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Fundamental understanding of interatomic forces in molecules must emerge from quantum mechanics, yet widely used empirical force fields rely on simplified mechanistic approximations that often fail to capture the complexity of many-body…

We introduce a novel computational approach for the investigation of complex correlated electron materials which makes it possible to evaluate interatomic forces and thereby determine atomic displacements and structural transformations…

Strongly Correlated Electrons · Physics 2014-04-24 I. Leonov , V. I. Anisimov , D. Vollhardt

This study presents a fractional-order continuum mechanics approach that allows combining selected characteristics of nonlocal elasticity, typical of classical integral and gradient formulations, under a single frame-invariant framework.…

Numerical Analysis · Mathematics 2020-05-21 Sansit Patnaik , Sai Sidhardh , Fabio Semperlotti

When the effects of dispersion are included, neither the Abraham nor the Minkowski expression for electromagnetic momentum in a dielectric medium gives the correct recoil momentum for absorbers or emitters of radiation. The total momentum…

Optics · Physics 2015-05-14 Douglas H. Bradshaw , Zhimin Shi , Robert W. Boyd , Peter W. Milonni

This work contributes to the study of non-equilibrium aspects of the Casimir forces with the introduction of squeezed states in the calculations. Throughout this article two main results can be found, being both strongly correlated.…

Quantum Physics · Physics 2017-01-18 Adrian E. Rubio Lopez

Structural and thermodynamic consistency of coarse-graining models across multiple length scales is essential for the predictive role of multi-scale modeling and molecular dynamic simulations that use mesoscale descriptions. Our approach is…

Soft Condensed Matter · Physics 2014-07-04 J. McCarty , A. J. Clark , J. Copperman , M. G. Guenza

We study the contributions of off-resonant transitions to the dynamics of a system of N multilevel atoms sharing one excitation and interacting with the quantized vector electromagnetic field. The Rotating Wave Approximation significantly…

Quantum Physics · Physics 2013-12-02 Yevhen Miroshnychenko , Klaus Mølmer

We present a review of our recent work in extending the successful dynamical mean-field theory from the equilibrium case to nonequilibrium cases. In particular, we focus on the problem of turning on a spatially uniform, but possibly time…

Strongly Correlated Electrons · Physics 2008-08-14 V. Turkowski , J. K. Freericks

Non-equilibrium Green's function theory for non-adiabatic effects in quantum transport [Kershaw and Kosov, J.Chem. Phys. 2017, 147, 224109 and J. Chem. Phys. 2018, 149, 044121] is extended to the case of interacting electrons. We consider a…

Mesoscale and Nanoscale Physics · Physics 2019-02-20 Vincent F. Kershaw , Daniel S. Kosov

The molecular junction geometry is modelled in terms of nuclear degrees of freedom that are embedded in a stochastic quantum environment of non-equilibrium electrons. Time-evolution of the molecular geometry is governed via a mean force, a…

Mesoscale and Nanoscale Physics · Physics 2020-10-28 Vincent F. Kershaw , Daniel S. Kosov

The impact of lossy multi-layer structures on nonequilibrium atom-surface interactions is discussed. Specifically, the focus lies on a fully non-Markovian and nonequilibrium description of quantum friction, the fluctuation-induced drag…

Mesoscale and Nanoscale Physics · Physics 2018-06-27 Marty Oelschläger , Kurt Busch , Francesco Intravaia

We study the phenomenon of quantum friction in a system consisting of a polarizable atom moving at a constant speed parallel to a metallic plate. The metal is described using a charged hydrodynamic model for the electrons. This model…

Quantum Physics · Physics 2020-12-21 Kunmin Wu , Thomas L. Schmidt , M. Belén Farias

We introduce a group-theoretical extension of the Dicke model which describes an ensemble of two-level atoms interacting with a finite radiation field. The latter is described by a spin model whose main feature is that it possesses a…

Quantum Physics · Physics 2020-06-17 L. F. Quezada , A. Martín-Ruiz , A. Frank

Classical atomistic simulations based on interatomic potentials resolve lattice instabilities, defect nucleation, and microstructure evolution with high fidelity, but their accessible system sizes remain far below those required for…

Numerical Analysis · Mathematics 2026-05-26 Aagashram Neelakandan , Karsten Albe , Bernhard Eidel

We present an approach for carrying out non-adiabatic molecular dynamics simulations of systems in which non-adiabatic transitions arise from the coupling between the classical atomic motions and a quasi-continuum of electronic quantum…

Computational Physics · Physics 2018-11-21 Jerome Daligault , Dmitry Mozyrsky

We experimentally investigate the distribution of the non-equilibrium work done by an external force on a mesoscopic system with many coupled degrees of freedom: a colloidal monolayer mechanically driven across a periodic light field. Since…

Statistical Mechanics · Physics 2015-04-30 Juan Ruben Gomez-Solano , Christoph July , Jakob Mehl , Clemens Bechinger

We review some recent coarse-graining and multi-scale methods, but also put forward some new ideas for addressing such issues. We find that, if one is guided by nonequilibrium statistical mechanics and thermodynamics, it is possible to…

Soft Condensed Matter · Physics 2009-11-06 Patrick Ilg , Vlasis Mavrantzas , Hans Christian Öttinger

The decay of an excited atom in the presence of a medium that both scatters and absorbs radiation is studied with the help of a quantum-electrodynamical model. The medium is represented by a half space filled with a randomly distributed set…

Quantum Physics · Physics 2018-07-23 L. G. Suttorp , A. J. van Wonderen

The paper introduces a simple quantum model to calculate in a general way allowed frequencies and energy levels of the anharmonic oscillator. The theoretical basis of the approach has been introduced in two early papers aimed to infer the…

Quantum Physics · Physics 2011-05-19 Sebastiano Tosto

We consider the problem of computing energy distribution of inner harmonic oscillations of a nanoparticle in its phase space, when the particle moves in a medium in heat equilibrium under certain temperature. It is assumed that the particle…

Mathematical Physics · Physics 2016-10-04 E. M. Beniaminov