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Radiative emission during cold collisions between trapped laser-cooled Rb atoms and alkaline-earth ions (Ca$^+$, Sr$^+$, Ba$^+$) and Yb$^+$, and between Li and Yb$^+$, are studied theoretically, using accurate effective-core-potential based…

Atomic Physics · Physics 2015-06-23 Humberto Da Silva , Maurice Raoult , Mireille Aymar , Olivier Dulieu

We explore the feasibility of producing ultracold diatomic molecules with nonzero electric and magnetic dipole moments by magnetically associating two atoms, one with zero electron spin and one with nonzero spin. Feshbach resonances arise…

Atomic Physics · Physics 2013-05-28 Daniel A. Brue , Jeremy M. Hutson

We report on photoassociation (PA) spectroscopy of a degenerate Fermi gas of $^{173}$Yb atoms near the dissociation limit of the spin-forbidden ${^1}S_0-{^3}P_1$ intercombination transition. An atom-loss spectrum is measured from a trapped…

Atomic Physics · Physics 2018-01-10 Jeong Ho Han , Jin Hyoun Kang , Moosong Lee , Yong-il Shin

The creation of ultracold molecules is currently limited to diatomic species. In this letter we present a theoretical description of the photoassociation of ultracold atoms and molecules to create ultracold excited triatomic molecules, thus…

Atomic Physics · Physics 2015-09-02 Jesús Pérez-Ríos , Maxence Lepers , Olivier Dulieu

We generalize the idea of chainwise stimulated Raman adiabatic passage (STIRAP) [Kuznetsova \textit{et al.} Phys. Rev. A \textbf{78}, 021402(R) (2008)] to a photoassociation-based chainwise atom-molecule system, with the goal of directly…

Quantum Gases · Physics 2015-05-18 Jing Qian , Weiping Zhang , Hong Y. Ling

We consider the magnetically tunable Feshbach resonances that may exist in ultracold mixtures of molecules in $^2\Sigma$ states and alkali-metal atoms. We focus on Rb+CaF as a prototype system. There are likely to be Feshbach resonances…

Atomic Physics · Physics 2023-06-05 Robert C. Bird , Michael R. Tarbutt , Jeremy M. Hutson

We consider performing adiabatic rapid passage (ARP) using frequency-swept driving pulses to excite a collection of interacting two-level systems. Such a model arises in a wide range of many-body quantum systems, such as cavity QED or…

Mesoscale and Nanoscale Physics · Physics 2012-08-21 R. T. Brierley , C. Creatore , P. B. Littlewood , P. R. Eastham

Ultracold metastable RbCs molecules are observed in a double species MOT through photoassociation near the Rb(5S$_{1/2}$)+Cs(6P$_{3/2}$) dissociation limit followed by radiative stabilization. The molecules are formed in their lowest…

Atomic Physics · Physics 2017-09-13 C. Gabbanini , O. Dulieu

We have produced ultracold heteronuclear YbRb$^*$ molecules in a combined magneto-optical trap by photoassociation. The formation of electronically excited molecules close to the dissociation limit was observed by trap loss spectroscopy in…

Quantum Physics · Physics 2016-01-20 N. Nemitz , F. Baumer , F. Münchow , S. Tassy , A. Görlitz

We study ultracold long-range collisions of heteronuclear alkali-metal dimers with a reservoir gas of alkali-metal Rydberg atoms in a two-photon laser excitation scheme. In a low density regime where molecules remain outside the Rydberg…

Atomic Physics · Physics 2021-09-15 Vanessa Olaya , Jesús Pérez-Ríos , Felipe Herrera

Photoassociation (PA) of ultracold metastable helium to the 2s2p manifold is theoretically investigated using a non-perturbative close-coupled treatment in which the laser coupling is evaluated without assuming the dipole approximation. The…

Atomic Physics · Physics 2015-05-14 Daniel G. Cocks , Ian B. Whittingham

We present a simple technique for studying collisions of ultracold atoms in the presence of a magnetic field and radio-frequency radiation (rf). Resonant control of scattering properties can be achieved by using rf to couple a colliding…

Quantum Gases · Physics 2010-09-28 Thomas M. Hanna , Eite Tiesinga , Paul S. Julienne

We report the observation of microwave coherent control of rotational states of ultracold $^{85}$Rb$^{133}$Cs molecules formed in their vibronic ground state by short-range photoassociation. Molecules are formed in the single rotational…

Atomic Physics · Physics 2020-07-10 Zhonghua Ji , Ting Gong , Yonglin He , Jeremy M. Hutson , Yanting Zhao , Liantuan Xiao , Suotang Jia

Photoassociation of ultracold atoms induced by chirped picosecond pulses is analyzed in a non-perturbative treatment by following the wavepackets dynamics on the ground and excited surfaces. The initial state is described by a Boltzmann…

Atomic and Molecular Clusters · Physics 2009-06-10 Eliane Luc-Koenig , Mihaela Vatasescu , Francoise Masnou-Seeuws

Exact and asymptotic lineshape expressions are derived from the semi-classical density matrix representation describing a set of closed three-level atomic or molecular states including decoherences, relaxation rates and light-shifts. An…

Atomic Physics · Physics 2012-11-22 Thomas Zanon , Emeric de Clercq , Ennio Arimondo

Ultracold collisions of cold atoms or molecules make the bound states of the collision complex formed from the two colliding species accessible for control and manipulation of the cold species or the complex. Such resonances are best…

Atomic Physics · Physics 2015-05-13 Paul S. Julienne

The influence of a tight isotropic harmonic trap on photoassociation of two ultracold alkali atoms forming a homonuclear diatomic is investigated using realistic atomic interaction potentials. Confinement of the initial atom pair due to the…

Quantum Physics · Physics 2009-11-13 Sergey Grishkevich , Alejandro Saenz

A broadband technique for robust adiabatic rotation and conversion of light polarization is proposed. It uses the analogy between the equation describing the polarization state of light propagating through an optically anisotropic medium…

Quantum Physics · Physics 2010-10-15 U. Gaubatz , A. A. Rangelov , N. V. Vitanov

Mergoassociation of two ultracold atoms to form a weakly bound molecule can occur when two optical traps that each contain a single atom are merged. Molecule formation occurs at an avoided crossing between a molecular state and the lowest…

Atomic Physics · Physics 2023-10-04 Robert C. Bird , C. Ruth Le Sueur , Jeremy M. Hutson

Motivated by the recent experimental developments on ultracold molecules and atoms, we propose a simplest theoretical model to address the disassociation, reflection and transmission probability of a 1-dimensional cold molecule via quantum…

Quantum Gases · Physics 2023-07-13 Wen-Liang Li , Hai-Jing Song , Tie-Ling Song , D. L. Zhou