Related papers: Ferromagnetically coupled dimers on the distorted …
We present a microscopic model of the spin-gap quantum magnet (CuCl)LaNb2O7 that was previously suggested as a realization of the spin-1/2 frustrated square lattice. Taking advantage of the precise atomic positions from recent crystal…
The ground state (gs) of antiferromagnetically coupled dimers on the Shastry-Sutherland lattice (SSL) stabilizes many exotic phases and has been extensively studied. The gs properties of ferromagnetically coupled dimers on SSL are equally…
We apply neutron diffraction, high-resolution synchrotron x-ray diffraction, magnetization measurements, electronic structure calculations, and quantum Monte-Carlo simulations to unravel the structure and magnetism of (CuCl)LaTa2O7. Despite…
Shastry-Sutherland magnet is a typical frustrated spin system hosting rich phases. While the Heisenberg limit has been extensively studied, the role of spin-orbit coupling is not well explored. Motivated by newly discovered rare-earth…
Using inelastic neutron scattering, x-ray, neutron diffraction, and the first-principle calculation techniques, we show that the crystal structure of the two-dimensional quantum spin system (CuCl)LaNb$_2$O$_7$ is orthorhombic with $Pbam$…
We consider the zero-temperature properties of the spin-half two-dimensional Shastry-Sutherland antiferromagnet by using a high-order coupled cluster method (CCM) treatment. We find that this model demonstrates various groundstate phases…
The Shastry-Sutherland model, which consists of a set of spin 1/2 dimers on a 2-dimensional square lattice, is simple and soluble, but captures a central theme of condensed matter physics by sitting precariously on the quantum edge between…
We present the magnetic properties of a strongly spin-orbit coupled quantum dimer magnet based on Co$^{2+}$. The metal-organic framework compound Co$_2$(BDC)$_2$(DPTTZ)$_2$$\cdot$DMF features Co$^{2+}$ dimers arranged nearly orthogonal to…
We study possible paramagnetic phases of antiferromagnets on the Shastry-Sutherland lattice by a gauge-theoretic analysis of fluctuations in a theory with Sp(2N) symmetry. In addition to the familiar dimer phase, we find a confining phase…
We report a comprehensive study on the origin of the enigmatic disordered ground state within the Shastry-Sutherland lattice, BaCe$_2$ZnS$_5$, at low temperatures. The magnetization and heat capacity data show a lack of magnetic ordering…
The ground state of the square lattice bilayer quantum antiferromagnet with nearest ($J_1$) and next-nearest ($J_2$) neighbour intralayer interaction is studied by means of the dimer expansion method up to the 6-th order in the interlayer…
We look into the quantum phase diagram of a spin-$\frac{1}{2}$ antiferromagnet on the square lattice with degenerate Shastry-Sutherland ground states, for which only a schematic phase diagram is known so far. Many exotic phases were…
The study of interacting spin systems is of fundamental importance for modern condensed matter physics. On frustrated lattices, magnetic exchange interactions cannot be simultaneously satisfied, and often give rise to competing exotic…
We report muon spin relaxation ($\mu$SR) and magnetic susceptibility measurements on Cu(Cl,Br)La(Nb,Ta)$_{2}$O$_{7}$, which demonstrate: (a) the absence of static magnetism in (CuCl)LaNb$_{2}$O$_{7}$ down to 15 mK confirming a spin-gapped…
The quantum dimer magnet (QDM) is the canonical example of quantum magnetism. The QDM state consists of entangled nearest-neighbor spin dimers and often exhibits a field-induced triplon Bose-Einstein condensate (BEC) phase. We report on a…
We present high-resolution measurements of the thermal expansion and the magnetostriction of TlCuCl$_{3}$ which shows field-induced antiferromagnetic order. We find pronounced anomalies in the field and temperature dependence of different…
We report magnetization, nuclear magnetic resonance (NMR), nuclear quadrupole resonance (NQR), and transmission electron microscopy (TEM) studies on the quasi-two-dimensional spin-gap system (CuCl)LaNb2O7, a possible candidate for the J1-J2…
We study the ground-state phase diagram of a Heisenberg model with spin $S=\frac{1}{2}$ on a diamond-like decorated square lattice. A diamond unit has two types of antiferromagnetic exchange interactions, and the ratio $\lambda$ between the…
We investigate the ground-state phase diagram of a spin-1/2 honeycomb-lattice antiferromagnetic (AF) Heisenberg model with three exchange interactions, $J_{\rm A}$, $J_{\rm B}$, and $J_{\rm C}$ that is realized in a distorted…
Sr$_{3}$Cr$_{2}$O$_{8}$ consist of a lattice of spin-1/2 Cr$^{5+}$ ions, which form hexagonal bilayers and which are paired into dimers by the dominant antiferromagnetic intrabilayer coupling. The dimers are coupled three-dimensionally by…