Related papers: Rydberg atom mediated polar molecule interactions:…
Proposals for quantum computing using rotational states of polar molecules as qubits have previously considered only diatomic molecules. For these the Stark effect is second-order, so a sizable external electric field is required to produce…
We propose an approach to detect individual Rydberg molecules with each molecule consisting of two atoms in different Rydberg states. The scheme exploits the movement of atoms in the presence of an external force that exerts only on atoms…
Laser cooling and trapping of atomic matter waves in optical potentials has enabled rapid progress in quantum science, particularly when combined with Rydberg excitation of the atoms to induce long-range interactions. Here, we propose the…
Neutral atoms are promising for large-scale quantum computing, but accurate neutral-atom entanglement depends on large Rydberg interactions which strongly limit the interatomic distances. Via a phase accumulation in detuned Rabi cycles…
State-dependent conformational changes play a central role in molecular dynamics, yet they are often difficult to observe or simulate due to their complexity and ultrafast nature. One alternative approach is to emulate such phenomena using…
We study a novel regime of the Rydberg excitation blockade using highly Stark-shifted, yet long-living, states of Rb atoms subject to electric fields above the classical ionization limit. Such states allow tuning the dipole-dipole…
We propose a platform for observing and controlling the interactions between atomic ions and a quantum gas of polar molecules in the ultracold regime. This approach is based on the combination of several recently developed methods in two…
We study the effect of resonances associated with complex molecular interaction of Rydberg atoms on Rydberg blockade. We show that densely-spaced molecular potentials between doubly-excited atomic pairs become unavoidably resonant with the…
Rydberg atoms provide a powerful platform for exploring strongly interacting quantum systems, both in free space and in structured electromagnetic environments, with growing applications in quantum technology. Accurately modeling their…
A remarkable property of Rydberg atoms is the possibility to create molecules formed by one highly excited atom and another atom in the ground state. The first realisation of such a Rydberg molecule has opened an active field of physical…
Cold atoms in highly excited Rydberg states are promising candidates to implement quantum logic gates of a quantum computer via long-range dipole-dipole interaction. Two-qubit gates require a controlled interaction of only two close Rydberg…
We show that with adiabatic passage, one can reliably drive two-photon optical transitions between the ground states and interacting Rydberg states in a pair of atoms. For finite Rydberg interaction strengths a new adiabatic pathway towards…
We explore the possibility of forming a oriented polar molecule directly from a pair of colliding atoms. The process comprises the photoassociation and vibrational stabilization along with the molecular orientation. These processes are…
When ultracold plasma is generated using photonization of laser cooled atoms, some atoms reach only upto Rydberg states. These in turn interact with the free electrons of the plasma and get ionized further. We study the interaction of…
We report the observation of cold Cs Rydberg atom molecules bound at internuclear separations of R~3-9 um. The bound states result from avoided crossings between Rydberg atom pair interaction potentials in an applied electric field. The…
Connectivity has an essential and indispensable role in the cold atom qubit platform. Whilst the two-qubit Rydberg blockade gate recently receives rapid progress on the fidelity side, a pressing challenge is to improve the connectivity in…
Quantum gates and entanglement based on dipole-dipole interactions of neutral Rydberg atoms are relevant to both fundamental physics and quantum information science. The precision and robustness of the Rydberg-mediated entanglement…
The interaction between the electric dipole moment of a trapped molecular ion and the configuration of the confined Coulomb crystal couples the orientation of the molecule to its motion. We consider the practical feasibility of harnessing…
Resonant electric dipole-dipole interactions between cold Rydberg atoms were observed using microwave spectroscopy. Laser-cooled Rb atoms in a magneto-optical trap were optically excited to 45d Rydberg states using a pulsed laser. A…
The ability to control and tune interactions in ultracold atomic gases has paved the way towards the realization of new phases of matter. Whereas experiments have so far achieved a high degree of control over short-ranged interactions, the…