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We show that when a molecular junction is under an external bias, its properties can not be uniquely determined by the total electron density in the same manner as the density functional theory (DFT) for ground state (GS) properties. In…

Mesoscale and Nanoscale Physics · Physics 2013-11-26 Shuanglong Liu , Yuan Ping Feng , Chun Zhang

A recently proposed density functional approach for steady-state transport through nanoscale systems (called i-DFT) is used to investigate junctions which are asymmetrically coupled to the leads and biased with asymmetric voltage drops. In…

Mesoscale and Nanoscale Physics · Physics 2018-07-04 Stefan Kurth , David Jacob

Electron-electron correlations affect the band gap of half-metallic ferromagnets by introducing non-quasiparticle states just above the Fermi level. In contrast to the spin-orbit coupling, a large asymmetric non-quasiparticle spectral…

Strongly Correlated Electrons · Physics 2014-04-15 L. Chioncel , E. Arrigoni , M. I. Katsnelson , A. I. Lichtenstein

Thermal conductivity measurements can provide key and experimentally verifiable insight into the electronic transport of unconventional superconductors. In this work, electronic thermal transport of two-dimensional tight-binding metallic…

Superconductivity · Physics 2023-08-16 Sean F Peterson , Sourav Sen Choudhury , Yves Idzerda

We present results of a detailed theoretical study of the electronic, magnetic, and structural properties of the chalcogenide parent system FeSe using a fully charge self-consistent implementation of the density functional theory plus…

Strongly Correlated Electrons · Physics 2017-07-26 S. L. Skornyakov , V. I. Anisimov , D. Vollhardt , I. Leonov

Strongly correlated systems have long been a central and highly non-trivial topic in condensed matter physics. At the non-interacting level, strong correlation can be associated with powerful (near) degeneracies between occupied and…

Strongly Correlated Electrons · Physics 2026-04-29 Daniel D. Rivera , Gustavo M. Dalpian , John P. Perdew

Optical spectroscopy, X-ray diffraction measurements, density functional theory (DFT) and density functional theory + embedded dynamical mean field theory (DFT+eDMFT) have been used to characterize structural and electronic properties of…

Strongly Correlated Electrons · Physics 2020-09-23 T. N. Stanislavchuk , G. L. Pascut , A. P. Litvinchuk , Z. Liu , S. Choi , M. J. Gutmann , B. Gao , K. Haule , V. Kiryukhin , S. -W. Cheong , A. A. Sirenko

The design of better exchange-correlation functionals for Density Functional Theory (DFT) is a central challenge of modern electronic structure theory. However, current developments are limited by the mathematical form of the functional,…

Chemical Physics · Physics 2024-08-19 Kyle Bystrom , Boris Kozinsky

It can be argued that electron correlation, as a concept, deserves the same prominence in general chemistry as molecular orbital theory. We show how it acts as Nature's "chemical glue" at both the molecular and supramolecular levels.…

Chemical Physics · Physics 2022-01-10 Jan M. L. Martin

A wide range of unconventional transport phenomena have recently been observed in single-crystal delafossite metals. Here, we present a theoretical framework to elucidate electron transport using a combination of first-principles…

Materials Science · Physics 2022-08-17 Georgios Varnavides , Yaxian Wang , Philip J. W. Moll , Polina Anikeeva , Prineha Narang

Recent high resolution Compton scattering experiments clearly reveal that there are fundamental limitations to the conventional local density approximation (LDA) based description of the ground state electron momentum density (EMD) in…

Strongly Correlated Electrons · Physics 2007-10-11 B. Barbiellini , A. Bansil

The electronic band structure of bulk ferromagnetic iron is explored by angle-resolved photoemission for electron correlation effects. Fermi surface cross-sections as well as band maps are contrasted with density functional calculations.…

Strongly Correlated Electrons · Physics 2015-06-24 J. Schaefer , M. Hoinkis , Eli Rotenberg , P. Blaha , R. Claessen

The effect of electron correlation on the angle dependence of magnetoconductivity is studied in quasi-one-dimensional organic conductors. We investigated the effect on the basis of the momentum dependence of both quasi-particle's lifetime…

Strongly Correlated Electrons · Physics 2007-05-23 Hirono Kaneyasu , Keita Kishigi , Yasumasa Hasegawa

Several new aspects of the subtle interplay between electronic correlations and disorder are reviewed. First, the dynamical mean-field theory (DMFT)together with the geometrically averaged ("typical") local density of states is employed to…

Strongly Correlated Electrons · Physics 2015-05-18 K. Byczuk , W. Hofstetter , U. Yu , D. Vollhardt

Multiple-band electronic structure and proximity to antiferromagnetic (AF) instability are the key properties of iron-based superconductors. We explore the influence of scattering by the AF spin fluctuations on transport of multiple-band…

Strongly Correlated Electrons · Physics 2016-11-03 A. E. Koshelev

We propose a hybrid approach which employs the dynamical mean-field theory (DMFT) self-energy for the correlated, typically rather localized orbitals and a conventional density functional theory (DFT) exchange-correlation potential for the…

Strongly Correlated Electrons · Physics 2021-06-16 Sumanta Bhandary , Karsten Held

Electrons in zero external magnetic field can be studied with density functional theory (DFT) or with spin-DFT (SDFT). The latter is normally used for open shell systems because its approximations appear to model better the exchange and…

Chemical Physics · Physics 2022-04-06 Timothy Callow , Benjamin Pearce , Nikitas Gidopoulos

We study the Fermi level structure of (2+1)-dimensional strongly interacting electron systems in external magnetic field using the AdS/CFT correspondence. The gravity dual of a finite density fermion system is a Dirac field in the…

High Energy Physics - Theory · Physics 2015-06-15 E. Gubankova , J. Brill , M. Cubrovic , K. Schalm , P. Schijven , J. Zaanen

In BaNiS2 a Dirac nodal-line band structure exists within a two-dimensional Ni square lattice system, in which significant electronic correlation effects are anticipated. Using scanning tunneling microscopy, we discover signs of…

Strongly Correlated Electrons · Physics 2022-12-28 C. J. Butler , Y. Kohsaka , Y. Yamakawa , M. S. Bahramy , S. Onari , H. Kontani , T. Hanaguri , S. Shamoto

In our theoretical study in which we combine a nonequilibrium Green's function (NEGF) approach with density functional theory (DFT) we investigate branched compounds containing Ru or Os metal complexes in two branches, which due to their…

Chemical Physics · Physics 2019-03-27 Xin Zhao , Robert Stadler