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The dynamics of the resonant Auger (RA) process of the core-excited C$^\ast$O(1s$^{-1}\pi^\ast,v_r=0$) molecule in an intense X-ray laser field is studied theoretically. The theoretical approach includes the analogue of the conical…

Atomic and Molecular Clusters · Physics 2011-09-27 Philipp V. Demekhin , Ying-Chih Chiang , Lorenz S. Cederbaum

We have unveiled coherent multiphoton interferences originating from different quantum paths taken by the Auger electron induced by a high-intensity x-ray/XUV pulse under the presence of a strong optical field. These interferences give rise…

Quantum Physics · Physics 2015-07-03 Antonio Picón , Phay J. Ho , Gilles Doumy , Stephen H. Southworth

We devise an ab initio formalism for the quantum dynamics of Auger decay by laser-dressed atoms which are inner-shell ionized by extreme ultraviolet (XUV) light. The optical dressing laser is assumed to be sufficiently weak such that…

Atomic Physics · Physics 2009-11-06 Christian Buth , Kenneth J. Schafer

The dynamics of atomic levels resonantly coupled by a coherent and intense short high-frequency laser pulse is discussed and it is advocated that this dynamics is sensitively probed by measuring the spectra of the particles emitted. It is…

Atomic and Molecular Clusters · Physics 2013-01-11 Philipp V. Demekhin , Lorenz S. Cederbaum

Several correlation and interference effects in strong-field physics are investigated. We show that the interference of continuum wave packets can be the dominant mechanism of high-harmonic generation (HHG) in the over-the-barrier regime.…

We discuss the possibility of non-exponential Auger decay of atoms irradiated by X-ray photons. This effect can occur at times, which are greater than the lifetime of a system under consideration. The mechanism for non-exponential depletion…

Atomic Physics · Physics 2015-07-14 A. M. Ishkhanyan , V. P. Krainov

We theoretically investigate resonant x-ray scattering from two non-interacting Ne+ ions driven by an intense attosecond pulse using a non-relativistic, QED-based time-dependent framework. Our model includes Rabi oscillations,…

Atomic Physics · Physics 2026-05-13 Akilesh Venkatesh , Phay J. Ho

Multiple electron processes occur widely in atoms, molecules, clusters, and condensed matters when they are interacting with energetic particles or intense laser fields. In this work, a unified and accurate theoretical formalism is proposed…

Atomic Physics · Physics 2018-04-18 Pengfei Liu , Jiaolong Zeng , Jianmin Yuan

Photoionization of an atom in the presence of a neighboring atom of different species is studied. The latter first undergoes resonant photoexcitation, leading to an autoionizing state of the diatomic system. Afterwards, the excitation…

Atomic Physics · Physics 2020-08-11 F. Grüll , A. B. Voitkiv , C. Müller

The ionization of an atom by a high-frequency intense laser pulse, where the energy of a single-photon is sufficient to ionize the system, is investigated from first principles. It is shown that as a consequence of an AC Stark effect in the…

Atomic Physics · Physics 2012-06-26 Philipp V Demekhin , Lorenz S Cederbaum

The resonance strength of the two-step process of nuclear excitation by electron capture followed by $\gamma$ decay of the nucleus can be significantly increased in highly charged ions if the resonant capture proceeds via an excited…

Characterization of the inner-shell decay processes in molecules containing heavy elements is key to understanding x-ray damage of molecules and materials and for medical applications with Auger-electron-emitting radionuclides. The 1s hole…

We theoretically show that core-excited state populations can be efficiently manipulated with strong optical fields during their decay, which takes place in a few femtoseconds. We focus on the $1s^{-1}3p$ resonant excitation in neon, where…

Modern x-ray sources enable the production of coherent x-ray pulses with a pulse duration in the same order as the characteristic lifetimes of core-hole states of atoms and molecules. These pulses enable the manipulation of the core-hole…

Atomic Physics · Physics 2018-01-11 Raymond Sullivan , Junteng Jia , Alvaro Vazquez-Mayagoitia , Antonio Picón

In the ultra-strong coupling regime of a light-matter system, the ground state exhibits non-trivial entanglement between the atom and photons. For the purposes of exploring the measurement and control of this ground state, here we analyze…

Quantum Physics · Physics 2020-08-25 Suguru Endo , Yuichiro Matsuzaki , Kosuke Kakuyanagi , Shiro Saito , Neill Lambert , Franco Nori

The consequences of the Auger effect on the population of heavy element ions are analyzed for the case of relatively cool gas irradiated by keV X-rays, with intended applications to the accretion disks of young stellar ob jects. Highly…

Astrophysics of Galaxies · Physics 2015-05-28 Máté Ádámkovics , Alfred E. Glassgold , Rowin Meijerink

We present the first investigation of excited state dynamics by resonant Auger-Meitner spectroscopy (also known as resonant Auger spectroscopy) using the nucleobase thymine as an example. Thymine is photoexcited in the UV and probed with…

The capability of generating two intense, femtosecond x-ray pulses with controlled time delay opens the possibility of performing time-resolved experiments for x-ray induced phenomena. We have applied this capability to study the…

This paper presents a nonperturbative treatment of strong-coupling induced effects in atom-field systems which cannot be seen in traditional perturbative treatments invoking compromising assumptions such as the Born-Markov, rotating wave or…

Quantum Physics · Physics 2020-02-25 Jen-Tsung Hsiang , Bei-Lok Hu

The Auger effect from inner shells, which arises from resonance excitation of the valence electron of an atom by a weak electromagnetic wave, is discussed.

Atomic Physics · Physics 2017-06-27 M. A. Kutlan
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