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In this paper we derive several quasi steady-state approximations (QSSAs) to the stochastic reaction network describing the Michaelis-Menten enzyme kinetics. We show how the different assumptions about chemical species abundance and…

Molecular Networks · Quantitative Biology 2017-11-09 Hye-Won Kang , Wasiur R. KhudaBukhsh , Heinz Koeppl , Grzegorz A. Rempała

We consider a stochastic model of the Michaelis-Menten (MM) enzyme kinetic reactions in terms of Stochastic Differential Equations (SDEs) driven by Poisson Random Measures (PRMs). It has been argued that among various Quasi-Steady State…

Probability · Mathematics 2025-12-04 Arnab Ganguly , Wasiur R. KhudaBukhsh

In biochemical systems the Michaelis-Menten (MM) scheme is one of the best-known models of the enzyme- catalyzed kinetics. In the academic literature the MM approximation has been thoroughly studied in the context of differential equation…

Chemical Physics · Physics 2015-01-13 Vahe Galstyan

The standard two-step model of homogeneous-catalyzed reactions had been theoretically analyzed at various levels of approximations from time to time. The primary aim was to check the validity of the quasi-steady-state approximation, and…

Chemical Physics · Physics 2019-11-14 Kamal Bhattacharyya , Sharmistha Dhatt

Stochastic models for biochemical reaction networks are widely used to explore their complex dynamics but face significant challenges, including difficulties in determining rate constants and high computational costs. To address these…

Molecular Networks · Quantitative Biology 2025-03-04 Yun Min Song , Kangmin Lee , Jae Kyoung Kim

All biological processes are controlled by complex systems of enzymatic chemical reactions. Although the majority of enzymatic networks have very elaborate structures, there are many experimental observations indicating that some turnover…

Statistical Mechanics · Physics 2015-05-27 Anatoly B. Kolomeisky

The application of the quasi-steady-state approximation to the Michaelis-Menten reaction embedded in large open chemical reaction networks is a popular model reduction technique in deterministic and stochastic simulations of biochemical…

Statistical Mechanics · Physics 2013-05-28 Philipp Thomas , Arthur V. Straube , Ramon Grima

The Michaelis-Menten mechanism is probably the best known model for an enzyme-catalyzed reaction. For spatially homogeneous concentrations, QSS reductions are well known, but this is not the case when chemical species are allowed to…

Analysis of PDEs · Mathematics 2022-09-20 Martin Frank , Christian Lax , Sebastian Walcher , Olaf Wittich

To understand the behaviour of complex systems it is often necessary to use models that describe the dynamics of subnetworks. It has previously been established using projection methods that such subnetwork dynamics generically involves…

Molecular Networks · Quantitative Biology 2016-06-08 Katy J. Rubin , Peter Sollich

There is a vast amount of literature concerning the appropriateness of various perturbation parameters for the standard quasi-steady state approximation in the Michaelis-Menten reaction mechanism, and also concerning the relevance of these…

Dynamical Systems · Mathematics 2024-02-01 Justin Eilertsen , Santiago Schnell , Sebastian Walcher

The quasi-steady state assumption (QSSA) forms the basis for rigorous mathematical justification of the Michaelis-Menten formalism commonly used in modeling a broad range of intracellular phenomena. A critical supposition of QSSA-based…

Quantitative Methods · Quantitative Biology 2011-03-08 Ed Reznik , Daniel Segre , William Erik Sherwood

Enzyme kinetics has historically been described by deterministic models, with the Michaelis-Menten (MM) equation serving as a paradigm. However, recent experimental and theoretical advances have made it clear that stochastic fluctuations,…

Molecular Networks · Quantitative Biology 2025-04-08 Jiaji Qu , Malini Rajbhandari

The Michaelis-Menten enzymatic reaction is sufficient to perceive many subtleties of network modeling, including the concentration and time scales separations, the formal equivalence between bulk phase and single-molecule approaches, or the…

Chemical Physics · Physics 2022-01-03 Denis Michel , Philippe Ruelle

Michaelis-Menten equation is a basic equation of enzyme kinetics and gives an acceptable approximation of real chemical reaction processes. Analyzing the derivation of this equation yields the fact that its good performance of approximating…

Molecular Networks · Quantitative Biology 2015-05-19 Banghe Li , Bo Li , Yuefeng Shen

The equilibration of enzyme and complex concentrations in deterministic Michaelis-Menten reaction networks underlies the hyperbolic dependence between the input (substrates) and output (products). This relationship was first obtained by…

Molecular Networks · Quantitative Biology 2024-09-30 Subham Pal , Manmath Panigrahy , R. Adhikari , Arti Dua

We study chemical reactions with complex mechanisms under two assumptions: (i) intermediates are present in small amounts (this is the quasi-steady-state hypothesis or QSS) and (ii) they are in equilibrium relations with substrates (this is…

Chemical Physics · Physics 2014-04-15 A. N. Gorban , M. Shahzad

Quasi-steady state reductions for the irreversible Michaelis--Menten reaction mechanism are of interest both from a theoretical and an experimental design perspective. A number of publications have been devoted to extending the parameter…

Chemical Physics · Physics 2023-03-21 Justin Eilertsen , Santiago Schnell , Sebastian Walcher

The classic Michaelis-Menten equation describes the catalytic activities for ensembles of enzyme molecules very well. But recent single-molecule experiment showed that the waiting time distribution and other properties of single enzyme…

Soft Condensed Matter · Physics 2009-11-11 Xiaochuan Xue , Fei Liu , Zhong-can Ou-Yang

In a conformational nonequilibrium steady state (cNESS), enzyme turnover is modulated by the underlying conformational dynamics. Based on a discrete kinetic network model, we use the integrated probability flux balance method to derive the…

Biological Physics · Physics 2017-05-17 D. Evan Piephoff , Jianlan Wu , Jianshu Cao

The quasi-steady-state approximation is widely used to develop simplified deterministic or stochastic models of enzyme catalyzed reactions. In deterministic models, the quasi-steady-state approximation can be mathematically justified from…

Dynamical Systems · Mathematics 2023-03-21 Justin Eilertsen , Santiago Schnell
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