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The lifetimes of the lower-lying vibrational states of ultralong-range strontium Rydberg molecules comprising one ground-state 5s2 1S0 atom and one Rydberg atom in the 5s38s 3S1 state are reported. The molecules are created in an ultracold…

We perform a comprehensive investigation of the coupling between a Rydberg-dressed atomic gas and an ultra-cold plasma. Using simultaneous time-resolved measurements of both neutral atoms and ions, we show that plasma formation occurs via a…

Atomic Physics · Physics 2019-09-04 A. D. Bounds , N. C. Jackson , R. K. Hanley , E. M. Bridge , P. Huillery , M. P. A. Jones

By investigating the quantum properties of magnetically trapped nS Rydberg atoms, it is demonstrated that the composite nature of Rydberg atoms significantly alters their trapping properties opposed to point-like particles with the same…

Atomic Physics · Physics 2009-04-22 M. Mayle , I. Lesanovsky , P. Schmelcher

We study a novel regime of the Rydberg excitation blockade using highly Stark-shifted, yet long-living, states of Rb atoms subject to electric fields above the classical ionization limit. Such states allow tuning the dipole-dipole…

We present experimental evidence for spin-orbit interaction of an electron as it scatters from a neutral atom. The scattering process takes place within a Rb$_2$ ultralong-range Rydberg molecule, consisting of a Rydberg atomic core, a…

We investigate a possible mechanism for the autoionization of ultracold Rydberg gases, based on the resonant coupling of Rydberg pair states to the ionization continuum. Unlike an atomic collision where the wave functions begin to overlap,…

Atomic Physics · Physics 2015-05-13 T. Amthor , J. Denskat , C. Giese , N. N. Bezuglov , A. Ekers , L. Cederbaum , M. Weidemüller

We investigate the dynamics of Rydberg electrons excited from the ground state of ultracold atoms trapped in an optical lattice. We first consider a lattice comprising an array of double-well potentials, where each double well is occupied…

Other Condensed Matter · Physics 2009-11-13 B. Vaucher , S. J. Thwaite , D. Jaksch

Since their first experimental observation, ultralong-range Rydberg molecules consisting of a highly excited Rydberg atom and a ground state atom have attracted the interest in the field of ultracold chemistry. Especially the intriguing…

A Rydberg molecule is composed of an outer electron that collides on the residual ionic core. Typical states of Rydberg molecules display entanglement between the outer electron and the core. In this work we quantify the average…

Quantum Physics · Physics 2007-05-23 M Lombardi , A Matzkin

We report on the induction of magnetization in Rydberg systems by means of the inverse Faraday effect, and propose the appearance of the effect in two such systems, Rydberg atoms proper and shallow dopants in semiconductors. Rydberg atoms…

Atomic Physics · Physics 2025-03-05 Patrick J. Wong , Ivan M. Khaymovich , Gabriel Aeppli , Alexander V. Balatsky

Mean-field energy-level shifts arising as a result of strong electrostatic dipole interactions within dilute gases of polarized helium Rydberg atoms have been probed by microwave spectroscopy. The Rydberg states studied had principal…

Atomic Physics · Physics 2016-11-28 V. Zhelyazkova , R. Jirschik , S. D. Hogan

The level structure of negative-ions near the electron detachment limit dictates the low-energy scattering of an electron with the parent neutral atom. We demonstrate that a single ultracold atom bound inside a Rydberg orbit forming an…

We report on the observation of interactions between ultracold Rydberg atoms and ions in a Paul trap. The rate of observed inelastic collisions, which manifest themselves as charge transfer between the Rydberg atoms and ions, exceeds that…

Atomic Physics · Physics 2019-07-03 N. V. Ewald , T. Feldker , H. Hirzler , H. Fürst , R. Gerritsma

We report the observation of dipole-forbidden, but quadrupole-allowed, one-photon transitions to high Rydberg states in Rb. Using pulsed UV excitation of ultracold atoms in a magneto-optical trap, we excite $5s \to nd$ transitions over a…

Cold atomic gases resonantly excited to Rydberg states can exhibit strong optical nonlinearity at the single photon level. We observe that in such samples radiation trapping leads to an additional mechanism for Rydberg excitation.…

Atomic Physics · Physics 2017-03-16 D. P. Sadler , E. M. Bridge , D. Boddy , A. D. Bounds , N. C. Keegan , G. Lochead , M. P. A. Jones , B. Olmos

Vibrational dynamics in conventional molecules usually takes place on a timescale of picoseconds or shorter. A striking exception are ultralong-range Rydberg molecules, for which dynamics is dramatically slowed down as a consequence of the…

The coupling of weak light fields to Rydberg states of atoms under conditions of electromagnetically induced transparency (EIT) leads to the formation of Rydberg polaritons which are quasi-particles with tunable effective mass and…

Quantum Physics · Physics 2013-09-17 Johannes Otterbach , Matthias Moos , Dominik Muth , Michael Fleischhauer

Ultracold polar molecules offer the possibility of exploring quantum gases with interparticle interactions that are strong, long-range, and spatially anisotropic. This is in stark contrast to the dilute gases of ultracold atoms, which have…

Atomic Physics · Physics 2015-05-18 K. -K. Ni , S. Ospelkaus , D. Wang , G. Quemener , B. Neyenhuis , M. H. G. de Miranda , J. L. Bohn , J. Ye , D. S. Jin

We introduce the Rydberg Composite, a new class of Rydberg matter where a single Rydberg atom is interfaced with a dense environment of neutral ground state atoms. The properties of the Composite depend on both the Rydberg excitation, which…

Atomic Physics · Physics 2020-09-02 Andrew L. Hunter , Matthew T. Eiles , Alex Eisfeld , Jan M. Rost

In excited molecules, the interaction between the covalent Rydberg and ion-pair channels forms a unique class of excited Rydberg states, in which the infinite manifold of vibrational levels are the equivalent of atomic Rydberg states with a…

Atomic Physics · Physics 2016-06-22 Samuel Markson , Hossein Sadeghpour