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The dynamical response of metallic clusters up to $10^3$ atoms is investigated using the restricted molecular dynamics simulations scheme. Exemplarily, sodium like material is considered. Correlation functions are evaluated to investigate…

Atomic and Molecular Clusters · Physics 2015-05-28 Thomas Raitza , Heidi Reinholz , Igor Morozov , Gerd Röpke

We propose a multiconfigurational hybrid density-functional theory which rigorously combines a multiconfiguration self-consistent-field calculation with a density-functional approximation based on a linear decomposition of the…

Chemical Physics · Physics 2012-08-20 Kamal Sharkas , Andreas Savin , Hans Jørgen Aa. Jensen , Julien Toulouse

An approximation for the exchange-correlation energy of reduced-density-matrix-functional theory was recently derived from a study of the homogeneous electron gas (N.N. Lathiotakis, N. Helbig, E.K.U. Gross, Phys. Rev. B 75, 195120 (2007)).…

Strongly Correlated Electrons · Physics 2009-11-13 N. N. Lathiotakis , N. Helbig , A. Zacarias , E. K. U. Gross

We identify peak and valley structures in the exact exchange-correlation potential of time-dependent density functional theory that are crucial for time-resolved electron scattering in a model one-dimensional system. These structures are…

Chemical Physics · Physics 2018-01-03 Yasumitsu Suzuki , Lionel Lacombe , Kazuyuki Watanabe , Neepa T. Maitra

Using a pi-orbital tight-binding model, we study the elastic and photoassisted transport properties of metal-molecule-metal junctions based on oligophenylenes of varying lengths. The effect of monochromatic light is modeled with an ac…

Mesoscale and Nanoscale Physics · Physics 2009-05-24 J. K. Viljas , F. Pauly , J. C. Cuevas

We investigate the accuracy and efficiency of the semiclassical Frozen Gaussian method in describing electron dynamics in real time. Model systems of two soft-Coulomb-interacting electrons are used to study correlated dynamics under…

Chemical Physics · Physics 2015-05-30 Peter Elliott , Neepa T. Maitra

Strongly correlated electron systems require the development of new theoretical schemes in order to describe their unusual and unexpected properties. The usual perturbation schemes are inadequate and new concepts must be introduced. In our…

Strongly Correlated Electrons · Physics 2016-08-31 F. Mancini , A. Avella

In this paper, we have established the couple system of a spectroscope, CCD and computer and proposed a method of the rapid measurement on spectral characteristics such as central wavelengths, relative intensities, sensitivity lines and the…

Instrumentation and Detectors · Physics 2015-12-03 Chol-Sun Kim , Chol-Su Kim , Song-Jin Im

In the presence of a (time-dependent) macroscopic electric field the electron dynamics of dielectrics cannot be described by the time-dependent density only. We present a real-time formalism that has the density and the macroscopic…

Materials Science · Physics 2016-07-27 M. Grüning , D. Sangalli , C. Attaccalite

Condensates of active particles such as cells form almost-crystalline lattices which play a central role in many biological systems. Typically, their properties have been determined merely by analogy to the rather trivial one-dimensional…

Soft Condensed Matter · Physics 2025-12-02 Connor Roberts , Gunnar Pruessner

The properties of hydrogen at warm dense matter (WDM) conditions are of high importance for the understanding of astrophysical objects and technological applications such as inertial confinement fusion. In this work, we present extensive…

Plasma Physics · Physics 2023-06-12 Tobias Dornheim , Maximilian Böhme , Zhandos Moldabekov , Jan Vorberger

We present a new density-functional method of the self-consistent electronic-structure calculation which does not exploit any local density approximations (LDA). We use the exchange-correlation energy which consists of the exact exchange…

Statistical Mechanics · Physics 2009-10-30 Takao Kotani

We present exact results for the dynamical structure function, i.e.~the density-density correlations for the 1/r^2 system of interacting particles at three special values of the coupling constant. The results are interpreted in terms of…

Condensed Matter · Physics 2016-08-31 E. R. Mucciolo , B. S. Shastry , B. D. Simons , B. L. Altshuler

A theoretical approach was developed for an exact numerical description of a pair of ultracold atoms interacting via a central potential that are trapped in a three-dimensional optical lattice. The coupling of center-of-mass and…

Quantum Physics · Physics 2013-05-29 Sergey Grishkevich , Alejandro Saenz

Molecular photo-switches as, e.g., azobenzene molecules allow, when embedded into a polymeric matrix, for photo-active polymer compounds responding mechanically when exposed to light of certain wavelength. Photo-mechanics, i.e. light-matter…

Computational Engineering, Finance, and Science · Computer Science 2020-11-24 M Mehnert , W Oates , P Steinmann

We review various theoretical methods that have been used in recent years to calculate dynamical correlation functions of many-body systems. Time-dependent correlation functions and their associated frequency spectral densities are the…

Statistical Mechanics · Physics 2020-06-01 J. Florencio , O. F. de Alcantara Bonfim

One of the most important quantities characterizing the microscopic properties of quantum systems are dynamical correlation functions. These correlations are obtained by time-evolving a perturbation of an eigenstate of the system, typically…

Quantum Physics · Physics 2025-02-26 Reinis Irmejs , Raul A. Santos

We investigate theoretically and numerically the coupling between elastic and localized surface plasmon modes in a system of gold nanocylinders separated from a thin gold film by a dielectric spacer of few nanometers thickness. That system…

A simple geometric shaping method is proposed for optical wireless communication systems based on intensity modulation and direct detection (IM/DD) from an information-theoretic perspective. Constellations consisting of equiprobable levels…

Information Theory · Computer Science 2024-12-03 Suhua Zhou , Tianqi Li , Zhaoxi Fang , Jing Zhou , Wenyi Zhang
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