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Related papers: Equilibrium fluid-solid coexistence of hard sphere…

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We combine experiments, theory, and simulations to investigate the coexistence of nonequilibrium phases emerging from interacting colloidal particles that are electrokinetically propelled in a nematic liquid crystal solvent. We directly…

Soft Condensed Matter · Physics 2018-06-27 Josep M. Pagès , Arthur V. Straube , Pietro Tierno , Jordi Ignés-Mullol , Francesc Sagués

In the free energy of hydration of a solute, the chemical contribution is given by the free energy required to expel water molecules from the coordination sphere and the packing contribution is given by the free energy required to create…

Chemical Physics · Physics 2010-08-09 Valery Weber , Safir Merchant , Purushottam D. Dixit , D. Asthagiri

A detailed comparison between the Boubl\'ik-Mansoori-Carnahan-Starling-Leland (BMCSL)equation of state of hard-sphere mixtures is made with Molecular Dynamics (MD) simulations of the same compositions. The Lab\'ik and Smith simulation…

Soft Condensed Matter · Physics 2018-06-08 David M. Heyes , Andrés Santos

A free-energy functional for a crystal that contains both the symmetry conserved and symmetry broken parts of the direct pair correlation function is developed. The free-energy functional is used to investigate the crystallization of fluids…

Soft Condensed Matter · Physics 2015-05-13 Swarn Lata Singh , Yashwant Singh

Our recent quasi-two-dimensional thermodynamic description of thin-liquid films stabilized by colloidal particles is generalized to describe nonuniform equilibrium states of films in external potentials and nonequilibrium transport…

Soft Condensed Matter · Physics 2009-11-13 J. Blawzdziewicz , E. Wajnryb

We investigate sedimentation of model hard sphere-like colloidal dispersions confined in horizontal capillaries using laser scanning confocal microscopy, dynamical density functional theory, and Brownian dynamics computer simulations. For…

Soft Condensed Matter · Physics 2009-11-13 C. Patrick Royall , Joachim Dzubiella , Matthias Schmidt , Alfons van Blaaderen

Structure and thermodynamics of crystalline membranes are characterized by the long wavelength behavior of the normal-normal correlation function G(q). We calculate G(q) by Monte Carlo and Molecular Dynamics simulations for a quasi-harmonic…

Materials Science · Physics 2015-05-13 J. H. Los , M. I. Katsnelson , O. V. Yazyev , K. V. Zakharchenko , A. Fasolino

We present a study of hydrogen at pressures higher than molecular dissociation using the Coupled Electron-Ion Monte Carlo method. These calculations use the accurate Reptation Quantum Monte Carlo method to estimate the electronic energy and…

Materials Science · Physics 2013-05-29 Miguel A. Morales , Carlo Pierleoni , David Ceperley

Monte Carlo simulations using a hybrid quantum and classical mechanical potential were performed for crystal and amorphous-like HCl-water(n) clusters The subsystem composed by HCl and one water molecule was treated within Density Functional…

Chemical Physics · Physics 2009-10-30 Dario A. Estrin , Jorge Kohanoff , Daniel H. Laria , Ruben O. Weht

A new Monte Carlo approach is proposed to investigate the fluid-solid phase transition of the polydisperse system. By using the extended ensemble, a reversible path was constructed to link the monodisperse and corresponding polydisperse…

Soft Condensed Matter · Physics 2008-07-08 Mingcheng Yang , Hongru Ma

We study the gap closure with pressure of crystalline molecular hydrogen. The gaps are obtained from grand-canonical Quantum Monte Carlo methods properly extended to quantum and thermal crystals, simulated by Coupled Electron Ion Monte…

Materials Science · Physics 2020-03-25 Vitaly Gorelov , Markus Holzmann , David M. Ceperley , Carlo Pierleoni

Colloidal crystals with a diamond and pyrochlore structure display wide photonic band gaps at low refractive index contrasts. However, these low-coordinated and open structures are notoriously difficult to self-assemble from colloids…

Soft Condensed Matter · Physics 2019-06-26 Tonnishtha Dasgupta , Gabriele M. Coli , Marjolein Dijkstra

A Lennard--Jones model of a binary dense liquid (A,B) with a symmetrical miscibility gap is investigated by means of computer simulation methods. Semigrand--canonical Monte Carlo simulations yield the phase diagram in the $T$--$x$ plane…

Statistical Mechanics · Physics 2007-05-23 Subir K. Das , Jürgen Horbach , Kurt Binder

The effect of surface roughness on the structure of liquid crystalline fluids near solid substrates is studied by Monte Carlo simulations. The liquid crystal is modelled as a fluid of soft ellipsoidal molecules and the substrate is modelled…

Soft Condensed Matter · Physics 2009-11-11 David Cheung , Friederike Schmid

Continuum Monte-Carlo simulations at constant pressure are performed on short chain molecules at surfaces. The rodlike chains, consisting of seven effective monomers, are attached at one end to a flat twodimensional substrate. It is found…

Condensed Matter · Physics 2007-05-23 R. Hilfer , F. M. Haas

We report a systematic molecular dynamics study of the isochoric equilibration of hard-sphere fluids in their metastable regime close to the glass transition. The thermalization process starts with the system prepared in a non-equilibrium…

We simulate the decay of isolated, spherically symmetric droplets in a cosmological phase transition. It has long been posited that such heated droplets of the metastable state could form, and they have recently been observed in 3D…

Cosmology and Nongalactic Astrophysics · Physics 2023-01-04 Daniel Cutting , Essi Vilhonen , David J. Weir

Mesoscopic particles immersed in a critical fluid experience long-range Casimir forces due to critical fluctuations. Using field theoretical methods, we investigate the Casimir interaction between two spherical particles and between a…

Condensed Matter · Physics 2009-10-28 E. Eisenriegler , U. Ritschel

Simple models for spherical particles with a soft shell have been shown to self-assemble into numerous crystal phases and even quasicrystals. However, most of these models rely on a simple pairwise interaction, which is usually a valid…

Soft Condensed Matter · Physics 2020-09-03 Emanuele Boattini , Nina Bezem , Sudeep N. Punnathanam , Frank Smallenburg , Laura Filion

New hybrid Molecular Dynamics-Monte Carlo methods are proposed to increase the efficiency of constant-pressure simulations. Two variations of the isobaric Molecular Dynamics component of the algorithms are considered. In the first, we use…

Soft Condensed Matter · Physics 2009-11-07 Roland Faller , Juan J. de Pablo
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