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Related papers: Probing single-photon ionization on the attosecond…

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Autocorrelation measurement is theoretically demonstrated to characterize attosecond pulses by studying the two-photon double ionization (TPDI) process. An interferometric autocorrelation curve is presented in the change of TPDI probability…

Atomic Physics · Physics 2024-09-25 Fei Li , Kun Zhao , Bing-Bing Wang , Xin-Kui He , Zhi-Yi Wei

We investigate ionization of neon atoms by an isolated attosecond pump pulse in the presence of two coherent extreme ultraviolet or x-ray probe fields. The probe fields are tuned to a core-valence transition in the residual ion and induce…

Atomic Physics · Physics 2016-03-30 Jhih-An You , Nina Rohringer , Jan Marcus Dahlström

We develop a first-principles simulation method for attosecond time-resolved photoelectron spectroscopy. This method enables us to directly simulate the whole experimental processes, including excitation, emission and detection on equal…

Atomic Physics · Physics 2018-08-01 Shunsuke A. Sato , Hannes Hübener , Angel Rubio , Umberto De Giovannini

We calculate the transient absorption of an isolated attosecond pulse by helium atoms subject to a delayed infrared (\ir) laser pulse. With the central frequency of the broad attosecond spectrum near the ionization threshold, the absorption…

Atomic Physics · Physics 2015-06-12 Shaohao Chen , Mengxi Wu , Mette B. Gaarde , Kenneth J. Schafer

Photoionisation is a process where absorption of one or several photons liberates an electron and creates a hole in a quantum system, such as an atom or a molecule. Is it faster to remove an electron using one or many photons, and how to…

Quantum Physics · Physics 2015-09-25 Jivesh Kaushal , Felipe Morales , Lisa Torlina , Misha Ivanov , Olga Smirnova

We propose a general technique to retrieve the information of dipole-forbidden resonances in the autoionizing region. In the simulation, a helium atom is pumped by an isolated attosecond pulse in the extreme ultraviolet (EUV) combined with…

Atomic Physics · Physics 2014-03-28 Wei-Chun Chu , Toru Morishita , C. D. Lin

Electronic processes within atoms and molecules reside on the timescale of attoseconds. Recent advances in the laser-based pump-probe interrogation techniques have made possible the temporal resolution of ultrafast electronic processes on…

Atomic Physics · Physics 2024-02-16 Yongzhe Ma , Hongcheng Ni , Jian Wu

The photoionization of the CO molecule from the C$-1s$ orbital does not obey the Franck-Condon approximation, as a consequence of the nuclear recoil that accompanies the direct emission and intra-molecular scattering of the photoelectron.…

Atomic Physics · Physics 2021-11-24 Bejan Ghomashi , Nicolas Douguet , Luca Argenti

Time-resolved photoelectron spectroscopy provides access to the electronic structure and non-equilibrium electron dynamics in matter. At solid surfaces photoemission dynamics can be investigated on its natural time scale by measuring…

The Wigner delay is defined as the energy derivative of the scattering phase of a particle in a given potential, unveiling the time taken (or gained) due to the interaction. The characterisation of this delay plays a central role in…

We explore the interactions between Argon and extreme ultraviolet (XUV) laser pulses across photon energies of 200 eV, 260 eV, and 315 eV, scrutinizing the influence of photon energy on Argon ion yields and unraveling the associated…

Atomic Physics · Physics 2024-04-15 Linhao Xiong

We examine the archetype of an interference experiment for Auger electrons: two electron wave packets are launched by inner-shell ionizing a krypton atom using two attosecond light pulses with a variable time delay. This setting is an…

Atomic Physics · Physics 2015-03-13 Christian Buth , Kenneth J. Schafer

We study the ionization of atomic hydrogen in the direction of polarization due to a linearly polarized XUV pulse in the presence a strong field IR. We describe the photoelectron spectra as an interference problem in the time domain.…

Atomic Physics · Physics 2016-11-15 Ana Alicia Gramajo , Renata Della Picca , Carlos Roberto Garibotti , Diego Arbó

In this work, we present temporally resolved measurements of electron numbers created at photoionization of various gases by femtosecond laser pulse at 800 nm wavelength. The experiments were conducted in $O_2$, $Xe$, $Ar$, $N_2$, $Kr$ and…

Plasma Physics · Physics 2019-06-05 A. Sharma , M. Slipchenko , K. A. Rahman , M. N. Shneider , A. Shashurin

We apply time-dependent R-matrix theory to study inner-shell ionization of C atoms in ultra-short high-frequency light fields with a photon energy between 170 and 245 eV. At an intensity of 10$^{17}$ W/cm$^2$, ionization is dominated by…

Atomic Physics · Physics 2015-08-12 H. F. Rey , H. W. van der Hart

We consider the time delay of electron detachment from a Coulomb center and two-center systems in the process of ionization. It is shown that the attosecond streaking, most usual method of time delay measure, can be formally described by…

Atomic Physics · Physics 2015-06-15 Vladislav V. Serov , Vladimir L. Derbov , Tatyana A. Sergeeva

We present the first numerical simulation of the time delay in the photoionization of the simplest diatomic molecule H$_2^+$ as observed by attosecond streaking. We show that the strong variation of the Eisenbud-Wigner-Smith time delay as a…

Understanding initial electron thermalization has relevance to both fundamental scientific knowledge and application to the construction of novel devices. In this study, attosecond transient absorption is used to directly measure initial…

Materials Science · Physics 2024-06-07 Bethany R. de Roulet , Lorenz Drescher , Shunsuke A. Sato , Stephen R. Leone

Attosecond interferometry in a two-color field is central to attosecond metrology and spectroscopy. In this technique, a photoelectron wave packet is released when a single photon from an extreme ultraviolet comb is absorbed. The wave…

Relative phases of atomic above-threshold ionization wavepackets have been investigated in a recent experiment [L. J. Zipp, A. Natan, and P. H. Bucksbaum, Optica \textbf{1}, 361-364 (2014)] exploiting interferences between different…

Atomic Physics · Physics 2021-11-10 S. D. López , S. Donsa , S. Nagele , D. G. Arbó , J. Burgdörfer