Related papers: Rubidium Rydberg macrodimers
The exceptionally large polarisability of highly excited Rydberg atoms (six orders of magnitude higher than ground-state atoms) makes them of great interest in fields such as quantum optics, quantum computing, quantum simulation and…
Pulsed laser excitation of a dense ultracold Cs vapor has been used to study the pairwise interactions between Cs atoms excited to $n$p$_{3/2}$ Rydberg states of principal quantum numbers in the range $n=22-36$. Molecular resonances were…
Assembled arrays of individual atoms with Rydberg-mediated interactions provide a powerful platform for the simulation of many-body spin Hamiltonians as well as the implementation of universal gate-based quantum information processing. We…
We report a set of adiabatic potential energy surfaces (PESs) for diiodomethane, including the ground electronic state and all excited states accessible via single-photon absorption near 260 nm. Although constrained to four dimensions,…
Ultra-long-range Rydberg molecules (ULRMs) have attracted significant interest due to their unique electronic properties and potential applications in quantum technologies. We theoretically investigate the formation and characteristics of…
We show that the resonant dipole-dipole interaction can give rise to bound states between two and three Rydberg atoms with non-overlapping electron clouds. The dimer and trimer states arise from avoided level crossings between states…
Cold Rydberg atoms are a promising platform for quantum technologies and combining them with optical waveguides has the potential to create robust quantum information devices. Here, we experimentally observe the excitation of cold rubidium…
We characterize the two-photon excitation of an ultracold gas of Rubidium atoms to Rydberg states analysing the induced atomic losses from an optical dipole trap. Extending the duration of the Rydberg excitation to several ms, the ground…
We demonstrate spatially resolved, coherent excitation of Rydberg atoms on an atom chip. Electromagnetically induced transparency (EIT) is used to investigate the properties of the Rydberg atoms near the gold coated chip surface. We measure…
We consider two rubidium atoms, prepared in the same S or P Rydberg states near an optical nanofibre. We determine the van der Waals interaction between them and identify novel features, including the reshaping of the interaction anisotropy…
The Rb-NH interaction is investigated as a prototype for interactions between alkali metal atoms and stable molecules. For spin-aligned Rb and NH that interact on a quartet surface ($^4A''$), the interaction is relatively weak, with a well…
We review experimental and theoretical tools to excite, study and understand strongly interacting Rydberg gases. The focus lies on the excitation of dense ultracold atomic samples close to, or within quantum degeneracy, to high lying…
We show that the dipole-dipole interaction between two Rydberg atoms can give rise to long range molecules. The binding potential arises from two states that converge to different separated atom asymptotes. These states interact weakly at…
Long-range Rydberg molecules (LRMs) form when a highly excited Rydberg electron scatters from ground-state atoms inside its orbit, creating oscillatory, long-range potentials. We present a combined theoretical and experimental study of…
The production of very-high-$n$, $n\sim300$-500, strontium Rydberg atoms is explored using a crossed laser-atom beam geometry. $n$$^{1}$S$_{0}$ and $n$$^{1}$D$_{2}$ states are created by two-photon excitation via the 5s5p $^{1}$P$_{1}$…
The electric dipole moment (EDM) of paramagnetic atoms is sensitive to the intrinsic EDM contribution from that of its constituent electrons and a scalar--pseudo-scalar (S-PS) electron-nucleus interactions. The electron EDM and the S-PS EDM…
We report the observation of cold Cs Rydberg atom molecules bound at internuclear separations of R~3-9 um. The bound states result from avoided crossings between Rydberg atom pair interaction potentials in an applied electric field. The…
We present evidence for Rydberg-Rydberg interaction in a gas of rubidium atoms above room temperature. Rabi oscillations on the nanosecond timescale to different Rydberg states are investigated in a vapor cell experiment. Analyzing the…
Dipole-dipole interactions between helium atoms in Rydberg-Stark states with principal quantum number $n=53$ and approximately linear Stark energy shifts, resulting from induced electric dipole moments of approximately 7900 D, have been…
Precise control and study of molecules is challenging due to the variety of internal degrees of freedom and local coordinates that are typically not controlled in an experiment. Employing quantum gas microscopy to position and resolve the…