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First principles molecular dynamics simulations reveal a liquid-liquid phase transition in supercooled elemental silicon. Two phases coexist below $T_c\approx 1232K$. The low density phase is nearly tetra-coordinated, with a pseudogap at…

Materials Science · Physics 2009-11-13 P. Ganesh , M. Widom

Structural glasses prepared by bulk quenching a liquid melt universally exhibit puzzling low-energy excitations commonly known as the ``two-level systems'' (TLSs). Recent studies indicate that ultrastable glassy films made by vapor…

Disordered Systems and Neural Networks · Physics 2026-04-24 Vassiliy Lubchenko

Molecular dynamics simulations were carried out to test the thermodynamic theory of weakly excited, two-dimensional granular systems [Hayakawa and Hong, Phys. Rev. Lett. 78, 2764 (1997)], where granular materials are viewed as a collection…

Statistical Mechanics · Physics 2009-09-25 Paul V. Quinn , Daniel C. Hong

We present an extensive experimental study of mode-I, steady, slow crack dynamics in gelatin gels. Taking advantage of the sensitivity of the elastic stiffness to gel composition and history we confirm and extend the model for fracture of…

Soft Condensed Matter · Physics 2009-11-11 Tristan Baumberger , Christiane Caroli , David Martina

Glass-like materials are nonequilibrium systems where the relaxation time may exceed reasonable time scales of observations. In the present paper a dynamic percolation model is introduced in order to explain the principal properties of…

Condensed Matter · Physics 2007-05-23 A. Vazquez , O. Sotolongo-Costa

We propose a dynamic structure of coupled dynamic molecular strings for supercooled small polar molecule liquids and accordingly we obtain the Hamiltonian of the rotational degrees of freedom of the system. From the Hamiltonian, the…

Disordered Systems and Neural Networks · Physics 2009-11-10 Y. N. Huang , C. J. Wang , E. Riande

The study of the properties of glass-forming liquids is difficult for many reasons. Analytic solutions of mean field models are usually available only for systems embedded in a space with an unphysically high number of spatial dimensions;…

Disordered Systems and Neural Networks · Physics 2015-02-26 Manuel Sebastian Mariani , Giorgio Parisi , Corrado Rainone

Molecular dynamic simulations were employed to study a water-like model confined between hydrophobic and hydrophilic plates. The phase behavior of this system is obtained for different distances between the plates and particle-plate…

Soft Condensed Matter · Physics 2015-06-17 Leandro B. Krott , Marcia C. Barbosa

Our lives are surrounded by a rich assortment of disordered materials. In particular, glasses are well known as dense, amorphous materials, whereas gels exist in low-density, disordered states. Recent progress has provided a significant…

Soft Condensed Matter · Physics 2022-01-07 Hideyuki Mizuno , Makoto Hachiya , Atsushi Ikeda

We report a molecular dynamics simulation study of a model gel whose interaction potential is obtained by modifying the three body Stillinger-Weber model potential for silicon. The modification reduces the average coordination number, and…

Soft Condensed Matter · Physics 2015-05-14 Shibu Saw , Niels L. Ellegaard , Walter Kob , Srikanth Sastry

Interactions between colloidal particles have hitherto usually been fixed by the suspension composition. Recent experimental developments now enable the control of interactions \emph{in-situ}. Here we use Brownian dynamics simulations to…

Soft Condensed Matter · Physics 2017-02-08 C. Patrick Royall , Alex Malins

We use large-scale molecular dynamics simulations to study the kinetics of the liquid-gas phase separation if the temperature is lowered across the glass transition of the dense phase. We observe a gradual change from phase separated…

Statistical Mechanics · Physics 2011-06-01 Vincent Testard , Ludovic Berthier , Walter Kob

This perspective article reviews arguments that glass-forming liquids are different from those of standard liquid-state theory, which typically have a viscosity in the mPa$\cdot$s range and relaxation times of order picoseconds. These…

Soft Condensed Matter · Physics 2024-02-13 Jeppe C. Dyre

Using high-resolution {\sc Romulus} simulations, we explore the origin and evolution of the circumgalactic medium (CGM) in the region 0.1 $\leq \mathrm{R}/\mathrm{R}_\mathrm{500} \leq$ 1 around massive central galaxies in group-scale halos.…

Low-density "equilibrium" gels that consist of a percolated, kinetically arrested network of colloidal particles and are resilient to aging can be fabricated by restricting the number of effective bonds that form between the colloids.…

We use theory and simulations to investigate the existence of amorphous glassy states in ultrasoft colloids. We combine the hyper-netted chain approximation with mode-coupling theory to study the dynamic phase diagram of soft repulsive…

Soft Condensed Matter · Physics 2010-12-16 Ludovic Berthier , Angel J. Moreno , Grzegorz Szamel

We present simulation results addressing the dynamics of a colloidal system with attractive interactions close to gelation. Our interaction also has a soft, long range repulsive barrier which suppresses liquid-gas type phase separation at…

Soft Condensed Matter · Physics 2007-05-23 Antonio M. Puertas , Matthias Fuchs , Michael E. Cates

Glasses and gels, widely encountered amorphous solids with diverse industrial and everyday applications, share intriguing similarities such as rigidity without crystalline order and dynamic slowing down during aging. However, the underlying…

Soft Condensed Matter · Physics 2023-08-09 Yinqiao Wang , Michio Tateno , Hajime Tanaka

Solids deform and fluids flow, but soft glassy materials, such as emulsions, foams, suspensions, and pastes, exhibit an intricate mix of solid and liquid-like behavior. While much progress has been made to understand their elastic (small…

Soft Condensed Matter · Physics 2018-04-20 Simon Dagois-Bohy , Ellák Somfai , Brian P. Tighe , Martin van Hecke

Monodisperse ensembles of particles that have cluster crystalline phases at low temperatures can model a number of physical systems, such as vortices in type-1.5 superconductors, colloidal suspensions and cold atoms. In this work we study a…

Soft Condensed Matter · Physics 2019-04-29 Wenlong Wang , Rogelio Díaz-Méndez , Mats Wallin , Jack Lidmar , Egor Babaev