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Complex crystal structures are composed of multiple local environments, and how this type of order emerges spontaneously during crystal growth has yet to be fully understood. We study crystal growth across various structures and along…

Soft Condensed Matter · Physics 2024-06-03 Maya M. Martirossyan , Matthew Spellings , Hillary Pan , Julia Dshemuchadse

In this paper, we report dynamic Monte Carlo simulation results on the crystallization of crystalline/crystalline (A/B) symmetric binary polymer blend, wherein the melting temperature of A-polymer is higher than B-polymer. Crystallization…

Soft Condensed Matter · Physics 2015-06-18 Ashok Kumar Dasmahapatra

The interplay between densification and positional ordering during the process of crystal nucleation is a greatly investigated topic. Even for the simplest colloidal model -- hard spheres -- there has been much debate regarding the…

Soft Condensed Matter · Physics 2025-02-19 Marjolein de Jager , Nena Slaats , Laura Filion

A phase field crystal model is used to investigate the mechanisms of formation and growth of early clusters in quenched/aged dilute binary alloys, a phenomenon typically outside the scope of molecular dynamics time scales. We show that…

Materials Science · Physics 2012-10-05 Vahid Fallah , Jonathan Stolle , Nana Ofori-Opoku , Shahrzad Esmaeili , Nikolas Provatas

We study a chemically active binary mixture undergoing phase separation and show that under non-equilibrium conditions, stable liquid spherical shells can form via a spinodal instability in the droplet center. A single liquid shell tends to…

Soft Condensed Matter · Physics 2023-06-21 Jonathan Bauermann , Giacomo Bartolucci , Job Boekhoven , Christoph A. Weber , Frank Jülicher

We present results from density functional theory and computer simulations that unambiguously predict the occurrence of first-order freezing transitions for a large class of ultrasoft model systems into cluster crystals. The clusters…

Soft Condensed Matter · Physics 2009-11-11 Bianca M. Mladek , Dieter Gottwald , Gerhard Kahl , Martin Neumann , Christos N. Likos

The morphology transition from the thermodynamically favorable to the unfavorable phase during growth of free-standing copper nanoclusters is studied by molecular dynamics simulations. We give a detailed description of the kinetics and…

Mesoscale and Nanoscale Physics · Physics 2015-07-15 Alexey A. Tal , E. Peter Müger , Igor A. Abrikosov

We report numerical investigations of a three-dimensional model of diffusive growth of fine particles, the internal structure of which corresponds to different crystal lattices. A growing cluster (particle) is immersed in, and exchanges…

Statistical Mechanics · Physics 2010-10-12 Vyacheslav Gorshkov , Alexandr Zavalov , Vladimir Privman

We study a quasi-two-dimensional macroscopic system of magnetic spherical particles settled on a shallow concave dish under a temporally oscillating magnetic field. The system reaches a stationary state where the energy losses from…

Soft Condensed Matter · Physics 2021-10-13 A. Escobar , F. Donado , R. E. Moctezuma , Eric R. Weeks

A model predicting the structure of repulsive, spherically symmetric, monodisperse particles confined between two walls is presented. We study the buckling transition of a single flat layer as the double layer state develops. Experimental…

Condensed Matter · Physics 2009-10-22 T Chou , David R. Nelson

Nucleation is an activated process in which the system has to overcome a free energy barrier in order for a first-order phase transition between the metastable and the stable phases to take place. In the liquid-to-solid transition the…

Soft Condensed Matter · Physics 2016-11-28 John Russo , Hajime Tanaka

We employ a molecular dynamics (MD) study to explore pattern selection in binary fluid mixtures ($AB$) undergoing surface-directed spinodal decomposition on a chemically patterned amorphous substrate. We chose a checkerboard pattern with…

Soft Condensed Matter · Physics 2025-12-12 Syed Shuja Hasan Zaidi , Hema Teherpuria , Santosh Mogurampelly , Prabhat K. Jaiswal

In this work we study morphological characteristics of the critically-sized crystalline nuclei at initial stage of the shear-induced crystallization of a model single-component amorphous (glassy) system. These characteristics are estimated…

Materials Science · Physics 2018-02-14 Bulat N. Galimzyanov , Anatolii V. Mokshin

Using Brownian dynamics computer simulations we show that a two-dimensional suspension of self-propelled ("active") colloidal particles crystallizes at sufficiently high densities. Compared to the equilibrium freezing of passive particles…

Soft Condensed Matter · Physics 2012-06-12 Julian Bialké , Thomas Speck , Hartmut Löwen

We study the appearance and properties of cluster crystals (solids in which the unit cell is occupied by a cluster of particles) in a two-dimensional system of self-propelled active Brownian particles with repulsive interactions.…

Statistical Mechanics · Physics 2017-09-06 Jean-Baptiste Delfau , Cristóbal López , Emilio Hernández-García

Spinodal decomposition process in the system of immiscible PbTe/CdTe compounds is analyzed as an example of a self-organizing structure. The immiscibility of the constituents leads to the observed morphological transformations like…

Using a generalized order parameter gradient expansion within density functional theory, we derive a phase-field-crystal model for liquid crystals composed by apolar particles in three spatial dimensions. Both the translational density and…

Soft Condensed Matter · Physics 2014-01-28 Raphael Wittkowski , Hartmut Löwen , Helmut R. Brand

We study the evolution from a liquid to a crystal phase in two-dimensional curved space. At early times, while crystal seeds grow preferentially in regions of low curvature, the lattice frustration produced in regions with high curvature is…

Soft Condensed Matter · Physics 2015-06-16 Nicolas A. Garcia , Richard A. Register , Daniel A. Vega , Leopoldo R. Gomez

Crystallization, a prototypical self-organization process during which a disordered state spontaneously transforms into a crystal characterized by a regular arrangement of its building blocks, usually proceeds by nucleation and growth. In…

Computational Physics · Physics 2017-10-06 Swetlana Jungblut , Christoph Dellago

We use molecular dynamics (MD) simulations to study surface-directed spinodal decomposition (SDSD) in unstable binary ($AB$) fluid mixtures at wetting surfaces. The thickness of the wetting layer $R_1$ grows with time $t$ as a power-law…

Soft Condensed Matter · Physics 2012-04-04 Prabhat K. Jaiswal , Sanjay Puri , Subir K. Das