English
Related papers

Related papers: Core-softened Fluids, Water-like Anomalies and the…

200 papers

Water is an unique material with a long list of thermodynamic, dynamic and structural anomalies, which are usually attributed to the competition between two characteristic length scales in the intermolecular interaction. It has been argued…

Statistical Mechanics · Physics 2021-06-25 Murilo S. Marques , Vinicius Fonseca Hernandes , Enrique Lomba , J. Rafael Bordin

2D competitive systems shows a large variety of solid and aggregate patterns, re-entrant fluid phase, a continuous melting as predicted by the KTHNY theory and, in some cases, waterlike anomalies. In this paper, we employ Langevin Dynamics…

Linearly-sloped or `ramp' potentials belong to a class of core-softened models which possess a liquid-liquid critical point (LLCP) in addition to the usual liquid-gas critical point. Furthermore they exhibit thermodynamic anomalies in the…

Statistical Mechanics · Physics 2009-11-11 Helen M. Gibson , Nigel B. Wilding

In this work, a two dimensional system of polymer grafted nanoparticles is analyzed using large-scale Langevin Dymanics simulations. Effective core-softened potentials were obtained for two cases: one where the polymers are free to rotate…

Soft Condensed Matter · Physics 2021-06-25 Murilo S. Marques , Thiago P. Nogueira , Marcia C. Barbosa , José Rafael Bordin

The thermodynamic behavior of a fluid near a vapor-liquid and, hence, asymmetric critical point is discussed within a general ``complete'' scaling theory incorporating pressure mixing in the nonlinear scaling fields as well as corrections…

Statistical Mechanics · Physics 2009-11-07 Young C. Kim , Michael E. Fisher , G. Orkoulas

We study fluid structure and water-like anomalies of a system constituted by dimeric particles interacting via a purely repulsive core-softened potential by means of integral equation theories. In our model, dimers interact through a…

Soft Condensed Matter · Physics 2017-03-08 Gianmarco Munaò , Franz Saija

It is well known that some liquids can demonstrate anomalous behavior. Interestingly, this be- havior can be qualitatively reproduced with simple core-softened isotropic pair-potential systems. Although anomalous properties of liquids…

Statistical Mechanics · Physics 2015-07-15 Eu. A. Gaiduk , Yu. D. Fomin , V. N. Ryzhov , E. N. Tsiok , V. V. Brazhkin

A core-softened model of a glass forming fluid is numerically studied in the limit of very low temperatures. The model shows two qualitatively different behaviors depending on the strength of the attraction between particles. For no or low…

Statistical Mechanics · Physics 2009-11-07 E. A. Jagla

Compressing or cooling a fluid typically enhances its static interparticle correlations. However, there are notable exceptions. Isothermal compression can reduce the translational order of fluids that exhibit anomalous waterlike trends in…

Soft Condensed Matter · Physics 2008-04-11 William P. Krekelberg , Jeetain Mittal , Venkat Ganesan , Thomas M. Truskett

Using event driven molecular dynamics simulations, we study a three dimensional one-component system of spherical particles interacting via a discontinuous potential combining a repulsive square soft core and an attractive square well. In…

Soft Condensed Matter · Physics 2009-11-10 A. Skibinsky , S. V. Buldyrev , G. Franzese , G. Malescio , H. E. Stanley

We use Molecular Dynamics simulations to study how the nanopore and the fluid structures affects the dynamic, thermodynamic and structural properties of a confined anomalous fluid. The fluid is modeled using an effective pair potential…

Soft Condensed Matter · Physics 2015-06-23 Leandro B. Krott , José Rafael Bordin , Ney Marçal Barraz , Marcia C. Barbosa

Molecular dynamics simulations and instantaneous normal mode (INM) analysis of a fluid with core-softened pair interactions and water-like liquid-state anomalies are performed to obtain an understanding of the relationship between…

Soft Condensed Matter · Physics 2015-05-18 Alan Barros de Oliveira , Evy A. Salcedo Torres , Charusita Chakravarty , Marcia C. Barbosa

Using molecular dynamics we studied the role of the anisotropy on the phase boundary and on the anomalous behavior of 250 dimeric particles interacting by a core-softened potential. This study led us to an unexpected result: the…

We report an extensive and systematic investigation of the multi-point and multi-time correlation functions to reveal the spatio-temporal structures of dynamic heterogeneities in glass-forming liquids. Molecular dynamics simulations are…

Soft Condensed Matter · Physics 2013-01-04 Kang Kim , Shinji Saito

We explore the structural properties of anomalous fluids confined in a nanopore using Molecular Dynamics simulations. The fluid is modeled by core-softened (CS) potentials that have a repulsive shoulder and an attractive well at a further…

Soft Condensed Matter · Physics 2014-10-22 Leandro B. Krott , José Rafael Bordin , Marcia Barbosa

Molecular dynamics simulations of water, liquid beryllium fluoride and silica melt are used to study the accuracy with which the entropy of ionic and molecular liquids can be estimated from atom-atom radial distribution function data. All…

Soft Condensed Matter · Physics 2009-11-13 Ruchi Sharma , Manish Agarwal , Charusita Chakravarty

The most accepted origin for the water anomalous behavior is the phase transition between two liquids (LLPT) in the supercooled regime connected to the glassy first order phase transition at lower temperatures. Two length scales potentials…

Soft Condensed Matter · Physics 2023-04-19 José Rafael Bordin , Leandro B. Krott

Liquid-state theory, computer simulation, and numerical optimization are used to investigate the extent to which positional correlations of a hard-sphere fluid--as characterized by the radial distribution function and the two-particle…

Soft Condensed Matter · Physics 2016-03-23 Ryan B. Jadrich , Beth A. Lindquist , Jonathan A. Bollinger , Thomas M. Truskett

The vapor-liquid critical behavior of intrinsically asymmetric fluids is studied in finite systems of linear dimensions, $L$, focusing on periodic boundary conditions, as appropriate for simulations. The recently propounded ``complete''…

Statistical Mechanics · Physics 2009-11-10 Young C. Kim , Michael E. Fisher

Three core-softened families of potentials are checked for the presence of density and diffusion anomalies. These potentials exhibit a repulsive core with a softening region and at larger distances an attractive well. We found that the…

Statistical Mechanics · Physics 2015-06-12 Evy Salcedo , Ney Barraz , Marcia Barbosa