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We use a density functional approach to calculate the contact angle of the water model on a heterogeneous, graphite-like surface. The surface heterogeneity results from the pre-adsorption of a layer of spherical species. The pre-adsorbed…

Soft Condensed Matter · Physics 2022-10-04 K. Dąbrowska , O. Pizio , S. Sokołowski

We investigate the solvation of methane and methane decorated with charges in spherically confined water droplets. Free energy profiles for a single methane molecule in droplets, ranging in diameter D, from 1 to 4 nm, show that the droplet…

Chemical Physics · Physics 2009-09-29 S. Vaitheeswaran , D. Thirumalai

Patchy colloidal model with three and four equivalent patches, confined in the attractive random porous media, undergo re-entrant gas-liquid phase separation with the possibility for the liquid phase density to approach zero. This unusual…

Soft Condensed Matter · Physics 2022-05-11 Taras Hvozd , Yurij V. Kalyuzhnyi , Vojko Vlachy , Peter T. Cummings

We present a theory that is able to account quantitatively for the surface and interfacial tensions of different electrolyte solutions. It is found that near the interface, ions can be separated into two classes: the kosmotropes and the…

Soft Condensed Matter · Physics 2018-02-21 Alexandre P. dos Santos , Yan Levin

We consider the behaviour of a dielectric fluid-fluid interface in the presence of a strong electric field from a point charge and line charge, respectively, both statically and, in the latter case, dynamically. The fluid surface is…

Soft Condensed Matter · Physics 2012-11-08 Simen Å. Ellingsen , Iver Brevik

The modification of the boundary condition for polyelectrolyte adsorption on charged surface with short-ranged interaction is investigated under two regimes. For weakly charged Gaussian polymer in which the short-ranged attraction…

Soft Condensed Matter · Physics 2007-05-23 Chi-Ho Cheng

In this Letter, we show that at low temperatures, zero-point fluctuations of the plasmon modes of two mutually coupled 2-D planar Wigner crystals give rise to a novel long-range attractive force. For the case where the distance $d$ between…

Soft Condensed Matter · Physics 2016-08-31 A. W. C. Lau , Dov Levine , P. Pincus

We report a mechanism which can lead to long range attractions between like-charged spherical macroions, stemming from the existence of metastable ionized states. We show that the ground state of a single highly charged colloid plus a few…

Soft Condensed Matter · Physics 2009-10-31 Rene Messina , Christian Holm , Kurt Kremer

We present a simple model for an associating liquid in which polymorphism and density anomaly are connected. Our model combines a two dimensional lattice gas with particles interacting through a soft core potential and orientational degrees…

Statistical Mechanics · Physics 2009-11-10 Vera B. Henriques , Marcia C Barbosa

The electro-osmotic flow through a channel between two undulated surfaces induced by an external electric field is investigated. The gap of the channel is very small and comparable to the thickness of the electrical double layers. A lattice…

Soft Condensed Matter · Physics 2016-05-24 Hiroaki Yoshida , Tomoyuki Kinjo , Hitoshi Washizu

We study the ionic distribution near a charged surface. A new method for performing Monte Carlo simulations in this geometry is discussed. A theory is then presented that allows us to accurately reproduce the density profiles obtained in…

Chemical Physics · Physics 2012-11-09 Alexandre P. dos Santos , Yan Levin

We study the phase structure of a dilute two-component Fermi system with attractive interactions as a function of the coupling and the polarization or number difference between the two components. In weak coupling, a finite number asymmetry…

Other Condensed Matter · Physics 2009-11-11 J. Carlson , Sanjay Reddy

Using density-functional theory in combination with a thermodynamic formalism we calculate the relative stability of various structural models of the polar O-terminated (000-1)-O surface of ZnO. Model surfaces with different concentrations…

Materials Science · Physics 2009-11-10 B. Meyer

A simple model is presented for the appearance of attraction between two like charged polyions inside a polyelectrolyte solution. The polyions are modeled as rigid cylinders in a continuum dielectric solvent. The strong electrostatic…

Soft Condensed Matter · Physics 2009-10-31 Alexandre Diehl , Humberto A. Carmona , Yan Levin

We experimentally show that dipolar interaction can stabilize otherwise unstable many-body systems like an attractive Bose gas. In a one dimensional lattice the repulsive dipolar on-site interaction balances negative scattering lengths up…

Quantum Gases · Physics 2012-02-03 S. Müller , J. Billy , E. A. L. Henn , H. Kadau , A. Griesmaier , M. Jona-Lasinio , L. Santos , T. Pfau

We develop a general formalism to investigate the effect of quenched fixed charge disorder on effective electrostatic interactions between charged surfaces in a one-component (counterion-only) Coulomb fluid. Analytical results are…

Soft Condensed Matter · Physics 2009-11-11 Ali Naji , Rudolf Podgornik

Carbon monoxide and nitrogen are among the potentially interesting high-energy density materials. However, in spite of the physical similarities of the molecules, they behave very differently at high pressures. Using density functional…

Materials Science · Physics 2013-12-06 Zamaan Raza , Chris J. Pickard , Carlos Pinilla , A. Marco Saitta

The electrostatic double layer force is key to determining the stability and self-assembly of charged colloids and many other soft matter systems. Fully understanding the attractive force between two like-charged surfaces remains a great…

Soft Condensed Matter · Physics 2024-02-27 Nikhil R. Agrawal , Ravtej Kaur , Carlo Carraro , Rui Wang

The ion distribution of electrolytes near interfaces with dielectric contrast has important consequences for electrochemical processes and many other applications. To date, most studies of such systems have focused on geometrically simple…

Soft Condensed Matter · Physics 2018-11-14 Huanxin Wu , Honghao Li , Francisco J. Solis , Monica Olvera de la Cruz , Erik Luijten

Molecular dynamic simulations were employed to study a water-like model confined between hydrophobic and hydrophilic plates. The phase behavior of this system is obtained for different distances between the plates and particle-plate…

Soft Condensed Matter · Physics 2015-06-17 Leandro B. Krott , Marcia C. Barbosa