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Transport and magnetic measurements and structural and NMR studies have been carried out on (Pr1-yR'y)1-xAxCoO3 {R'=(rare earth elements and Y); A=(Ca, Ba and Sr)} at ambient pressure or under high pressure. The system exhibits a phase…

Magneto-dielectric spectra of La0.95Ca0.05CoO3 covering the crossover of spin states reveals strong coupling of its spin and dipolar degrees of freedom. Signature of spin-state transition at 30K clearly manifests in magnetization, supported…

Materials Science · Physics 2016-02-29 Suchita Pandey , Jitender Kumar , A. M. Awasthi

Spin-state transitions, observed in many transition metal compounds containing Co$^{3+}$ and Fe$^{2+}$, may occur with the change of temperature, pressure, but also with doping, in which case the competition of single-site effects and…

Strongly Correlated Electrons · Physics 2009-07-24 A. O. Sboychakov , K. I. Kugel , A. L. Rakhmanov , D. I. Khomskii

Spin-state crossover beyond a conventional ligand-field theory has been a fundamental issue in condensed matter physics. Here, we report microscopic observations of spin states and low-energy dynamics through orbital-resolved NMR…

Strongly Correlated Electrons · Physics 2018-01-01 Yasuhiro Shimizu , Takuya Takahashi , Syunpei Yamada , Ayako Shimokata , Takaaki Jin-no , Masayuki Itoh

Motivated by recent observation of magnetic field induced transition in LaCoO3 we study the effect of external field in systems close to instabilities towards spin-state ordering and exciton condensation. We show that, while in both cases…

Strongly Correlated Electrons · Physics 2016-07-28 Andrii Sotnikov , Jan Kunes

We report on a 59Co NMR investigation of the trigonal cobaltate Ca3Co2O6 carried out on a single crystal, providing precise determinations of the electric field gradient and chemical shift tensors, and of the internal magnetic fields at the…

Strongly Correlated Electrons · Physics 2015-05-20 G. Allodi , R. De Renzi , S. Agrestini , C. Mazzoli , M. R. Lees

We investigate the evolution of spin and orbital order in undoped LaMnO$_3$ under increasing temperature with a model including both superexchange and Jahn-Teller interactions. We used several cluster mean field calculation schemes and find…

Strongly Correlated Electrons · Physics 2016-12-26 Mateusz Snamina , Andrzej M. Oleś

We study the asymmetric Hubbard model at half-filling as a generic model to describe the physics of two species of repulsively interacting fermionic cold atoms in optical lattices. We use Dynamical Mean Field Theory to obtain the…

Strongly Correlated Electrons · Physics 2012-01-11 E. A. Winograd , R. Chitra , M. J. Rozenberg

We investigate the influence of spin-orbit coupling $\lambda$ in strongly-correlated multiorbital systems that we describe by a three-orbital Hubbard-Kanamori model on a Bethe lattice. We solve the problem at all integer fillings $N$ with…

Strongly Correlated Electrons · Physics 2018-11-30 Robert Triebl , Gernot J. Kraberger , Jernej Mravlje , Markus Aichhorn

A two-dimensional Falicov-Kimball model, equivalent to the Hubbard model in an unconstrained slave-spin representation, is studied by quantum Monte Carlo simulations. The focus is on a fractionalized metallic phase that is characterized in…

Strongly Correlated Electrons · Physics 2019-09-17 Martin Hohenadler , Fakher F. Assaad

We present the first systematic observation of scaling of thermal hysteresis with the temperature scanning rate around an abrupt thermodynamic transition in correlated electron systems. We show that the depth of supercooling and…

Orbitally degenerate systems provide a promising platform for realizing novel quantum phases driven by spin-orbital exchange interactions, as described by the Kugel-Khomskii model. Spinel vanadates, in which orbital degrees of freedom…

Strongly Correlated Electrons · Physics 2026-05-06 Hiroki Nakai , Yusuke Nomura

V2O3 is the prototype system for the Mott transition, one of the most fundamental phenomena of electronic correlation. Temperature, doping or pressure induce a metal to insulator transition (MIT) between a paramagnetic metal (PM) and a…

The concept of spin-orbital entanglement on superexchange bonds in transition metal oxides is introduced and explained on several examples. It is shown that spin-orbital entanglement in superexchange models destabilizes the long-range (spin…

Strongly Correlated Electrons · Physics 2012-07-13 Andrzej M. Oleś

\lco{} is known for its two-step spin crossover as a function of temperature. Despite efforts spanning over half a century, the origin of this phenomenon is still debated, particularly regarding how the microscopic spin states are involved…

Strongly Correlated Electrons · Physics 2024-11-18 Akihiko Ikeda , Yasuhiro H. Matsuda , Keisuke Sato , Joji Nasu

The multiorbital Hubbard model in the strong coupling limit is analyzed for the effectively antiferromagnetic Hund's coupling relevant to fulleride superconductors with three orbitals per molecule. The localized spin-orbital model describes…

Strongly Correlated Electrons · Physics 2021-06-30 Ryuta Iwazaki , Shintaro Hoshino

We study ground-state properties of the two-dimensional Hubbard model at half filling by improving variational Monte Carlo method and by implementing quantum-number projection and multi-variable optimization. The improved variational wave…

Strongly Correlated Electrons · Physics 2008-08-30 Daisuke Tahara , Masatoshi Imada

Using configuration-state-constrained electronic structure calculations based on the generalized gradient approximation plus Hubbard U method, we sought the origin of the giant tetragonal ferroelectric distortion in the ambient phase of the…

Strongly Correlated Electrons · Physics 2011-05-25 Ting Jia , Hua Wu , Guoren Zhang , Xiaoli Zhang , Ying Guo , Zhi Zeng , Hai-Qing Lin

We present magnetization and magnetostriction studies of the insulating perovskite LaCoO3 in magnetic fields approaching 100 T. In marked contrast with expectations from single-ion models, the data reveal two distinct first-order spin…

Quantum Monte Carlo methods are used to study a quantum phase transition in a 1D Hubbard model with a staggered ionic potential (D). Using recently formulated methods, the electronic polarization and localization are determined directly…

Strongly Correlated Electrons · Physics 2009-10-31 Tim Wilkens , Richard M. Martin