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X-ray diffraction with synchrotron radiation has been used for the first time to study chemical interaction in the FeO-ZnO system at 4.8 GPa and temperatures up to 1300 K. Above 750 K, the chemical reaction between FeO and ZnO has been…

Materials Science · Physics 2011-02-09 P. S. Sokolov , A. N. Baranov , C. Lathe , V. L. Solozhenko

Series of metastable Me1-xZnxO solid solutions (Me = Ni2+, Co2+, Fe2+, Mn2+) with the rocksalt (rs) crystal structure have been synthesized from the binary oxides by quenching from 7.7 GPa and 1450-1650 K. Phase composition of the samples,…

Materials Science · Physics 2011-02-04 A. N. Baranov , P. S. Sokolov , O. O. Kurakevych , V. A. Tafeenko , D. Trots , V. L. Solozhenko

Metastable LiMeO2-ZnO (Me = Fe3+, Ti3+) solid solutions with rock salt crystal structure have been synthesized by solid state reaction of ZnO with LiMeO2 complex oxides at 7.7 GPa and 1350-1450 K. Structure, phase composition, thermal…

Materials Science · Physics 2011-05-31 P. S. Sokolov , A. N. Baranov , V. A. Tafeenko , V. L. Solozhenko

Lattice parameter of metastable high-pressure phase of zinc oxide, rock-salt ZnO was measured in the 10-300 K temperature range using synchrotron X-ray powder diffraction. No phase transition was observed down to 10 K. The lattice parameter…

Materials Science · Physics 2013-10-28 Petr S. Sokolov , Andrey N. Baranov , Anthony M. T. Bell , Vladimir L. Solozhenko

FeXMn1-XS (0 <x< 0.3) synthesized on the basis of {\alpha}-MnS are the novel Mott-type substances with the rock salt structure. Neutron diffraction study shows that the shift of the Neel temperature of these materials from 150 (x = 0) to…

Cubic zinc oxide (rs-ZnO), metastable under normal conditions, was synthesized from the wurtzite modification (w-ZnO) at 7.7 GPa and ~800 K in the form of nanoparticles isolated in the NaCl matrix. The phase transition rs-ZnO \rightarrow…

Materials Science · Physics 2011-02-09 P. S. Sokolov , A. N. Baranov , Zh. V. Dobrokhotova , V. L. Solozhenko

The phase diagram of Zn has been explored up to 140 GPa and 6000 K, by combining optical observations, x-ray diffraction, and ab-initio calculations. In the pressure range covered by this study, Zn is found to retain a hexagonal…

The Zn K-edge X-ray absorption spectroscopy has been used to investigate in situ the decomposition of zinc peroxide (ZnO$_2$) to zinc oxide (ZnO). Principal component and linear combination analyses of the EXAFS spectra have been employed…

Materials Science · Physics 2022-10-03 Alexei Kuzmin , Inga Pudza , Konstantin Klementiev

The enthalpies of dissolution of metastable rock salt and thermodynamically stable wurtzite polymorphs of zinc oxide in aqueous H2SO4 have been measured in direct calorimetric experiments at 303 K and 0.1 MPa and the obtained results…

Materials Science · Physics 2017-11-01 Felix Yu. Sharikov , Petr S. Sokolov , Andrey N. Baranov , Vladimir L. Solozhenko

The structure of La$_{1-x}$Ca$_{x}$MnO$_{3}$ solid solutions (x=0, 0.25, 0.50, 0.67, 1) under high pressure (up to 40-45 GPa) has been investigated by synchrotron X-ray powder diffraction (XRD) in order to characterize their volume…

Strongly Correlated Electrons · Physics 2007-05-23 A. Sani , C. Meneghini , S. Mobilio , Sugata Ray , D. D. Sarma , J. A. Alonso

Low-temperature heat capacities (Cp) of nanostructured rock salt (rs-ZnO) and wurtzite (w-ZnO) polymorphs of zinc oxide were measured in the 2-315 K temperature range. No significant influence of nanostructuring on Cp of w-ZnO has been…

In this paper we report structural and optical properties of Magnesium substituted Zinc Oxide (Zn1-xMgxO) nanocrystals (~10-12nm) synthesized by low temperature route. In the low temperature synthesis route it was possible to reach x = 0.17…

Materials Science · Physics 2011-09-15 Manoranjan Ghosh , A. K. Raychaudhuri

Nanostructured Zinc oxide (ZnO) was synthesized via a ball milling for 10 hours using high energy planetary ball mill. Phase purity and homogeneity of all the samples have been investigated by X-ray diffraction (XRD) and Field Emission…

Materials Science · Physics 2015-06-11 Pawan Kumar , M. Kar , Anup V. Sanchela , C. V. Tomy , Ajay D. Thakur

High entropy oxides (HEO)s have garnered much interest due to their available high degree of tunability. Here, we study the local structure of (MgNiCuCoZn)0.167(MnCr)0.083O, a composition based on the parent HEO (MgNiCuCoZn)0.2O.We…

Structural investigation on $Co_{3-x}Mn_xTeO_6$; ($0 \lt x \le 2$) solid solutions as a function of Mn concentration using Synchrotron X-ray diffraction (SXRD) and XANES measurements are presented. Phase diagram obtained from Rietveld…

Materials Science · Physics 2014-04-08 Harishchandra Singh , A. K. Sinha , Haranath Ghosh , M. N. Singh , Parasmani Rajput

We report the results of an x-ray scattering study that reveals oxidation kinetics and formation of a previously unreported crystalline phase of SnO at the liquid-vapour interface of Sn. Our experiments reveal that the pure liquid Sn…

The effect of Mg-substitution on the crystal structure of wurtzite ZnO is presented based on synchrotron X-ray diffraction studies of polycrystalline Zn1-xMgxO (0 <= x <= 0.15). Increase in Mg concentration results in pronounced c-axis…

Materials Science · Physics 2007-05-23 Young-Il Kim , Katharine Page , Ram Seshadri

Ternary nitride materials hold promise for many optical, electronic, and refractory applications yet their preparation via solid-state synthesis remains challenging. Often, high pressures or reactive gasses are used to manipulate the…

Materials Science · Physics 2021-08-19 Paul K. Todd , M. Jewels Fallon , James R. Neilson , Andriy Zakutayev

The influence of thermal disorder and static distortions on the local structure in microcrystalline solid solutions of tungstates ZncNi1-cWO4 with c=0.0-1.0 was investigated using temperature-dependent (10-300 K) x-ray absorption…

Materials Science · Physics 2020-12-24 G. Bakradze , A. Kalinko , A. Kuzmin

The structural phase transitions and the fundamental band gaps of Mg(x)Zn(1-x)O alloys are investigated by detailed first-principles calculations in the entire range of Mg concentrations x, applying a multiple-scattering theoretical…

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