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In this work using the density functional theory (DFT), we have studied the structural, electronic and magnetic properties of uranium dioxide with antiferromagnetic 1k-, 2k-, and 3k-order structures. Ordinary approximations in DFT, such as…

Materials Science · Physics 2020-08-25 Samira Sheykhi , Mahmoud Payami

Structural investigations by means of transmission electron microscopy (TEM) on KFexSe2 with 1.5 \leq x \leq 1.8 have revealed a rich variety of microstructure phenomena, the KFe1.5Se2 crystal often shows a superstructure modulation along…

Superconductivity · Physics 2013-05-29 Z. Wang , Y. J. Song , H. L. Shi , Z. W. Wang , Z. Chen , H. F. Tian , G. F. Chen , J. G. Guo , H. X. Yang , J. Q. Li

Iron-chalcogenide superconductors display rich phenomena caused by orbital-dependent band shifts and electronic correlations. Additionally, they are potential candidates for topological superconductivity due to the band inversion between…

We report a systematic study of the $5d$-electron-doped system Ce(Fe$_{1-x}$Ir$_x$)$_2$Al$_{10}$ ($0 \leq x \leq 0.15$). With increasing $x$, the orthorhombic $b$~axis decreases slightly while accompanying changes in $a$ and $c$ leave the…

We present here an investigation of the magnetic ordering in the Mott insulating oxyselenide materials Ln2O2Fe2OSe2 (Ln = Ce, Nd). Neutron powder diffraction data are consistent with a non-collinear multi-k ordering on the iron sublattice…

Strongly Correlated Electrons · Physics 2014-10-21 Emma E. McCabe , Andrew S. Wills , Laurent Chapon , Pascal Manuel , John S. O. Evans

The interplay between magnetism, band topology, and electronic correlation in low dimensions has been a fascinating subject of research. Here, we propose two-dimensional (2D) material systems which demonstrate such an interesting interplay.…

Materials Science · Physics 2020-12-24 Bo Tai , Weikang Wu , Xiaolong Feng , Yalong Jiao , Jianzhou Zhao , Yunhao Lu , Xian-Lei Sheng , Shengyuan A. Yang

The magnetic properties and electronic structure of (K,Tl)y Fe1.6 Se2 is studied using first-principles calculations. The ground state is checkerboard antiferromagnetically coupled blocks of the minimal Fe4 squares, with a large block spin…

Superconductivity · Physics 2015-03-18 Chao Cao , Jianhui Dai

We report density functional studies of the Fe$_{1-x}$Cu$_x$Se alloy done using supercell and coherent potential approximation methods. Magnetic behavior was investigated using the disordered local moment approach. We find that Cu occurs in…

Superconductivity · Physics 2013-08-08 S. Chadov , D. Schärf , G. H. Fecher , C. Felser , L. Zhang , D. J. Singh

The relationship between vacancy ordering and magnetism in TlFe1.6Se2 has been investigated via single crystal neutron diffraction, nuclear forward scattering, and transmission electron microscopy. The examination of chemically and…

Using the ab initio FLAPW-GGA method we examine the electronic band structure, densities of states, and the Fermi surface topology for a very recently synthesized ThCr2Si2-type potassium intercalated iron selenide superconductor KxFe2Se2.…

Superconductivity · Physics 2015-05-20 I. R. Shein , A. L. Ivanovskii

We study the magnetic, structural, and electronic properties of the recently discovered iron- based superconductor BaFe2S3 based on density functional theory with the generalized gradient approximation. The calculations show that the…

Strongly Correlated Electrons · Physics 2015-08-19 Michi-To Suzuki , Ryotaro Arita , Hiroaki Ikeda

The antiferromagnetic structure of Sr3Ir2O7, the bilayer analogue of a spin-orbital Mott insulator Sr2IrO4, was revealed by resonant magnetic x-ray diffraction. Contrasting intensities of the magnetic diffraction at the Ir LIII and LII…

Strongly Correlated Electrons · Physics 2015-06-05 Shigeki Fujiyama , K. Ohashi , H. Ohsumi , K. Sugimoto , T. Takayama , T. Komesu , M. Takata , T. Arima , H. Takagi

Magnetism in the insulating BaFe$_2$Se$_3$ was examined through susceptibility, specific heat, resistivity and neutron diffraction measurements. After formation of a short-range magnetic correlation, a long-range ordering was observed below…

We have investigated the electronic structure of ordered and disordered Sr$_2$FeMoO$_6$ using {\it ab-initio} band structure methods. The effect of disorder was simulated within super-cell calculations to realize several configurations with…

Materials Science · Physics 2009-11-07 T. Saha-Dasgupta , D. D. Sarma

The iron-based superconductors represent a promising platform for high-temperature superconductivity, but the interactions underpinning their pairing present a puzzle. The EuFe$_2$As$_2$ family is unique among these materials for having…

Using a combination of th local-density approximtion (LDA) and dynamicla mean-field theory (DMFT) calculations, we explore the correlated electronic structure of a member of the layered Iron oxychalcogenide Na_{2}Fe_{2}OSe_{2}. We find that…

Strongly Correlated Electrons · Physics 2013-07-08 Luis Craco , Mukul S. Laad , Stefano Leoni

Ge$_{1-x}$Fe$_{x}$ (Ge:Fe) shows ferromagnetic behavior up to a relatively high temperature of 210 K, and hence is a promising material for spintronic applications compatible with Si technology. We have studied its electronic structure by…

The single-crystal growth, stoichiometry, and structure of Rb1-xFe2-ySe2-zSz crystals with substitution of Se by S are reported. The variation of the magnetic and thermodynamic parameters of samples was studied by differential-scanning…

The electronic structure of FeSe, the simplest iron based superconductor (Fe-SC), conceals a potential of dramatic increase of Tc that realizes under pressure or in a single layer film. This is also the system where nematicity, the…

Superconductivity · Physics 2017-02-14 Yu. V. Pustovit , A. A. Kordyuk

The electronic structure and magnetic properties of LiFeAs and FeSe have been studied using hybrid exchange density functional theory. The total energies for a unit cell in LiFeAs and FeSe with different spin states including non-magnetic…

Superconductivity · Physics 2015-03-20 Wei Wu