Related papers: Resonant two-photon single ionization of two atoms
Based on quantum electrodynamics, we reexamine the two-photon decay of one-electron atoms. Special attention is paid to the calculation of the (two-photon) total decay rates which can be viewed as the imaginary part of the two-loop…
The ignition of two-quantum collective emission of inverted sub-ensemble of radiators due to mutual interaction of this sub-ensemble with other two dipole active atomic subsystems in process of two-photon exchanges between the atoms through…
Multi-photon absorption is a well-known phenomenon. With atom lasers a similar process could take place for massive particles, the ionization of an atom or molecule by the successive interaction with various particles. This process would…
The shape and absolute values of the generalized cross-sections of the two-photon resonant single ionization of the K-shell of ions of the isonuclear sequence of a heavy nickel atom (28Ni - Ni26+ - Ni24+ - Ni18+) have been theoretically…
Intense light with frequencies above typical atomic or molecular ionization potentials as provided by free-electron lasers couples many photons into extended targets such as clusters and biomolecules. This implies, in contrast to…
Quantum coherence plays a fundamental role in the study and control of ultrafast dynamics in matter. In the case of photoionization, entanglement of the photoelectron with the ion is a well known source of decoherence when only one of the…
Ozone (O3) is a triatomic molecule of central importance in the chemistry and physics of the Earth's and other planetary atmospheres. Beyond its environmental significance, a detailed understanding of the electronic structure and ionization…
The ionization of two-active-electron systems by intense laser fields is investigated theoretically. In comparison with time-dependent Hartree-Fock and exact two electron simulation, we show that the ionization rate is overestimated in SAE…
Triple-differential cross sections for two-photon double ionization of molecular hydrogen are presented for a central photon energy of 30 eV. The calculations are based on a fully {\it ab initio}, nonperturbative, approach to the…
Unravelling two-electron correlation is a long-standing challenge at the heart of few-body quantum physics, underlying correlated phenomena across atomic, molecular and condensed-matter science. In prototypical three-body Coulomb systems,…
Two-photon decay rates in simple atoms such as hydrogenlike systems represent rather interesting fundamental problems in atomic physics. The sum of the energies of the two emitted photons has to fulfill an energy conservation condition, the…
Coherent control of interfering one- and two-photon processes has for decades been the subject of research to achieve the redirection of photocurrent. The present study develops two-pathway coherent control of ground state helium atom…
Mapping equations of motion of the highly exited classical atom in a monochromatic field are generalized for the two-frequency microwave field. Analysis of the obtained equations indicates to the weak sensitivity of the position of the…
A free electron can form a bound state with an atomic center $A$ upon photo emission (radiative recombination). In the presence of a neighboring atom $B$, such a bound state can, under certain conditions, be also formed via resonant…
We present an experimental study on the photoionization dynamics of non-resonant one-color two-photon single valence ionization of neutral argon atoms. Using 9.3 eV photons produced via high harmonic generation and a 3-D momentum imaging…
Two efficient and isotope-selective resonant two-photon ionization techniques for loading barium ions into radio-frequency (RF)-traps are demonstrated. The scheme of using a strong dipole-allowed transition at \lambda=553 nm as a first step…
Intense laser ionization expands Einstein's photoelectric effect rules giving a wealth of phenomena widely studied over the last decades. In all cases, so far, photons were assumed to carry one unit of angular momentum. However it is now…
Highly charged relativistic heavy ions have high cross-sections for two-photon interactions. The photon flux is high enough that two-photon interactions may be accompanied by additional photonuclear interactions. Except for the shared…
Above 54.4 eV, two-photon double ionization of helium is dominated by a sequential absorption process, producing characteristic behavior in the single and triple differential cross sections. We show that the signature of this process is…
We present the results of experimental studies of photon-negative ion interactions involving the dynamics of two electrons. Resonances associated with doubly excited states of Li^- and He^- have been observed using laser photodetachment…