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We study, by means of a Monte Carlo simulator, the hot phonon effect on the relaxation dynamics in photoexcited graphene and its quantitative impact as compared to considering an equilibrium phonon distribution. Our multi-particle approach…

Mesoscale and Nanoscale Physics · Physics 2016-02-02 José M. Iglesias , María J. Martín , Elena Pascual , Raúl Rengel

Using ultrafast optical pump-probe spectroscopy, we study the relaxation dynamics of hot optical phonons in few-layer and multi-layer graphene films grown by epitaxy on silicon carbide substrates and by chemical vapor deposition on nickel…

Many promising optoelectronic devices, such as broadband photodetectors, nonlinear frequency converters, and building blocks for data communication systems, exploit photoexcited charge carriers in graphene. For these systems, it is…

We perform a femtosecond-THz optical pump-probe spectroscopy to investigate the cooling dynamics of hot carriers in quasi-free standing bilayer epitaxial graphene. We observed longer decay time constants, in the range of 2.6 to 6.4 ps,…

Mesoscale and Nanoscale Physics · Physics 2023-02-03 Sachin Sharma , Rachael L. Myers-Ward , David Kurt Gaskill , Ioannis Chatzakis

In this work, high field carrier transport in two dimensional (2D) graphene is investigated. Analytical models are applied to estimate the saturation currents in graphene, based on the high scattering rate of optical phonon emission.…

Materials Science · Physics 2011-09-13 Tian Fang , Aniruddha Konar , Huili Xing , Debdeep Jena

The broadband and ultrafast photoresponse of graphene has been extensively studied in recent years, although the photoexcited carrier dynamics is still far from being completely understood. Different experimental approaches imply either one…

Mesoscale and Nanoscale Physics · Physics 2017-08-22 Sergey Menabde , Hyunwoo Cho , Namkyoo Park

The decay of the optical phonon into the two phonons of smaller energy is calculated for Si nanocrystals. The rate of the process is in the range of 1 to 10 ps. Such anharmonic phonon decay may control the energy relaxation rate of excited…

Materials Science · Physics 2013-04-08 A. A. Prokofiev , A. N. Poddubny , I. N. Yassievich

Hot electron effects in graphene are significant because of graphene's small electronic heat capacity and weak electron-phonon coupling, yet the dynamics and cooling mechanisms of hot electrons in graphene are not completely understood. We…

Graphene is widely recognized for its ultrafast and broadband photocurrent response, but whether the broadband ultrafast characteristics are preserved at mid-infrared wavelengths with photon energies below the optical phonon energy remains…

The properties of pristine, free-standing graphene monolayers prepared by mechanical exfoliation of graphite are investigated. The graphene monolayers, suspended over open trenches, are examined by means of spatially resolved Raman…

Materials Science · Physics 2009-01-08 Stephane Berciaud , Sunmin Ryu , Louis E. Brus , Tony F. Heinz

Using electrical transport experiments and shot noise thermometry, we investigate electron-phonon heat transfer rate in a suspended bilayer graphene. Contrary to monolayer graphene with heat flow via three-body supercollision scattering, we…

Mesoscale and Nanoscale Physics · Physics 2014-09-23 Antti Laitinen , Manohar Kumar , Mika Oksanen , Bernard Plaçais , Pauli Virtanen , Pertti Hakonen

Understanding and controlling hot-carrier relaxation in graphene is crucial for advancing ultrafast optoelectronic and terahertz technologies. Here, we investigate carrier cooling dynamics in monolayer and bilayer graphene using…

Mesoscale and Nanoscale Physics · Physics 2026-05-21 Sachin Sharm , Elliott Walker , Rachael Myers-Ward , Jenifer Hajzus , Yijing Liu , Paola Barbara , Ioannis Chatzakis

We report ultrafast response of femtosecond photoexcited carriers in single layer reduced graphene oxide flakes suspended in water as well as few layer thick film deposited on indium tin oxide coated glass plate using pump-probe…

Materials Science · Physics 2011-06-30 Sunil Kumar , N. Kamaraju , K. S. Vasu , A. K. Sood

Epitaxial growth of graphene on transition metal substrates is an important route for obtaining large scale graphene. However, the interaction between graphene and the substrate often leads to multiple orientations, distorted graphene band…

We study hot carrier transport under magnetic fields up to 15 T in suspended graphitic multilayers through differential conductance (dI/dV) spectroscopy. Distinct high-energy dI/dV anomalies have been observed and shown to be related to…

Mesoscale and Nanoscale Physics · Physics 2011-09-05 Carlos Diaz Pinto , Sungbae Lee , Viktor G. Hadjiev , Haibing Peng

We present an ab-initio study of photocarrier dynamics in graphene due to electron-phonon (EP) interactions. Using the Boltzmann relaxation-time approximation with parameters determined from density functional theory (DFT) and a…

Materials Science · Physics 2019-04-17 Dinesh Yadav , Maxim Trushin , Fabian Pauly

The temperature ($\it T$) dependence of electrical resistivity in graphene has been experimentally investigated between 10 and 400 K for samples prepared on various substrates; HfO$_2$, SiO$_2$ and h-BN. The resistivity of graphene shows a…

Mesoscale and Nanoscale Physics · Physics 2019-07-29 Y. G. You , J. H. Ahn , B. H. Park , Y. Kwon , E. E. B. Campbell , S. H. Jhang

Graphene exhibits extraordinary electronic and mechanical properties, and extremely high thermal conductivity. Being a very stable atomically thick membrane that can be suspended between two leads, graphene provides a perfect test platform…

Ultrafast optical pump-probe spectroscopy is used to track carrier dynamics in the large magnetoresistance material WTe$_{2}$. Our experiments reveal a fast relaxation process occurring on a sub-picosecond time scale that is caused by…

Ultrafast dynamics of graphite is investigated by time-resolved photoemission spectroscopy. We observe spectral features of direct photoexcitations, non-thermal electron distributions, and recovery dynamics occurring with two time scales…

Materials Science · Physics 2011-08-24 Y. Ishida , T. Togashi , K. Yamamoto , M. Tanaka , T. Taniuchi , T. Kiss , M. Nakajima , T. Suemoto , S. Shin
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