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Magnetic properties of the natural mineral Cu$_2$(OH)$_2$CO$_3$ (malachite) were investigated through DC and AC susceptibility measurements. The analysis of the low-temperature part reveals a quantum spin-gap behavior with $\Delta \approx…

Strongly Correlated Electrons · Physics 2009-10-31 E. Janod , L. Leonyuk , V. Maltsev

Spin-1/2 kagome-lattice Heisenberg antiferromagnet is theoretically known to have a quantum spin liquid ground state, one of the frontiers of condensed matter physics. The search for the model substances has been continued for a long time,…

Strongly Correlated Electrons · Physics 2024-08-21 Hidekazu Tanaka

The magnetic ground-state of copper metaborate is investigated by means of elastic neutron scattering.The magnetic structure of CuB2O4 is incommensurate with respect to the chemical lattice at T=1.8K and undergoes a continuous phase…

Strongly Correlated Electrons · Physics 2009-01-23 B. Roessli , J. Schefer , G. Petrakovskii , B. Ouladdiaf , M. Boehm , U. Staub , A. Vorontinov , L. Bezmaternikh

We report the magnetic susceptibility and the low-temperature specific heat of a double perovskite compound, Sr2CuTeO6, which is expected as the spin-1/2 square-lattice Heisenberg antiferromagnet with nearest-neighbor J1 and…

Strongly Correlated Electrons · Physics 2015-06-23 Tomoyuki Koga , Nobuyuki Kurita , Hidekazu Tanaka

We investigate the structural, electronic and magnetic properties of the newly synthesized mineral barlowite Cu4(OH)6FBr which contains Cu2+ ions in a perfect kagome arrangement. In contrast to the spin-liquid candidate herbertsmithite…

We report the isolation of thin flakes of cylindrite, a naturally occurring van der Waals superlattice, by means of mechanical and liquid phase exfoliation. We find that this material is a heavily doped p-type semiconductor with a narrow…

Search for a new quantum state of matter emerging in a crystal is one of recent trends in condensed matter physics. For magnetic materials, geometrical frustration and high magnetic field are two key ingredients to realize it: a…

Strongly Correlated Electrons · Physics 2019-03-19 R. Okuma , D. Nakamura , T. Okubo , A. Miyake , A. Matsuo , K. Kindo , M. Tokunaga , N. Kawashima , S. Takeyama , Z. Hiroi

Materials with a perfect kagome lattice structure of magnetic ions are intensively sought for, because they may exhibit exotic ground states like the a quantum spin liquid phase. Barlowite is a natural mineral that features perfect kagome…

Strongly Correlated Electrons · Physics 2016-09-22 Daniel Guterding , Roser Valenti , Harald O. Jeschke

We synthesized single crystals of the new hexagonal compounds A$_2$Cu$_3$SnF$_{12}$ with A=Cs and Rb, and investigated their magnetic properties. These compounds are composed of Kagom\'{e} layers of corner-sharing CuF$_6$-octahedra.…

Strongly Correlated Electrons · Physics 2009-11-13 T. Ono , K. Morita , M. Yano , H. Tanaka , K. Fujii , H. Uekusa , Y. Narumi , K. Kindo

We have investigated the magnetic properties of a non-symmorphic correlated material, TbAgSb2. It consists of a quasi-two-dimensional structure of Sb atoms which hosts topologically non-trivial fermions. We prepared high quality single…

Strongly Correlated Electrons · Physics 2024-10-04 Saswata Halder , Kalobaran Maiti

A two-staged, uniaxial magnetoresistive effect has been discovered in SrCo6O11 having a layered hexagonal structure. Conduction electrons and localized Ising spins are in different sublattices but their interpenetration makes the conduction…

Strongly Correlated Electrons · Physics 2009-11-13 S. Ishiwata , I. Terasaki , F. Ishii , N. Nagaosa , H. Mukuda , Y. Kitaoka , T. Saito , M. Takano

Magnetization and specific heat measurements have been carried out on Cs$_2$Cu$_3$ZrF$_{12}$ and Cs$_2$Cu$_3$HfF$_{12}$ single crystals, in which Cu$^{2+}$ ions with spin-1/2 form a regular Kagom\'{e} lattice. The antiferromagnetic exchange…

Strongly Correlated Electrons · Physics 2015-06-25 Y. Yamabe , T. Ono , T. Suto , H. Tanaka

We study magnetism on the fcc lattice with tetragonal distortions, with general exotic directional magnetic interactions allowed by symmetry. We consider two models, corresponding to a uniform tetragonal distortion, or a two-sublattice…

Strongly Correlated Electrons · Physics 2014-12-05 Hiroaki Ishizuka , Leon Balents

We study thermodynamic properties of an antiferromagnetic Ising model on the inverse perovskite lattice by using Monte Carlo simulations. The lattice structure is composed of corner-sharing octahedra and contains three-dimensional…

Statistical Mechanics · Physics 2007-05-23 Daisuke Tahara , Yukitoshi Motome , Masatoshi Imada

We report the synthesis, crystal structure, and magnetic properties of two new quantum antiferromagnets A3ReO5Cl2 (A = Sr and Ba). The crystal structure is isostructural with the mineral pinalite Pb3WO5Cl2, in which the Re6+ ion is…

Strongly Correlated Electrons · Physics 2021-04-06 Daigorou Hirai , Takeshi Yajima , Kazuhiro Nawa , Mitsuaki Kawamura , Zenji Hiroi

We study polycrystalline samples of KCu3As2O7(OH)3, a new candidate spin-1/2 kagome antiferromagnet, by magnetic susceptibility and heat capacity measurements above 2 K. The unique arrangement of the 3z2 - r2 and x2 - y2 orbitals on the…

Materials Science · Physics 2015-06-04 Yoshihiko Okamoto , Hajime Ishikawa , Gøran J. Nilsen , Zenji Hiroi

Magnetism of layered cobaltites Na$_x$CoO$_2$ with $x$ = 0.6 and 0.9 has been investigated by a positive muon spin rotation and relaxation ($\mu^+$SR) spectroscopy together with magnetic susceptibility and specific heat measurements, using…

Strongly Correlated Electrons · Physics 2009-11-10 J. Sugiyama , J. H. Brewer , E. J. Ansaldo , B. Hitti , M. Mikami , Y. Mori , T. Sasaki

Dielectric study on Ca3Mn2O7 features relaxor-like segmented dynamics below the antiferromagnetic ordering. Dipolar relaxations of different origin are spectrally resolved exhibiting distinct H-field alterations. This identifies their…

Materials Science · Physics 2019-09-10 Pooja Sahlot , Gaurav Sharma , Vasant Sathe , Anand Mohan Awasthi

Based on the first-principles evolutionary materials design, we report a stable boron Kagome lattice composed of triangles in triangles on a two-dimensional sheet. The Kagome lattice can be synthesized on a silver substrate, with selecting…

Materials Science · Physics 2019-08-01 Sunghyun Kim , W. H. Han , In-Ho Lee , K. J. Chang

For temperatures T well above the ordering temperature T*=3.0+-0.2K the magnetic properties of the metal-organic material Mn[C10H6(OH)(COO)]2x2H20 built from Mn^2+ ions and 3-hydroxy-2-naphthoic anions can be described by a S=5/2 quantum…