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A first-principle theoretical approach to study the process of radiative electron attachment is developed and applied to the negative molecular ions CN$^-$, C$_4$H$^-$, and C$_2$H$^-$. Among these anions, the first two have already been…

The Hubbard model is a prototype for strongly correlated electrons in condensed matter, for molecules and fermions or bosons in optical lattices. While the equilibrium properties of these systems have been studied in detail, the excitation…

Strongly Correlated Electrons · Physics 2014-07-08 M. Bonitz , S. Hermanns , K. Balzer

Neutral molecules with sufficiently large dipole moments can bind electrons in diffuse nonvalence orbitals with most of their charge density far from the nuclei, forming so-called dipole-bound anions. Because long-range correlation effects…

Chemical Physics · Physics 2018-10-30 Hongxia Hao , James Shee , Shiv Upadhyay , Can Ataca , Kenneth D. Jordan , Brenda M. Rubenstein

Strong light-matter interactions facilitate not only emerging applications in quantum and non-linear optics but also modifications of materials properties. In particular the latter possibility has spurred the development of advanced…

Mesoscale and Nanoscale Physics · Physics 2021-08-17 Jakub Fojt , Tuomas P. Rossi , Tomasz J. Antosiewicz , Mikael Kuisma , Paul Erhart

A detailed theoretical investigation of rare gas atom clusters under intense short laser pulses reveals that the mechanism of energy absorption is akin to {\it enhanced ionization} first discovered for diatomic molecules. The phenomenon is…

Atomic and Molecular Clusters · Physics 2009-11-07 Christian Siedschlag , Jan-Michael Rost

A decade ago, an electron-attachment process called interatomic Coulombic electron capture has been predicted to be possible through energy transfer to a nearby neighbor. It has been estimated to be competitive with environment-independent…

Chemical Physics · Physics 2023-06-22 Axel Molle , Oleg Zatsarinny , Thomas Jagau , Alain Dubois , Nicolas Sisourat

We study the ultrafast structural dynamics, in response to electronic excitations, in heterostructures composed of Au$_{923}$ nanoclusters on thin-film substrates with the use of femtosecond electron diffraction. Various forms of atomic…

We employ a novel Monte Carlo simulation scheme to elucidate the stabilization of neutral colloidal microspheres by means of highly-charged nanoparticles [V. Tohver et al., Proc. Natl. Acad. Sci. U.S.A. 98, 8950 (2001)]. In accordance with…

Soft Condensed Matter · Physics 2009-11-10 Jiwen Liu , Erik Luijten

We study the electronic properties (density of states, conductivity and thermopower) of some nearly--free--electron systems: the liquid alkali metals and two liquid alloys, Li-Na and Na-K. The study has been performed within the…

Disordered Systems and Neural Networks · Physics 2015-06-24 W. Geertsma , D. Gonzalez , L. H. Gonzalez

We report measurements of resonant low-energy electron attachment to O\(_2\) molecular impurities in neon gas in the temperature range \(46.5\,\mbox{K}\le T\le 101\,\mbox{K}\). The reduced attachment frequency \(\nu_A/N\) shows a well…

Plasma Physics · Physics 2020-04-22 A. F. Borghesani

We study two correlated electrons in a nearest neighbour tight- binding chain, with both on site and nearest neighbour interaction. Both the cases of parallel and antiparallel spins are considered. In addition to the free electron band for…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 J. F. Weisz , F. Claro

We present a quantitative theory of optical absorption polarized transverse to the tube axes in semiconducting single-walled carbon nanotubes. Transverse optical absorption in semiconducting single-walled carbon nanotubes is to an exciton…

Materials Science · Physics 2009-11-13 Zhendong Wang , Hongbo Zhao , Sumit Mazumdar

Electronic states in metallic nanoclusters form energy shells and degree of their filling depends on the number of delocalized electrons. In the region close to half-filling the cluster geometry oscillates between the prolate and oblate…

Superconductivity · Physics 2015-06-23 Vladimir Kresin , Yurii Ovchinnikov , Jacques Friedel

Understanding the substructure of atomic nuclei, particularly the clustering of nucleons inside them, is essential for comprehending nuclear dynamics. Various cluster configurations can emerge depending on excitation energy, the number and…

Electronic resonances are metastable states with finite lifetimes, encountered in processes such as photodetachment, electron transmission, and Auger decay. Resonances appear in Hermitian quantum mechanics as increased density of states in…

Chemical Physics · Physics 2025-11-10 Cansu Utku , Garrette Pauley Paran , Thomas-C. Jagau

Inclusive electron scattering off few-nucleon systems is investigated at $x>1$ and high momentum transfer, including the contributions from quasi-elastic and deep inelastic scattering processes. It is shown that at $x>1$ the inclusive cross…

Nuclear Theory · Physics 2011-04-15 S. Simula

We study the thermodynamics of Na_8 and Na_{20} clusters using multiple-histogram methods and an ab initio treatment of the valence electrons within density functional theory. We consider the influence of various electron kinetic-energy…

Atomic and Molecular Clusters · Physics 2009-11-06 Abhijat Vichare , D. G. Kanhere , S. A. Blundell

While evaporating solvent is a widely used technique to assemble nano-sized objects into desired superstructures, there has been limited work on how the assembled structures are affected by the physical aspects of the process. We present…

Soft Condensed Matter · Physics 2013-11-20 Shengfeng Cheng , Gary S. Grest

We study the formation and growth of equilibrium clusters in a suspension of weakly-charged colloidal particles and small non-adsorbing polymers. The effective potential is characterised by a short-range attraction and a long-range…

Soft Condensed Matter · Physics 2009-11-11 Rodrigo Sanchez , Paul Bartlett

Extensive first-principle calculations on embedded clusters containing few O, Y, Ti, and Cr atoms as well as vacancies are performed to obtain interaction parameters to be applied in Metropolis Monte Carlo simulations, within the framework…

Materials Science · Physics 2014-11-05 M. Posselt , D. Murali , B. K. Panigrahi
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