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Using neutron inelastic scattering, we investigate the role of interstitial iron on the low-energy spin fluctuations in powder samples of Fe_{1+x}Te_{0.7}Se_{0.3}. We demonstrate how combining the principle of detailed balance along with…

Superconductivity · Physics 2015-06-04 C. Stock , E. E. Rodriguez , M. A. Green

The superconducting series, Fe(Te,Se), has a complex structural and magnetic phase diagram that is dependent on composition and occupancy of a secondary interstitial Fe site. In this letter, we show that superconductivity in Fe1+xTe0.7Se0.3…

Superconductivity · Physics 2011-07-12 E. E. Rodriguez , C. Stock , P-Y Hsieh , N. Butch , J. Paglione , M. A. Green

We present a systematic study of the nematic fluctuations in the iron chalcogenide superconductor Fe$_{1+y}$Te$_{1-x}$Se$_{x}$ ($0 \leq x \leq 0.53$) using the elastoresistivity technique. Near $x = 0$, in proximity to the double-stripe…

The nature of the superconducting state in the recently discovered Fe-based superconductors1-3 is the subject of intense scrutiny. Neutron scattering investigations have already elucidated a strong correlation between magnetism and…

The Fe1+yTe1-xSex series of materials is one of the prototype families of Fe-based superconductors. To provide further insight into these materials we present systematic inelastic neutron scattering measurements of the low energy spin…

We use inelastic neutron scattering to study the low energy spin excitations in moderately doped non-superconducting Fe$_{1.01}$Te$_{0.72}$Se$_{0.28}$. The spin excitations in this system contain components near (0.5,0,0) and (0.5,0.5,0) in…

Strongly Correlated Electrons · Physics 2011-12-07 Songxue Chi , J. A. Rodriguez-Rivera , J. W. Lynn , Chenglin Zhang , D. Phelan , D. K. Singh , R. Paul , Pengcheng Dai

Elucidating the microscopic origin of nematic order in iron-based superconducting materials is important because the interactions that drive nematic order may also mediate the Cooper pairing. Nematic order breaks fourfold rotational…

We construct a phase diagram of the parent compound Fe1+xTe as a function of interstitial iron x in terms of the electronic, structural, and magnetic properties. For a concentration of x < 10%, Fe1+xTe undergoes a "semimetal" to metal…

Strongly Correlated Electrons · Physics 2015-06-17 E. E. Rodriguez , D. A. Sokolov , C. Stock , M. A. Green , O. Sobolev , J. A. Rodriguez-Rivera , H. Cao , A. Daoud-Aladine

Polarized Raman-scattering spectra of superconducting, single-crystalline FeSe evidence pronounced phonon anomalies with temperature reduction. A large 6.5% hardening of the B_1g(Fe) phonon mode is attributed to the suppression of local…

We study the magnetic properties of Fe_1+y Te, a parent compound of the iron-based high-temperature superconductors. Motivated by recent neutron scattering experiments, we show that a spin-1 exchange model, supplemented by a single-ion spin…

Strongly Correlated Electrons · Physics 2013-10-30 G. Chen , S. Choi , L. Radzihovsky

Neutron spectroscopy is used to investigate the magnetic fluctuations in Fe_{1+x}Te - a parent compound of chalcogenide superconductors. Incommensurate "stripe-like" excitations soften with increased interstitial iron concentration. The…

Strongly Correlated Electrons · Physics 2015-06-22 C. Stock , E. E. Rodriguez , O. Sobolev , J. A. Rodriguez-Rivera , R. A. Ewings , J. W. Taylor , A. D. Christianson , M. A. Green

Magnetic fluctuations in the molecular-intercalated FeSe superconductor Li{x}(ND2){y}(ND3){1-y}Fe2Se2 (Tc = 43K) have been measured by inelastic neutron scattering from a powder sample. The strongest magnetic scattering is observed at a…

Electronic structure calculations are used to analyze the electronic and magnetic properties in {K$_{2}$Fe$_{4+x}$Se$_{5}$}. Fe atoms can be divided into two distinct groups. The $x{=}0$ (parent) compound forms an insulating, collinear,…

Materials Science · Physics 2012-09-04 Liqin Ke , Mark van Schilfgaarde , Vladimir Antropov

The Fe1+xTe phase diagram consists of two distinct magnetic structures with collinear order present at low interstitial iron concentrations and a helical phase at large values of x with these phases separated by a Lifshitz point. We use…

Strongly Correlated Electrons · Physics 2017-11-21 C. Stock , E. E. Rodriguez , P. Bourges , R. A. Ewings , H. Cao , S. Chi , J. A. Rodriguez-Rivera , M. A. Green

Intertwined spin and charge orders have been widely studied in high-temperature superconductors, since their fluctuations may facilitate electron pairing; however, they are rarely identified in heavily electron-doped iron selenides. Here,…

The Fe1+y Te1-x Sex compounds belong to the family of iron-based high temperature superconductors, in which superconductivity often appears upon doping antiferromagnetic parent compounds. Unlike other Fe-based superconductors (in which the…

Superconductivity · Physics 2015-03-19 D. Parshall , G. Chen , L. Pintschovius , D. Lamago , Th. Wolf , L. Radzihovsky , D. Reznik

Using polarized and unpolarized neutron scattering we show that interstitial Fe in superconducting Fe_{1+y}Te_{1-x}Se_x induces a magnetic Friedel-like oscillation that diffracts at Q_(in-plane)=(1/2,0) and involves >50 neighboring Fe…

We review neutron scattering investigations of the crystal structures, magnetic structures, and spin dynamics of the iron-based RFe(As,P)O (R=La, Ce, Pr, Nd), (Ba,Sr,Ca)Fe2As2, and Fe1+x(Te-Se) systems. On cooling from room temperature all…

Superconductivity · Physics 2009-05-20 Jeffrey W. Lynn , Pengcheng Dai

High-temperature superconductivity remains arguably the largest outstanding enigma of condensed matter physics. The discovery of iron-based high-temperature superconductors has renewed the importance of understanding superconductivity in…

We report neutron scattering studies on static magnetic orders and spin excitations in the Fe-based chalcogenide system Fe$_{1+\delta}$Se$_{x}$Te$_{1-x}$ with different Fe and Se compositions. Short-range static magnetic order with the…

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