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In most of the realistic ab initio and model calculations which have appeared on the emission of light from Si nanocrystals, the role of surface oxygen has been usually ignored, underestimated or completely ruled out. We investigate…

Mesoscale and Nanoscale Physics · Physics 2016-08-03 Shanawer Niaz , Aristides D. Zdetsis , Emmanuel N. Koukaras , Oguz Gulseren , Imran Sadiq

In this work, atomic calculations were performed within the local-density and generalized-gradient approximations of exchange and correlation density functionals within density-functional theory to provide accurate periodic trends of first…

Atomic Physics · Physics 2016-11-04 Mauro Ribeiro

The oxidation of magnetite to maghemite is a naturally occurring process that leads to the degradation of the magnetic properties of magnetite nanoparticles. Despite being systematically observed with traditional macroscopic magnetization…

A magnetite (Fe3O4) single crystal (111) surface has been studied at various oxygen-iron surface stoichiometries. The stoichiometry was modified by controlling the in-situ sample anneal conditions. We have found the conditions that lead to…

Soft Condensed Matter · Physics 2007-05-23 N. Berdunov , S. Murphy , G. Mariotto , I. V. Shvets

Bimetallic nanoparticles are widely studied, for example in catalysis. However, possible restructuring in the environment of use, such as segregation or alloying, may occur. Taken individually, state-of-the-art analytical tools fail to give…

Materials Science · Physics 2018-11-19 Sophie Carenco , Cecile S. Bonifacio , Judith C. Yang

We present a new methodology to analyze complicated multi-physics simulations by introducing a fictitious parameter. Using the method, we study quantum mechanical aspects of an organic molecule in water. The simulation is variationally…

Chaotic Dynamics · Physics 2007-05-23 Toshiya Takami , Jun Maki , Jun-ichi Ooba , Taizo Kobayashi , Rie Nogita , Mutsumi Aoyagi

Quantum molecular dynamic simulations are introduced to study the shock compressed oxygen. The principal Hugoniot points derived from the equation of state agree well with the available experimental data. With the increase of pressure,…

Materials Science · Physics 2015-05-14 Cong Wang , Ping Zhang

The isotope effect in the scattering of methane is studied by wavepacket simulations of oriented CH4 and CD4 molecules from a flat surface including all nine internal vibrations. At a translational energy up to 96 kJ/mol we find that the…

Chemical Physics · Physics 2009-11-06 R. Milot , A. P. J. Jansen

The angular distribution function of multiple scattering experienced by 855 MeV electrons passing through an amorphous silicon plate and an oriented silicon crystal has been studied by means of relativistic molecular dynamics simulations…

Oxygen exchange at oxide/liquid and oxide/gas interfaces is important in technology and environmental studies, as it is closely linked to both catalytic activity and material degradation. The atomic-scale details are mostly unknown,…

The solvation structures and ion dynamics of CaCl$_2$ aqueous electrolytes have been investigated using ab initio molecular dynamics simulations and molecular dynamics simulations with deep learning potentials. We found multiple solvation…

Chemical Physics · Physics 2023-07-20 Zhou Yu , Lei Cheng

We present results of molecular dynamics simulations of the electron system on the surface of liquid helium. The simulations are done for 1600 electrons with periodic boundary conditions. Electron scattering by capillary waves and phonons…

Mesoscale and Nanoscale Physics · Physics 2018-09-03 K. Moskovtsev amd M. I. Dykman

Silicon-oxygen compounds are among the most important ones in the natural sciences, occurring as building blocks in minerals and being used in semiconductors and catalysis. Beyond the well known silicon dioxide, there are phases with…

Materials Science · Physics 2025-04-16 Linus C. Erhard , Jochen Rohrer , Karsten Albe , Volker L. Deringer

For a long time a crystal structure of high-pressure epsilon-phase of solid oxygen was a mistery. Basing on the results of recent experiments that have solved this riddle we show that the magnetic and crystal structure of epsilon-phase can…

Statistical Mechanics · Physics 2010-03-16 Helen V. Gomonay , Vadim M. Loktev

We study the effect of different heating rates of a dilute Bose gas confined in a quasi-1D finite, leaky box. An optical kicked-rotor is used to transfer energy to the atoms while two repulsive optical beams are used to confine the atoms.…

Atomic Physics · Physics 2007-05-23 K. Henderson , H. Kelkar , T. C. Li , B. Gutierrez-Medina , M. G. Raizen

The emergence of superlattice periodicities at metal to insulator transitions in hole doped perovskite oxides responds to a rearrangement of the local atomic structure, and electron and spin density distribution. Originally, the ionic model…

Strongly Correlated Electrons · Physics 2015-05-14 Javier Herrero-Martin , Joaquín García , Blasco Javier , Claudio Mazzoli , G. Subías

The locally self-consistent real space multiple scattering technique has been applied to calculate the electronic structure and chemical binding for the c(2x2)O/Cu(001) system, as a function of $d_{O-Cu1}$ -- the height of oxygen above the…

Materials Science · Physics 2009-11-07 Sergey Stolbov , Abdelkader Kara , Talat S. Rahman

Manipulation of oxygen vacancies (V_O) in single oxide layers by varying the electric field can result in significant modulation of the ground state. However, in many oxide multilayers with strong application potentials, e.g. ferroelectric…

Applied Physics · Physics 2017-12-06 B. Cui , C. Song , F. Li , X. Y. Zhong , Z. C. Wang , P. Werner , Y. D. Gu , H. Q. Wu , J. J. Peng , M. S. Saleem , S. S. P. Parkin , F. Pan

We investigate the structural and dynamical properties of binary aluminum-titanium liquid metallic alloys, as a function of temperature and composition. We make use of MD-simulations, using a transferable machine-learning potential…

Controlled introduction of oxygen vacancies offers an effective route to induce metal-to-insulator transition in strongly correlated rare-earth nickelates ($R$NiO$_3$) at room temperature. However, the role played by the rare-earth cations…

Materials Science · Physics 2024-12-30 Devang Bhagat , Ranga Teja Pidathala , Badri Narayanan