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From low-temperature Synchrotron X-ray diffraction, a precise thermal characterization of octahedral distortions in single phase Ruddlesden-Popper Ca3Mn2O7 is performed. Highly sensitive close-steps temperature dependences of Mn-O-Mn bond…

Materials Science · Physics 2020-04-24 Pooja Sahlot , A. K. Sinha , A. M. Awasthi

We report on a novel spin-charge fluctuation in the all-in-all-out pyrochlore magnet Cd$_2$Os$_2$O$_7$, where the spin fluctuation is driven by the conduction of thermally excited electrons/holes and associated fluctuation of Os valence.…

Strongly Correlated Electrons · Physics 2019-12-10 A. Koda , H. T. Hirose , M. Miyazaki , H. Okabe , M. Hiraishi , I. Yamauchi , K. M. Kojima , I. Nagashima , J. Yamaura , Z. Hiroi , R. Kadono

We apply the finite-temperature variational cluster approach to a strongly correlated and spin-orbit coupled model for four electrons (i.e. two holes) in the $t_{2g}$ subshell. We focus on parameters suitable for antiferromagnetic Mott…

Strongly Correlated Electrons · Physics 2021-07-21 Jan Lotze , Maria Daghofer

Giant softening by 30 cm$^{-1}$ of the 490- and 620-cm$^{-1}$ modes is observed by Raman scattering measurements below the Curie temperature of single crystalline LaMnO$_{3+\delta}$ ($0.085\leq \delta\leq0.125$). A pseudogap-like electronic…

We study with the Raman scattering technique two types of phase transitions in the pyroxene compounds NaMSi$_2$O$_6$ (with M=Ti, V, and Cr). In the quasi one-dimensional S=1/2 system NaTiSi$_2$O$_6$ we observe anomalous high-temperature…

Strongly Correlated Electrons · Physics 2007-05-23 M. J. Konstantinović , J. van den Brink , Z. V. Popović , V. V. Moshchalkov , M. Isobe , Y. Ueda

We have measured temperature dependence of low-frequency Raman spectra in CuGeO$_3$, and have observed the quasi-elastic scattering in the $(c,c)$ polarization above the spin-Peierls transition temperature. We attribute it to the…

Single crystals of the spin-gap system $\rm (VO)_2P_2O_7$ have been investigated by means of Raman scattering. At temperatures below T=75 K~$\approx 2\Delta_{01}({\bf k}=0)$, with $\Delta_{01}$ the singlet-triplet gap, a shoulder appears at…

Superconductivity · Physics 2009-10-31 M. Grove , P. Lemmens , G. Güntherodt , B. C. Sales , F. Büllesfeld , W. Assmus

The combination of electronic correlation and spin-orbit coupling is thought to precipitate a variety of highly unusual electronic phases in solids, including topological and quantum spin liquid states. We report a Raman scattering study…

Strongly Correlated Electrons · Physics 2015-04-22 Luke J. Sandilands , Yao Tian , Kemp W. Plumb , Young-June Kim , Kenneth S. Burch

Inelastic scattering of visible light (Raman effect) offers a window into properties of correlated metals such as spin, electron and lattice dynamics as well as their mutual interactions. In this review we focus on electronic and spin…

Superconductivity · Physics 2020-07-20 N Lazarevic , R Hackl

We investigated microscopic lattice states in the donor-acceptor ionic Mott insulator, TTF-BA, by $^{79}$Br-NQR spectroscopy to explore cross-correlated fluctuations between spin, charge and lattice. A ferroelectric transition with lattice…

Strongly Correlated Electrons · Physics 2021-08-11 Keishi Sunami , Tomohiro Baba , Kazuya Miyagawa , Sachio Horiuchi , Kazushi Kanoda

We test the fluctuation-dissipation relation (FDR) in spin ice materials Dy$_2$Ti$_2$O$_7$ and Ho$_2$Ti$_2$O$_7$ by measuring both the magnetic noise and the out-of-phase part of the susceptibility and comparing their ratio. We show that it…

Strongly Correlated Electrons · Physics 2025-10-09 F. Morineau , V. Cathelin , P. C. W. Holdsworth , S. R. Giblin , G. Balakhrishnan , K. Matsuhira , C. Paulsen , E. Lhotel

The spectrum of spin fluctuations in the stacked-triangular antiferromagnet YMnO3 was studied above the Neel temperature using both unpolarized and polarized inelastic neutron scattering. We find an in-plane and an out-of-plane excitation.…

Strongly Correlated Electrons · Physics 2009-11-11 B. Roessli , S. N. Gvasaliya , E. Pomjakushina , K. Conder

The entanglement of electronic spin and orbital degrees of freedom is often the precursor to emergent behaviors in condensed matter systems. With considerable spin-orbit coupling strength, the cobalt atom on a honeycomb lattice offers a…

Using Raman scattering we studied the effect of substitutions on 1D spin fluctuations in CuGeO_3 observed as a spinon continuum in frustration induced exchange scattering. For temperatures below the spin-Peierls transition (T_{SP}=14K) the…

Strongly Correlated Electrons · Physics 2016-08-31 M. Fischer , P. Lemmens , G. Güntherodt , M. Weiden , W. Richter , C. Geibel , F. Steglich

The relationships among charge order, spin fluctuations, and superconductivity in underdoped cuprates remain controversial. We use neutron scattering techniques to study these phenomena in La$_{1.93}$Sr$_{0.07}$CuO$_4$, a superconductor…

Superconductivity · Physics 2015-11-25 H. Jacobsen , I. A. Zaliznyak , A. T. Savici , B. L. Winn , S. Chang , M. Huecker , G. D. Gu , J. M. Tranquada

We report comprehensive Raman-scattering measurements on a single crystal of double-perovskite Nd2ZnIrO6 in temperature range of 4-330 K, and spanning a broad spectral range from 20 cm-1 to 5500 cm-1. The paper focuses on lattice vibrations…

Strongly Correlated Electrons · Physics 2020-05-20 Birender Singh , M. Vogl , S. Wurmehl , S. Aswartham , B. Büchner , Pradeep Kumar

Neutron scattering has been used to study the structure and spin dynamics of La$_{0.85}$Sr$_{0.15}$MnO$_3$. The magnetic structure of this system is ferromagnetic below T_C = 235 K. We see anomalies in the Bragg peak intensities and new…

Strongly Correlated Electrons · Physics 2009-10-31 L. Vasiliu-Doloc , J. W. Lynn , A. H. Moudden , A. M. de Leon-Guevara , A. Revcolevschi

The interactions among lattice, charge, and spin degrees of freedom fundamentally shape material properties. In FeSe, symmetry-breaking perturbations serve as highly sensitive probes of these couplings. Previous work has shown that defects…

We investigate the evolution of spin and orbital order in undoped LaMnO$_3$ under increasing temperature with a model including both superexchange and Jahn-Teller interactions. We used several cluster mean field calculation schemes and find…

Strongly Correlated Electrons · Physics 2016-12-26 Mateusz Snamina , Andrzej M. Oleś

We present a detailed analysis of light scattering experiments performed on the quarter-filled spin ladder compound $\alpha^\prime$-NaV$_{2}$O$_{5}$ for the temperature range 5 K$\le$T$\le$300 K. This system undergoes a phase transition…

Strongly Correlated Electrons · Physics 2009-10-31 M. Fischer , P. Lemmens , G. Els , G. Güntherodt , E. Sherman , E. Morre , C. Geibel , F. Steglich