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The complexation of a polyelectrolyte with an oppositely charged spherical macroion is studied for both salt free and salty solutions. When a polyelectrolyte winds around the macroion, its turns repel each other and form an almost…

Soft Condensed Matter · Physics 2009-10-31 T. T. Nguyen , B. I. Shklovskii

Polymer electrolytes typically exhibit diminished ionic conductivity due to the presence of correlation effects between the cations and anions. Microscopically, transient ionic aggregates, e.g. {\it ion-pairs}, {\it ion-triplets} or higher…

Materials Science · Physics 2008-04-15 Arijit Maitra , Andreas Heuer

A novel statistical model for the cooperative binding of monomeric ligands to a linear lattice is developed to study the interaction of ionic surfactant molecules with flexible polyion chain in dilute solution. Electrostatic binding of a…

Soft Condensed Matter · Physics 2015-01-13 T. Nishio , T. Shimizu , Sh. Yoshida , A. Minakata

We study the effective interaction between a planar array of uniformly negatively charged, stiff rods parallel to a negatively charged planar substrate in the absence of salt in a continuous, isotropic dielectric medium. Using Brownian…

Soft Condensed Matter · Physics 2009-10-31 R. Jay Mashl , Niels Grønbech-Jensen

We use the recently developed soft-potential-enhanced Poisson-Boltzmann (SPB) theory to study the interaction between two parallel polyelectrolytes (PEs) in monovalent ionic solutions in the weak-coupling regime. The SPB theory is fitted to…

Soft Condensed Matter · Physics 2022-09-28 Xiang Yang , Alberto Scacchi , Hossein Vahid , Maria Sammalkorpi , Tapio Ala-Nissila

In this article we develop an algorithm for the efficient simulation of electrolytes in the presence of physical boundaries. In previous work the Discrete Ion Stochastic Continuum Overdamped Solvent (DISCOS) algorithm was derived for triply…

We investigate the interaction between highly charged lipid bilayers in the presence of monovalent counterions. Neutron and X-ray reflectivity experiments show that the water layer between like-charged bilayers is thinner than for…

Recently developed analytic approximation for the equation of state of fully ionized nonideal electron-ion plasma mixtures [Potekhin et al., Phys. Rev. E, 79, 016411 (2009); arXiv:0812.4344], which covers the transition between the weak and…

Plasma Physics · Physics 2010-02-01 A. Y. Potekhin , G. Chabrier , A. I. Chugunov , H. E. DeWitt , F. J. Rogers

We investigate the effect of quenched surface charge disorder on electrostatic interactions between two charged surfaces in the presence of dielectric inhomogeneities and added salt. We show that in the linear weak-coupling regime (i.e., by…

Soft Condensed Matter · Physics 2007-05-23 Rudolf Podgornik , Ali Naji

Ion clustering has been proposed as a mechanism leading to the peculiar 'anomalous underscreening' phenomenon seen for electrostatic interactions between charge surfaces immersed in concentrated electrolytes. These interactions have been…

Soft Condensed Matter · Physics 2025-12-01 Clifford E. Woodward , David Ribar , Jan Forsman

We present results of molecular dynamics simulations of strong, flexible polyelectrolyte chains in solution with added salt. The effect of added salt on the polyelectrolyte chain structure is fully treated for the first time as a function…

Soft Condensed Matter · Physics 2008-02-03 Mark J. Stevens , Steve Plimpton

We study a solution of long polyanions (PA) with shorter polycations (PC) and focus on the role of Coulomb interaction. A good example is solutions of DNA and PC which are widely studied for gene therapy. In the solution, each PA attracts…

Soft Condensed Matter · Physics 2025-02-11 Rui Zhang , B. I. Shklovskii

We develop a lattice-based Monte Carlo simulation method for charged mixtures capable of treating dielectric heterogeneities. Using this method, we study oil-water mixtures containing an antagonistic salt, with hydrophilic cations and…

Soft Condensed Matter · Physics 2017-11-29 Nikos Tasios , Sela Samin , René van Roij , Marjolein Dijkstra

Membranes consist of pores and the walls of these pores are often charged. In contact with an aqueous solution, the pores fill with water and ions migrate from solution into the pores until chemical equilibrium is reached. The distribution…

Chemical Physics · Physics 2024-03-06 R. Wang , M. Elimelech , P. M. Biesheuvel

We study the effective interaction between differently charged polyelectrolyte-colloid complexes in electrolyte solutions via Monte Carlo simulations. These complexes are formed when short and flexible polyelectrolyte chains adsorb onto…

Soft Condensed Matter · Physics 2010-05-05 D. Truzzolillo , F. Bordi , F. Sciortino , S. Sennato

From cement cohesion to DNA condensation, a proper statistical physics treatment of systems with long range forces is important for a number of applications in physics, chemistry, and biology. We compute here the effective force between…

Soft Condensed Matter · Physics 2018-03-14 E. Trizac , G. Téllez

X-ray reflectivity studies demonstrate the condensation of a monovalent ion at the electrified interface between electrolyte solutions of water and 1,2-dichloroethane. Predictions of the ion distributions by standard Poisson-Boltzmann…

An effective pair potential for systems of uniformly charged lamellar colloids in the presence of an electrolytic solution of microscopic co- and counterions is derived. The charge distribution on the discs is expressed as a collection of…

Soft Condensed Matter · Physics 2009-10-31 D. G. Rowan , J. -P. Hansen , E. Trizac

We present an updated theoretical treatment of ultraperipheral collisions (UPCs) of heavy ions, within the SuperChic Monte Carlo generator. This in particular accounts for mutual ion excitation through additional photon exchanges between…

High Energy Physics - Phenomenology · Physics 2024-07-08 L. A. Harland-Lang

Properties of polyelectrolytes in tetravalent salt solutions are intensively investigated by a coarse-grained model. The concentration of salt and the size of tetravalent counterions are found playing a decisive role on chain properties. If…

Soft Condensed Matter · Physics 2009-09-29 Pai-Yi Hsiao
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