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This work is devoted to the \textit{ab initio} calculation of transport and optical properties of aluminum. The calculation is based on the quantum molecular dynamics simulation, density functional theory and the Kubo-Greenwood formula.…

Computational Physics · Physics 2013-10-16 D. V. Knyazev , P. R. Levashov

In order to provide a comprehensive theoretical description of MgSiO$_3$ at extreme conditions, we combine results from path integral Monte Carlo (PIMC) and density functional molecular dynamics simulations (DFT-MD) and generate a…

Materials Science · Physics 2020-02-19 Felipe González-Cataldo , François Soubiran , Henry Peterson , Burkhard Militzer

The equation of state and the shock Hugoniot of deuterium are calculated using a first-principles approach, for the conditions of the recent shock experiments. We use density functional theory within a classical mapping of the quantum…

Strongly Correlated Electrons · Physics 2017-03-22 M. W. C. Dharma-wardana , Francois Perrot

Using density functional theory molecular dynamics simulations, we predict shock Hugoniot curves of precompressed methane up to 75000 K for initial densities ranging from 0.35 to 0.70 g/cc. At 4000 K, we observe the transformation into a…

Materials Science · Physics 2015-06-05 Benjamin L. Sherman , Hugh F. Wilson , Dayanthie Weeraratne , Burkhard Militzer

Using two first-principles computer simulation techniques, path integral Monte-Carlo and density functional theory molecular dynamics, we derive the equation of state of magnesium in the regime of warm dense matter, with densities ranging…

Materials Science · Physics 2020-08-20 Felipe González-Cataldo , François Soubiran , Burkhard Militzer

Density Functional Theory calculations using the quasi-harmonic approximation have been used to calculate the solid Hugoniot of two polytypes of boron carbide up to 100 GPa. Under the assumption that segregation into the elemental phases…

Materials Science · Physics 2017-06-28 Andrew Shamp , Eva Zurek , Tadashi Ogitsu , Dayne E. Fratanduono , Sebastien Hamel

Using path integral Monte Carlo and density functional molecular dynamics (DFT-MD) simulations, we study the properties of MgSiO$_3$ enstatite in the regime of warm dense matter. We generate a consistent equation of state (EOS) that spans…

Materials Science · Physics 2020-12-02 Felipe González-Cataldo , Burkhard Militzer

Shock compression of silicon (Si) under extremely high pressures (>100 Mbar) was investigated by using two first-principles methods of orbital-free molecular dynamics (OFMD) and path integral Monte Carlo (PIMC). While pressures from the two…

Materials Science · Physics 2016-12-21 S. X. Hu , B. Militzer , L. A. Collins , K. P. Driver , J. D. Kress

We use path integral Monte Carlo and density functional molecular dynamics to construct a coherent set of equation of state for a series of hydrocarbon materials with various C:H ratios (2:1, 1:1, 2:3, 1:2, and 1:4) over the range of…

Plasma Physics · Physics 2017-07-26 Shuai Zhang , Kevin P. Driver , François Soubiran , Burkhard Militzer

We calculate the equation of state of dense deuterium with two ab initio simulations techniques, path integral Monte Carlo and density functional theory molecular dynamics, in the density range of 0.67 < rho < 1.60 g/cc. We derive the…

Soft Condensed Matter · Physics 2009-11-07 B. Militzer , D. M. Ceperley , J. D. Kress , J. D. Johnson , L. A. Collins , S. Mazevet

The properties of hot dense helium at megabar pressures were studied with two first-principles computer simulation techniques, path integral Monte Carlo and density functional molecular dynamics. The simulations predicted that the…

Materials Science · Physics 2009-11-11 B. Militzer

This study overviews and extends a recently developed stochastic finite-temperature Kohn-Sham density functional theory to study warm dense matter using Langevin dynamics, specifically under periodic boundary conditions. The method's…

Materials Science · Physics 2024-04-16 Rebecca Efrat Hadad , Argha Roy , Eran Rabani , Ronald Redmer , Roi Baer

Recent laser-shock experiments on an H--He mixture containing 11~$\%$ helium (atomic fraction) have suggested the presence of an immiscibility region inside Jupiter. Reflectivity measurements were used as the primary diagnostic of H--He…

Other Condensed Matter · Physics 2026-05-05 Ammar A. Ellaboudy , Valentin V. Karasiev , S. X. Hu

A caloric model, which describes the pressure--density--internal-energy relationship in a broad region of condensed-phase states, is applied for tungsten. As distinct from previously known caloric equations of state for this material, a new…

Materials Science · Physics 2015-11-18 Konstantin V. Khishchenko

We present estimates of the critical properties, thermodynamic functions, and principal shock Hugoniot of hot dense aluminum fluid as predicted from a chemical model for the equation-of-state of hot dense, partially ionized and partially…

Plasma Physics · Physics 2018-04-04 Mofreh R. Zaghloul

We perform all-electron path integral Monte Carlo (PIMC) and density functional theory molecular dynamics (DFT-MD) calculations to explore warm dense matter states of oxygen. Our simulations cover a wide density-temperature range of…

Plasma Physics · Physics 2016-01-22 K. P. Driver , F. Soubiran , Shuai Zhang , B. Militzer

Using Kubo's linear response theory, we derive expressions for the frequency-dependent electrical conductivity (Kubo-Greenwood formula), thermopower, and thermal conductivity in a strongly correlated electron system. These are evaluated…

Plasma Physics · Physics 2012-05-04 Bastian Holst , Martin French , Ronald Redmer

Quantum molecular dynamic (QMD) simulations have been applied to study the thermophysical properties of liquid xenon under dynamic compressions. The equation of state (EOS) obtained from QMD calculations are corrected according to Saha…

Materials Science · Physics 2010-05-13 Cong Wang , Yun-Jun Gu , Qi-Feng Chen , Xian-Tu He , Ping Zhang

A systematic study of the Hugoniot equation of state, phase transition, and the other thermodynamic properties including the Hugoniot temperature, the electronic and ionic heat capacities, and the Gr\"{u}neisen parameter for…

Materials Science · Physics 2007-05-23 Qili Zhang , Ping Zhang , Haifeng Song , Haifeng Liu

We study the high-pressure melting behavior of titanium using laser-driven shock compression with in situ femtosecond x-ray diffraction and molecular-dynamics simulations based on a machine-learned interatomic potential. The MD simulations…