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Collisions between cold polar molecules represent a fascinating research frontier, but have proven hard to probe experimentally. We report measurements of inelastic cross sections for collisions between NO and ND 3 molecules at energies…

The electrostatic interactions of phosphate groups and counter ions critically affect the structure, function and reactivity of DNA or RNA. We present a joint experimental-theoretical investigation of dimethyl phosphate (DMP-) in aqueous…

We experimentally demonstrate the occurrence of negative absolute resistance (NAR) up to about $-1\Omega$ in response to an externally applied dc current for a shunted Nb-Al/AlO$_x$-Nb Josephson junction, exposed to a microwave current at…

Chaotic Dynamics · Physics 2009-11-13 J. Nagel , D. Speer , T. Gaber , A. Sterck , R. Eichhorn , P. Reimann , K. Ilin , M. Siegel , D. Koelle , R. Kleiner

Coherent electronic transport through individual molecules is crucially sensitive to quantum interference. Using exact diagonalization techniques, we investigate the zero-bias and zero-temperature conductance through $\pi$-conjugated…

Strongly Correlated Electrons · Physics 2015-05-14 Julian Rincon , K. Hallberg , S. Ramasesha

Many nanoelectronic devices rely on thin dielectric barriers through which electrons tunnel. For instance, aluminium oxide barriers are used as Josephson junctions in superconducting electronics. The reproducibility and drift of circuit…

Mesoscale and Nanoscale Physics · Physics 2020-02-05 M. J. Cyster , J. S. Smith , J. A. Vaitkus , N. Vogt , S. P. Russo , J. H. Cole

A system of an array of side-coupled quantum-dots attached to a quantum wire is studied theoretically. Transport through the quantum wire is investigated by means of a noninteracting Anderson tunneling Hamiltonian. Analytical expressions of…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 P. A. Orellana , F. Dominguez-Adame , E. Diez

In this work we theoretically consider the OPE-3 molecule bridging two metallic leads and show that because of the electron-phonon interaction and the transition of cation to triplet states, we can have a light induced negative differential…

Mesoscale and Nanoscale Physics · Physics 2021-04-29 Amir Eskandari-asl

Nanoscale molecular-electronic devices and machines are emerging as promising functional elements, naturally flexible and efficient, for next generation technologies. A deeper understanding of carrier dynamics in molecular junctions is…

Mesoscale and Nanoscale Physics · Physics 2018-04-04 K. Beltako , F. Michelini , N. Cavassilas , L. Raymond

We propose a model to describe a gas of pyramidal molecules interacting via dipole-dipole interactions. The interaction modifies the tunneling properties between the classical equilibrium configurations of the single molecule and, for…

Condensed Matter · Physics 2009-11-07 Giovanni Jona-Lasinio , Carlo Presilla , Cristina Toninelli

We study entanglement of charge qubits in a vertical tunnel-coupled double quantum dot containing two interacting electrons. Exact diagonalization is used to compute the negativity characterizing entanglement. We find that entanglement can…

Other Condensed Matter · Physics 2007-05-23 S. Weiss , M. Thorwart , R. Egger

Stable organic radicals integrated into molecular junctions represent a practical realization of the single-orbital Anderson impurity model. Motivated by recent experiments for perchlorotriphenylmethyl (PTM) molecules contacted to gold…

Strongly Correlated Electrons · Physics 2018-10-02 W. H. Appelt , A. Droghetti , L. Chioncel , M. M. Radonjic , E. Munoz , S. Kirchner , D. Vollhardt , I. Rungger

We consider a single molecule circuit embedded into solvent. The Born dielectric solvation model is combined with Keldysh nonequilibrium Green's functions to describe the electron transport properties of the system. Depending on the…

Mesoscale and Nanoscale Physics · Physics 2012-01-26 Alan A. Dzhioev , D. S. Kosov

We derive the nonequilibrium conductance matrix for open stationary Chemical Reaction Networks (CRNs) described by a deterministic mass action kinetic equation. As an illustration, we determine the nonequilibrium conductance matrix of a CRN…

Statistical Mechanics · Physics 2025-06-27 Paul Raux , Christophe Goupil , Gatien Verley

In molecular dynamics (MD), neural network (NN) potentials trained bottom-up on quantum mechanical data have seen tremendous success recently. Top-down approaches that learn NN potentials directly from experimental data have received less…

Chemical Physics · Physics 2021-11-29 Stephan Thaler , Julija Zavadlav

We investigate the non-equilibrium transport properties of a disordered molecular nanowire. The nanowire is regarded as a quasi-one-dimensional organic crystal composed of self-assembled molecules. One orbital and a single random energy are…

Mesoscale and Nanoscale Physics · Physics 2017-06-07 P. Thiessen , E. Diaz , R. A. Roemer , F. Dominguez-Adame

The interplay between interference effects and electron-electron interactions in electron transport through an interacting double quantum dot system is investigated using a hierarchical quantum master equation approach which becomes exact…

Mesoscale and Nanoscale Physics · Physics 2013-12-24 R. Härtle , G. Cohen , D. R. Reichman , A. J. Millis

We theoretically investigate electronic transport through a junction where a quantum dot (QD) is tunnel coupled on both sides to semiconductor nanowires with strong spin-orbit interaction and proximity-induced superconductivity. The results…

Superconductivity · Physics 2014-12-09 Guang-Yao Huang , Martin Leijnse , Karsten Flensberg , Hongqi Xu

We investigate sequential tunneling through a multilevel quantum dot confining multiple electrons, in the regime where several channels are available for transport within the bias window. By analyzing solutions to the master equations of…

Mesoscale and Nanoscale Physics · Physics 2009-02-23 Eduardo Vaz , Jordan Kyriakidis

Transport through molecular magnets is studied in the regime of strong coupling to the leads. We consider a resonant-tunneling model where the electron spin in a quantum dot or molecule is coupled to an additional local, anisotropic spin…

Mesoscale and Nanoscale Physics · Physics 2013-05-29 Florian Elste , Carsten Timm

A four-terminal donor quantum dot (QD) is used to characterize potential barriers between degenerately doped nanoscale contacts. The QD is fabricated by hydrogen-resist lithography on Si(001) in combination with $n$-type doping by…

Mesoscale and Nanoscale Physics · Physics 2016-08-24 Nikola Pascher , Szymon Hennel , Susanne Mueller , Andreas Fuhrer