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The morphological scaling properties of linear polymer films grown by vapor deposition polymerization (VDP) are studied by 1+1D Monte Carlo simulations. The model implements the basic processes of random angle ballistic deposition ($F$),…

Computational Physics · Physics 2010-10-25 Sairam Tangirala , David P. Landau , Y. -P. Zhao

Scaling predictions and results from self-consistent field calculations for bottle-brush polymers with a rigid backbone and flexible side chains under good solvent conditions are summarized and their validity and applicability is assessed…

Soft Condensed Matter · Physics 2007-11-26 Hsiao-Ping Hsu , Wolfgang Paul , Kurt Binder

We determine the distribution of free ends and the monomer insertion potential in the strongly-stretched limit for regularly and statistically branched polymer brushes. We find that the end density flattens in the limit of very strong…

Soft Condensed Matter · Physics 2015-07-14 Daniel O. LeSher , Grant L Metheny , Galen T. Pickett

An innovative method is proposed to generate configurations of coarse grained models for polymer melts. This method, largely inspired by chemical ``radical polymerization'', is divided in three stages: (i) nucleation of radicals (reacting…

Statistical Mechanics · Physics 2007-12-24 Fabien Leonforte , Michel Perez , Olivier Lame , Jena-Louis Barrat

We use computer simulations to investigate the stability of a two-component polymer brush de-mixing on a curved template into phases of different morphological properties. It has been previously shown via molecular dynamics simulations that…

Soft Condensed Matter · Physics 2015-06-03 William L. Miller , Behnaz Bozorgui , Katherine Klymko , Angelo Cacciuto

Ordering nanoparticles into a desired super-structure is often crucial for their technological applications. We use molecular dynamics simulations to study the assembly of nanoparticles in a polymer brush randomly grafted to a planar…

Soft Condensed Matter · Physics 2017-12-11 Shengfeng Cheng , Mark J. Stevens , Gary S. Grest

The reaction of $AB_m$ monomers (m=2,3) with a multifunctional B_f-type polymer chain ("hypergrafting") is studied by coarse-grained molecular dynamics simulations. The $AB_m$ monomers are hypergrafted using the slow monomer addition…

Soft Condensed Matter · Physics 2015-11-09 Hauke Rabbel , Holger Frey , Friederike Schmid

Polymer-grafted nanoparticles (PGNPs) can provide property profiles than cannot be obtained individually by polymers or nanoparticles (NPs). Here, we have studied the mixing--demixing transition of symmetric copolymer melts of…

Soft Condensed Matter · Physics 2020-01-23 Peter Yatsyshin , Nikolaos G. Fytas , Panagiotis E. Theodorakis

Simple homogeneous shear flows of frictionless, deformable particles are studied by particle simulations at large shear rates and for differently soft, deformable particles. The particle stiffness sets a time-scale that can be used to scale…

Soft Condensed Matter · Physics 2024-07-25 Dalila Vescovi , Stefan Luding

A simple application of classical density functional theory is derived and applied to a system of polymers grafted to a plane. The system is assumed to have symmetry in directions parallel to the grafting plane hence it being a…

Soft Condensed Matter · Physics 2016-12-02 Luke Kristopher Davis

Motivated by recent nanofluidics experiments, we use Brownian dynamics and Monte Carlo simulations to study the conformation, organization and dynamics of two polymer chains confined to a single box-like cavity. The polymers are modeled as…

Soft Condensed Matter · Physics 2021-05-19 James M. Polson , Desiree A. Rehel

Ring, or cyclic, polymers have unique properties compared to linear polymers, due to their topologically closed structure that has no beginning or end. Experimental measurements on molecular ring polymers are challenging due to their…

Soft Condensed Matter · Physics 2023-03-15 Ruben Verweij , Julio Melio , Indrani Chakraborty , Daniela J Kraft

Ladder polymers, known for their rigid, ladder-like structures, exhibit exceptional thermal stability and mechanical strength, positioning them as candidates for advanced applications. However, accurately determining their structure from…

Soft Condensed Matter · Physics 2025-05-23 Lijie Ding , Chi-Huan Tung , Zhiqiang Cao , Zekun Ye , Xiaodan Gu , Yan Xia , Wei-Ren Chen , Changwoo Do

We have generalized the Edwards' method of collective description of dense polymer systems in terms of effective potentials to polymer blends in the presence of a surface. With this method we have studied conformationally asymmetric…

Soft Condensed Matter · Physics 2009-11-11 Semjon Stepanow , Andrei A. Fedorenko

Recent developments of microscopic mechanical experiments allow the manipulation of individual polymer molecules in two main ways: \textit{uniform} stretching by external forces and \textit{non-uniform} stretching by external fields. Many…

Biological Physics · Physics 2015-06-11 Fabio Manca , Stefano Giordano , Pier Luca Palla , Fabrizio Cleri , Luciano Colombo

Collapse of the polymer chain upon the sharp decrease of solvent quality is studied. During collapse, any pair of polymer units appearing in a sufficiently close vicinity in space has the possibility with a certain probability to form an…

Soft Condensed Matter · Physics 2019-11-07 A. M. Astakhov , S. K. Nechaev , K. E. Polovnikov

We present a Monte Carlo algorithm that provides efficient and unbiased sampling of polymer melts consisting of two chains of equal length that jointly visit all the sites of a cubic lattice with rod geometry L x L x rL and non-periodic…

Statistical Mechanics · Physics 2010-11-03 Jesper Lykke Jacobsen

We describe a microscope-based optical setup that allows us to perform space-and time-resolved measurements of the spectral reflectance of transparent substrates coated with ultrathin films. This technique is applied to investigate the…

Soft Condensed Matter · Physics 2016-03-25 Siddhartha Varma , Lionel Bureau , Delphine Débarre

We consider flexible branched polymer, with quenched branch structure, and show that its conformational entropy as a function of its gyration radius $R$, at large $R$, obeys, in the scaling sense, $\Delta S \sim R^2/(a^2L)$, with $a$ bond…

Statistical Mechanics · Physics 2015-09-02 Alexander Y. Grosberg , Sergei K. Nechaev

The process of adsorption on a planar repulsive, "marginal" and attractive wall of long-flexible polymer chains with excluded volume interactions is investigated. The performed scaling analysis is based on formal analogy between the polymer…

Soft Condensed Matter · Physics 2009-10-08 Z. Usatenko
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