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Since the 1970s, spin-selective reactions of radical pairs have been modelled theoretically by adding phenomenological rate equations to the quantum mechanical equation of motion of the radical pair spin density matrix. Here, using a…

Quantum Physics · Physics 2010-03-04 Jonathan A. Jones , Peter J. Hore

Recently, spin-selective radical pair reactions have been studied using concepts from quantum measurement theory. In this Article, we show that the approach taken by Kominis (Physical Review E, 83, 2011, 056118) leads to erroneous results…

Quantum Physics · Physics 2011-10-12 Alpha Lee

Spin-selective reactions of radical pairs have traditionally been modelled theoretically by adding phenomenological rate equations to the quantum mechanical equation of motion of the radical pair spin density matrix. More recently an…

Quantum Physics · Physics 2011-05-03 Jonathan A. Jones , Kiminori Maeda , Peter J. Hore

The so-called "phenomenological" kinetic equation for one-pair density operator for spin-selective reactions is defended. We derive this equation from the kinetic equation for density operator of all pairs which are treated as singlet and…

Quantum Physics · Physics 2013-04-24 Leonid V. Il'ichov , Sergey V. Anishchik

It is shown that the Jones-Hore theory is either inconsistent or cannot describe single-molecule experiments.

Quantum Physics · Physics 2015-05-28 I. K. Kominis

Radical-ion-pair reactions were recently shown to represent a rich biophysical laboratory for the application of quantum measurement theory methods and concepts. We here show that radical-ion-pair reactions essentially form a non-linear…

Quantum Physics · Physics 2015-05-19 I. K. Kominis

Radical-ion-pair reactions were recently shown to represent a rich biophysical laboratory for the application of quantum measurement theory methods and concepts, casting doubt on the validity of the theoretical treatment of these reactions…

Quantum Physics · Physics 2010-09-16 I. K. Kominis

Radical pair recombination reactions are normally described using a quantum mechanical master equation for the electronic and nuclear spin density operator. The electron spin state selective (singlet and triplet) recombination processes are…

Chemical Physics · Physics 2018-08-10 Thomas P. Fay , Lachlan P. Lindoy , David E. Manolopoulos

Radical pairs and the dynamics they undergo are prevalent in many chemical and biological systems. Specifically, it has been proposed that the radical pair mechanism results from a relatively strong hyperfine interaction with its intrinsic…

Quantum Physics · Physics 2021-03-26 Amit Finkler , Durga Dasari

Radical-ion-pair reactions were recently shown to represent a rich biophysical laboratory for the application of quantum measurement theory methods and concepts. We here propose a concrete experimental test that can clearly discriminate…

Quantum Physics · Physics 2015-05-30 A. T. Dellis , I. K. Kominis

Magnetic field effects on radical pair reactions arise due to the interplay of coherent electron spin dynamics and spin relaxation effects, a rigorous treatment of which requires the solution of the Liouville-von Neumann equation. However,…

Chemical Physics · Physics 2019-04-22 Thomas P Fay , David E Manolopoulos

Radical-ion pairs and their reactions have triggered the study of quantum effects in biological systems. This is because they exhibit a number of effects best understood within quantum information science, and at the same time are central…

Quantum Physics · Physics 2017-04-06 K. M. Vitalis , I. K. Kominis

We review and compare several measures that identify quantum states that are "macroscopically quantum". These measures were initially formulated either for photonic systems or spin ensembles. Here, we compare them through a simple model…

Quantum Physics · Physics 2014-12-04 F. Fröwis , N. Sangouard , N. Gisin

We use a simple example to illustrate why it is not possible to consider that a measurement reveals an underlying objective reality of a property of a quantum system, that continues the same after the measurement is performed. This kind of…

Quantum Physics · Physics 2020-07-06 Pablo L. Saldanha

We provide optimal measurement schemes for estimating relative parameters of the quantum state of a pair of spin systems. We prove that the optimal measurements are joint measurements on the pair of systems, meaning that they cannot be…

Quantum Physics · Physics 2007-05-23 Stephen D. Bartlett , Terry Rudolph , Robert W. Spekkens

The usual conjectures of quantum measurements approaches, inspired from the traditional interpretation of Heisenberg's ("uncertainty") relations, are proved as being incorrect. A group of reconsidered conjectures and a corresponding new…

Quantum Physics · Physics 2007-05-23 Spiridon Dumitru

Assuming a well-behaving quantum-to-classical transition, measuring large quantum systems should be highly informative with low measurement-induced disturbance, while the coupling between system and measurement apparatus is "fairly simple"…

Quantum Physics · Physics 2017-07-19 Tomer Jack Barnea , Marc-Olivier Renou , Florian Fröwis , Nicolas Gisin

For theoretical approach of quantum measurements it is proposed a set of reconsidered conjectures. The proposed approach implies linear functional transformations for probability density and current but preserves the expressions for…

Quantum Physics · Physics 2007-05-23 S. Dumitru

Quantum mechanics dictates that a continuous measurement of the position of an object imposes a random back action perturbation on its momentum. This randomness translates with time into position uncertainty, thus leading to the well known…

Quantum metrology makes use of coherent superpositions to detect weak signals. While in principle the sensitivity can be improved by increasing the density of sensing particles, in practice this improvement is severely hindered by…

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