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Solutions of semiflexible polymers confined by repulsive planar walls are studied by density functional theory and Molecular Dynamics simulations, to clarify the competition between the chain alignment favored by the wall and the depletion…

Soft Condensed Matter · Physics 2016-05-25 Sergei A. Egorov , Andrey Milchev , Peter Virnau , Kurt Binder

Binary mixtures of semiflexible polymers with the same chain length but different persistence lengths separate into two coexisting different nematic phases when the osmotic pressure of the lyotropic solution is varied. Molecular Dynamics…

Soft Condensed Matter · Physics 2020-09-15 Andrey Milchev , Sergei A. Egorov , Jiarul Midya , Kurt Binder , Arash Nikoubashman

There is so far no clear-cut experimental analysis that can determine whether dipole-dipole interactions enhance or reduce the blocking temperature $T_{B}$ of nanoparticle assemblies. It seems that the samples play a central role in the…

Mesoscale and Nanoscale Physics · Physics 2019-07-12 F. Vernay , H. Kachkachi

We present simulation results for a model polymer melt, consisting of short, nonentangled chains, in the supercooled state. The analysis focuses on the monomer dynamics, which is monitored by the incoherent intermediate scattering function.…

Soft Condensed Matter · Physics 2007-05-23 C. Bennemann , J. Baschnagel , W. Paul

We report a numerical study of the diffusiophoresis of short polymers using non-equilibrium molecular dynamics simulations. More precisely, we consider polymer chains in a fluid containing a solute which has a concentration gradient, and…

Soft Condensed Matter · Physics 2020-05-20 Simón Ramírez-Hinestrosa , Hiroaki Yoshida , Lydéric Bocquet , Daan Frenkel

We investigate the thermal and structural properties of knotted diblock copolymer rings using a coarse-grained lattice model in an implicit solvent. The system is studied by means of the Wang--Landau Monte Carlo algorithm, allowing us to…

Soft Condensed Matter · Physics 2026-05-18 Neda Abbasi Taklimi , Franco Ferrari , Marcin R. Piątek , Luca Tubiana

Oriented block copolymers exhibit a buckling instability when submitted to a tensile test perpendicular to the lamellae direction. In this paper we study this behavior using a coarse grained molecular dynamics simulation approach. Coarse…

Materials Science · Physics 2014-03-05 Ali Makke , Olivier Lame , Michel Perez , Jean-Louis Barrat

We study the conformational properties of heteropolymers containing two types of monomers A and B, modeled as self-avoiding random walks on a regular lattice. Such a model can describe in particular the sequences of hydrophobic and…

Disordered Systems and Neural Networks · Physics 2014-09-01 Viktoria Blavatska , Wolfhard Janke

Molecular dynamics simulations were conducted to investigate the dynamic properties of melts of nonconcatenated ring polymers and compared to melts of linear polymers. The longest rings were composed of N=1600 monomers per chain which…

Soft Condensed Matter · Physics 2011-05-02 Jonathan D. Halverson , Won Bo Lee , Gary S. Grest , Alexander Y. Grosberg , Kurt Kremer

Understanding the (de)mixing behavior of multicomponent lipid bilayers is an important step towards unraveling the nature of spatial composition heterogeneities in cellular membranes and their role in biological function. We use…

Soft Condensed Matter · Physics 2018-05-17 Shushan He , Lutz Maibaum

In this work, Flory-Huggins phase diagrams for correlated random copolymers with realistic chain lengths are calculated. This is achieved in two steps. At first we derive a distribution function of copolymer chains with respect to…

Soft Condensed Matter · Physics 2021-03-17 Elena Patyukova , Erte Xi , Mark R. Wilson

Amphiphilic block copolymer solutions form various micellar structures including micelles and vesicles. We applied the density functional theory for block copolymers which we have proposed to amphiphilic block copolymer systems. The 3…

Soft Condensed Matter · Physics 2007-05-23 Takashi Uneyama , Masao Doi

We derive the mean-field theory of disordered block-copolymers composed of two monomeric species, combining Edwards' functional method with the replica technique of disordered systems. In the absence of disorder we recover the canonical…

Soft Condensed Matter · Physics 2011-01-17 Gabriele Migliorini

A technique is presented which maps the parameters of a bead spring model, using the Flory Huggins theory, to a specific experimental system. By keeping only necessary details, for the description of these systems, the mapping procedure…

Soft Condensed Matter · Physics 2016-04-19 George J. Papakonstantopoulos , Kostas Ch. Daoulas , Marcus Muller , Juan J. de Pablo

In this paper we extend the Gaussian self-consistent method to permit study of the equilibrium and kinetics of conformational transitions for heteropolymers with any given primary sequence. The kinetic equations earlier derived by us are…

Soft Condensed Matter · Physics 2009-10-31 E. G. Timoshenko , Yu. A. Kuznetsov , K. A. Dawson

We consider the dynamics of freely translating and rotating diblock (A-B), Gaussian copolymers, in dilute solutions. Using the multiple scattering technique, we have computed the diffusion and the friction coefficients D_AB and Zeta_AB, and…

Soft Condensed Matter · Physics 2009-10-30 Radu P. Mondescu , M. Muthukumar

Amphiphilic block copolymers self-assemble into diverse nanoscale morphologies with significant implications for drug delivery. This work presents systematic Brownian dynamics simulations of multi-chain diblock and triblock copolymers…

Soft Condensed Matter · Physics 2026-04-21 Ehsan Kamali Ahangar , Dominic Robe , Elnaz Hajizadeh

Photon correlation spectroscopy and rheological measurements are performed to investigate the microscopic dynamics and mechanical responses of aqueous solutions of triblock copolymers and aqueous mixtures of triblock copolymers and anionic…

Soft Condensed Matter · Physics 2011-09-28 Rajib Basak , Nabaneeta Mukhopadhyay , Ranjini Bandyopadhyay

We examine the condensed states of a simple semiflexible copolymer in which there are two monomer types that are immiscible with each other and with the solvent. Although this is similar to the well known problem of collapse for a…

Soft Condensed Matter · Physics 2007-05-23 E. Hernandez-Zapata , I. R. Cooke , D. R. M. Williams

The effects of the length of each hydrophobic end block N_{st} and polymer concentration \bar{\phi}_{P} on the transition broadness in amphiphilic ABA symmetric triblock copolymer solutions are studied using the self-consistent field…

Soft Condensed Matter · Physics 2013-09-25 X. -G. Han , Y. -H. Ma , S. -L. Ouyang