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We propose and experimentally demonstrate a method to strongly increase the sensitivity of spin measurements on nitrogen-vacancy (NV) centers in diamond, which can be readily implemented in existing quantum sensing experiments. While charge…

Shallow Nitrogen-Vacancy (NV) centers are promising candidates for high-precision sensing applications; these defects, when positioned a few nanometers below the surface, provide an atomic-scale resolution along with substantial…

The Zeeman splitting of a localized single spin can be used to construct a magnetometer allowing high precision measurements of magnetic fields with almost atomic spatial resolution. While sub-{\mu}T sensitivity can in principle be obtained…

Instrumentation and Detectors · Physics 2011-01-28 Rolf Simon Schoenfeld , Wolfgang Harneit

Time-resolved magnetic sensing is of great importance from fundamental studies to applications in physical and biological sciences. Recently the nitrogen-vacancy (NV) defect center in diamond has been developed as a promising sensor of…

Nitrogen vacancy (NV) centers in diamond have been used as ultrasensitive magnetometers to perform nuclear magnetic resonance (NMR) spectroscopy of statistically polarized samples at 1 - 100 nm length scales. However, the spectral linewidth…

The measurement of vector magnetic fields with high sensitivity and spatial resolution is important for both fundamental science and engineering applications. In particular, magnetic-field sensing with nitrogen-vacancy (NV) centers in…

Quantum Physics · Physics 2023-07-12 Takuya Isogawa , Yuichiro Matsuzaki , Junko Ishi-Hayase

Sensing vector magnetic fields is critical to many applications in fundamental physics, bioimaging, and material science. Magnetic-field sensors exploiting nitrogen-vacancy (NV) centers are particularly compelling as they offer high…

Methods and techniques to measure and image beyond the state-of-the-art have always been influential in propelling basic science and technology. Because current technologies are venturing into nanoscopic and molecular-scale fabrication,…

Quantum Physics · Physics 2015-05-13 Andrii Lazariev , Gopalakrishnan Balasubramanian

We describe a real-time data processing and frequency control method to track peaks in optically detected magnetic resonance of nitrogen-vacancy centers in diamond. This procedure allows us to measure magnetic field continuously with…

Mesoscale and Nanoscale Physics · Physics 2019-02-19 Kapildeb Ambal , Robert D. McMichael

We present a protocol that detects molecular conformational changes with two nitroxide electron-spin labels and a nitrogen-vacancy (NV) center in diamond. More specifically, we demonstrate that the NV can detect energy shifts induced by the…

Quantum Physics · Physics 2022-12-21 C. Munuera-Javaloy , R. Puebla , B. D'Anjou , M. B. Plenio , J. Casanova

We demonstrate a robust, scale-factor-free vector magnetometer, which uses a closed-loop frequency-locking scheme to simultaneously track Zeeman-split resonance pairs of nitrogen-vacancy (NV) centers in diamond. Compared with open-loop…

Quantum Physics · Physics 2018-08-01 Hannah Clevenson , Linh M. Pham , Carson Teale , Kerry Johnson , Dirk Englund , Danielle Braje

Precise coherent control of the individual electronic spins associated with atom-like impurities in the solid state is essential for applications in quantum information processing and quantum metrology. We demonstrate all-optical…

Quantum Physics · Physics 2015-03-05 Yiwen Chu , Matthew Markham , Daniel J. Twitchen , Mikhail D. Lukin

Precise control of the resonant frequency of a spin qubit is of fundamental importance to quantum sensing protocols. We demonstrate a control technique on a single nitrogen-vacancy (NV) centre in diamond where the applied magnetic field is…

The implementation of nuclear magnetic resonance (NMR) at the nanoscale is a major challenge, as conventional systems require relatively large ensembles of spins and limit resolution to mesoscopic scales. New approaches based on quantum…

Optically-detected paramagnetic centers in wide-bandgap semiconductors are emerging as a promising platform for nanoscale metrology at room temperature. Of particular interest are applications where the center is used as a probe to…

Mesoscale and Nanoscale Physics · Physics 2015-12-09 Abdelghani Laraoui , Daniela Pagliero , Carlos A. Meriles

We utilize nonlinear absorption to design all-optical protocols that improve both charge state initialization and spin readout for the nitrogen-vacancy (NV) center in diamond. Non-monotonic variations in the equilibrium charge state as a…

Quantum Physics · Physics 2016-12-14 David A. Hopper , Richard R. Grote , Annemarie L. Exarhos , Lee C. Bassett

The negatively charged tin-vacancy center in diamond (SnV$^-$) is an emerging platform for building the next generation of long-distance quantum networks. This is due to the SnV$^-$'s favorable optical and spin properties including bright…

Biocompatible nanoscale probes for sensitive detection of paramagnetic species and molecules associated with their (bio)chemical transformations would provide a desirable tool for a better understanding of cellular redox processes. Here, we…

A nitrogen-vacancy (NV) center in diamond is a promising sensor for nanoscale magnetic sensing. Here we report electron spin resonance (ESR) spectroscopy using a single NV center in diamond. First, using a 230 GHz ESR spectrometer, we…

Mesoscale and Nanoscale Physics · Physics 2016-10-05 Chathuranga Abeywardana , Viktor Stepanov , Franklin H. Cho , Susumu Takahashi

We demonstrate a spin-based, all-dielectric electrometer based on an ensemble of nitrogen-vacancy (NV$^-$) defects in diamond. An applied electric field causes energy level shifts symmetrically away from the NV$^-$'s degenerate triplet…