading singularity for the virial series…

Statistical Mechanics · Physics 2016-10-06 N. Clisby , B. M. McCoy

We characterize the high-temperature thermodynamics of rotating bosons and fermions in two- (2D) and three-dimensional (3D) isotropic harmonic trapping potentials. We begin by calculating analytically the conventional virial coefficients…

Quantum Gases · Physics 2020-08-12 C. E. Berger , K. J. Morrell , J. E. Drut

We explore quantitative descriptors that herald when a many-particle system in $d$-dimensional Euclidean space $\mathbb{R}^d$ approaches a hyperuniform state as a function of the relevant control parameter. We establish quantitative…

Soft Condensed Matter · Physics 2021-05-26 Salvatore Torquato

The demixing transition of a binary fluid mixture of additive hard spheres is analyzed for different size asymmetries by starting from the exact low-density expansion of the pressure. Already within the second virial approximation the fluid…

Statistical Mechanics · Physics 2009-11-10 M. Lopez de Haro , C. F. Tejero

Two-dimensional dry foams coarsen according to the von Neumann law as $dA/dt \propto (n-6)$ where $n$ is the number of sides of a bubble with area $A$. Such foams reach a self-similar scaling state where area and side-number distributions…

Soft Condensed Matter · Physics 2023-09-19 Anthony T. Chieco , James P. Sethna , Douglas J. Durian

We study the phase behavior of hard spheres confined between two parallel hard plates using extensive computer simulations. We determine the full equilibrium phase diagram for arbitrary densities and plate separations from one to five…

Soft Condensed Matter · Physics 2009-11-11 Andrea Fortini , Marjolein Dijkstra

We develop an extension of the original Reiss-Frisch-Lebowitz scaled particle theory that can serve as a predictive method for the hard sphere pair correlation function g(r). The reversible cavity creation work is analyzed both for a single…

Statistical Mechanics · Physics 2009-11-11 Frank H. Stillinger , Pablo G. Debenedetti , Swaroop Chatterjee

Based on the survey of the literatures on the new improvements on the equation of state (EOS) for the hard sphere fluids, we here compare lots of different EOSs and present a very accurate equation of state for this kind of fluids. The new…

Soft Condensed Matter · Physics 2025-12-08 Can Cui , Jianxiang Tian

In experimental systems, colloidal particles are virtually always at least somewhat polydisperse, which can have profound effects on their ability to crystallize. Unfortunately, accurately predicting the effects of polydispersity on phase…

Soft Condensed Matter · Physics 2025-10-09 Antoine Castagnède , Laura Filion , Frank Smallenburg

New proposals for the equation of state of four- and five-dimensional hard-hypersphere mixtures in terms of the equation of state of the corresponding monocomponent hard-hypersphere fluid are introduced. Such proposals (which are…

Soft Condensed Matter · Physics 2020-04-22 Mariano López de Haro , Andrés Santos , Santos B. Yuste

The most efficient way to pack equally sized spheres isotropically in 3D is known as the random close packed state, which provides a starting point for many approximations in physics and engineering. However, the particle size distribution…

Soft Condensed Matter · Physics 2010-01-05 Robert S. Farr , Robert D. Groot

We present the full thermodynamics of a fluid confined by an arbitrary external potential based on the virial expansion of the grand potential. The fluid may be classical or quantum and it is assumed that interatomic interactions are…

Statistical Mechanics · Physics 2008-08-13 Nadia Sandoval-Figueroa , Víctor Romero-Rochín

An equation of state for a multicomponent mixture of non-additive hard spheres in $d$ dimensions is proposed. It yields a rather simple density dependence and constitutes a natural extension of the equation of state for additive hard…

Soft Condensed Matter · Physics 2007-05-23 A. Santos , M. Lopez de Haro , S. B. Yuste

The Ornstein-Zernike equation is solved for the hard-sphere and square-well fluids using a diverse selection of closure relations; the attraction range of the square-well is chosen to be $\lambda=1.5.$ In particular, for both fluids we…

Statistical Mechanics · Physics 2022-07-20 Edwin Bedolla , Luis Carlos Padierna , Ramón Castañeda-Priego

We develop a simple analytical theory that relates dense sphere packings in a cylinder to corresponding disk packings on its surface. It applies for ratios R=D/d (where d and D are the diameters of the hard spheres and the bounding…

Soft Condensed Matter · Physics 2015-05-20 Adil Mughal , Ho Kei Chan , Denis Weaire

A fluid in equilibrium in a finite volume $V$ with particle number $N$ at a density $\rho = N/V$ exceeding the onset density $\rho_f $ of freezing may exhibit phase coexistence between a crystalline nucleus and surrounding fluid. Using a…

Statistical Mechanics · Physics 2015-06-23 Antonia Statt , Peter Virnau , Kurt Binder

Confined fluids display complex behavior due to layering and local packing. Here, we disentangle these effects by confining a hard-sphere fluid to the surface of a cylinder, such the circumference extends only over a few particle diameters.…

Soft Condensed Matter · Physics 2020-04-23 Charlotte F. Petersen , Lukas Schrack , Thomas Franosch

We use virial series to study the equilibrium properties of confined soft-spheres fluids interacting through the inverse-power potentials. The confinement is induced by hard walls with planar, spherical and cylindrical shapes. We evaluate…

Soft Condensed Matter · Physics 2016-09-28 Ignacio Urrutia