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The dynamics of photocarriers in reduced graphene oxide thin films is studied by using ultrafast pump-probe spectroscopy. Time dependent differential transmissions are measured with sample temperatures ranging from 9 to 300 K. At each…

Mesoscale and Nanoscale Physics · Physics 2015-05-18 Brian A. Ruzicka , Lalani K. Werake , Hui Zhao , Shuai Wang , Kian Ping Loh

Using optical-pump terahertz-probe spectroscopy, we study the relaxation dynamics of photoexcited carriers in graphene at different temperatures. We find that at lower temperatures the tail of the relaxation transients as measured by the…

Mesoscale and Nanoscale Physics · Physics 2015-05-30 Jared H. Strait , Haining Wang , Shriram Shivaraman , Virgil B. Shields , Michael G. Spencer , Farhan Rana

Understanding and controlling hot-carrier relaxation in graphene is crucial for advancing ultrafast optoelectronic and terahertz technologies. Here, we investigate carrier cooling dynamics in monolayer and bilayer graphene using…

Mesoscale and Nanoscale Physics · Physics 2026-05-21 Sachin Sharm , Elliott Walker , Rachael Myers-Ward , Jenifer Hajzus , Yijing Liu , Paola Barbara , Ioannis Chatzakis

We report ultrafast response of femtosecond photoexcited carriers in single layer reduced graphene oxide flakes suspended in water as well as few layer thick film deposited on indium tin oxide coated glass plate using pump-probe…

Materials Science · Physics 2011-06-30 Sunil Kumar , N. Kamaraju , K. S. Vasu , A. K. Sood

We study the carrier dynamics in epitaxially grown graphene in the range of photon energies from 10 - 250 meV. The experiments complemented by microscopic modeling reveal that the carrier relaxation is significantly slowed down as the…

Using ultrafast optical pump-probe spectroscopy, we study the relaxation dynamics of hot optical phonons in few-layer and multi-layer graphene films grown by epitaxy on silicon carbide substrates and by chemical vapor deposition on nickel…

A degenerate pump--probe technique is used to investigate the non equilibrium carrier dynamics in multi--layer graphene. Two distinctly different dynamics of the carrier relaxation are observed. A fast relaxation ($\sim 50$ fs) of the…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 P. Plochocka , P. Kossacki , A. Golnik , T. Kazimierczuk , C. Berger , W. A. de Heer , M. Potemski

We report an optical study of charge transport in graphene. Diffusion of hot carriers in epitaxial graphene and reduced graphene oxide samples are studied using an ultrafast pump-probe technique with a high spatial resolution.…

Mesoscale and Nanoscale Physics · Physics 2015-03-17 Brian A. Ruzicka , Shuai Wang , Lalani K. Werake , Ben Weintrub , Kian Ping Loh , Hui Zhao

Using ultrafast optical pump-probe spectroscopy, we have measured carrier relaxation times in epitaxial graphene layers grown on SiC wafers. We find two distinct time scales associated with the relaxation of nonequilibrium photogenerated…

Materials Science · Physics 2019-06-05 Jahan M. Dawlaty , Shriram Shivaraman , Mvs Chandrashekhar , Farhan Rana , Michael G. Spencer

We study, by means of a Monte Carlo simulator, the hot phonon effect on the relaxation dynamics in photoexcited graphene and its quantitative impact as compared to considering an equilibrium phonon distribution. Our multi-particle approach…

Mesoscale and Nanoscale Physics · Physics 2016-02-02 José M. Iglesias , María J. Martín , Elena Pascual , Raúl Rengel

For most optoelectronic applications of graphene a thorough understanding of the processes that govern energy relaxation of photoexcited carriers is essential. The ultrafast energy relaxation in graphene occurs through two competing…

We present an ab-initio study of photocarrier dynamics in graphene due to electron-phonon (EP) interactions. Using the Boltzmann relaxation-time approximation with parameters determined from density functional theory (DFT) and a…

Materials Science · Physics 2019-04-17 Dinesh Yadav , Maxim Trushin , Fabian Pauly

The nonequilibrium dynamics of carriers and phonons in graphene is investigated by solving the microscopic kinetic equations with the carrier-phonon and carrier-carrier Coulomb scatterings explicitly included. The Fermi distribution of hot…

Mesoscale and Nanoscale Physics · Physics 2012-03-15 B. Y. Sun , Y. Zhou , M. W. Wu

The ultrafast relaxation and recombination dynamics of photogenerated electrons and holes in epitaxial graphene are studied using optical-pump Terahertz-probe spectroscopy. The conductivity in graphene at Terahertz frequencies depends on…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 Paul A. George , Jared Strait , Jahan Dawlaty , Shriram Shivaraman , Mvs Chandrashekhar , Farhan Rana , Michael G. Spencer

Nonlinear optical properties and carrier relaxation dynamics in graphene, suspended in three different solvents, are investigated using femtosecond (80 fs pulses) Z-scan and degenerate pumpprobe spectroscopy at 790 nm. The results…

Materials Science · Physics 2015-05-14 Sunil Kumar , M. Anija , N. Kamaraju , K. S. Vasu , K. S. Subrahmanyam , A. K. Sood , C. N. R. Rao

The heating of carriers in an intrinsic graphene under an abrupt switching off a dc electric field is examined taking into account both the energy relaxation via acoustic and optic phonons and the interband generation-recombination…

Mesoscale and Nanoscale Physics · Physics 2015-05-20 P. N. Romanets , F. T. Vasko

Femtosecond time-resolved spectroscopy using 400 nm-pump and 800 nm-probe in CVD-grown multilayer graphene provides strong evidence for isotropic distribution of photoexcited carrier after initial relaxation. Indicative of such isotropic…

Mesoscale and Nanoscale Physics · Physics 2013-12-24 Xiao-Qing Yan , Zhi-Bo Liu , Jun Yao , Xin Zhao , Xu-Dong Chen , Yongsheng Chen , Jian-Guo Tian

NaOH-reacted graphite oxide film was prepared by decomposing epoxy groups in graphite oxide into hydroxyl and -ONa groups with NaOH solution. Ultrafast carrier dynamics of the sample were studied by time-resolved transient differential…

We investigate the energy relaxation of hot carriers produced by photoexcitation of graphene through coupling to both intrinsic and remote (substrate) surface polar phonons using the Boltzmann equation approach. We find that the energy…

Mesoscale and Nanoscale Physics · Physics 2012-08-15 Tony Low , Vasili Perebeinos , Raseong Kim , Marcus Freitag , Phaedon Avouris

We develop a theory for the energy relaxation of hot Dirac fermions in graphene. We obtain a generic expression for the energy relaxation rate due to electron-phonon interaction and calculate the power loss due to both optical and acoustic…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 Wang-Kong Tse , S. Das Sarma
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