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Using Brownian dynamics computer simulations we show that a two-dimensional suspension of self-propelled ("active") colloidal particles crystallizes at sufficiently high densities. Compared to the equilibrium freezing of passive particles…

Soft Condensed Matter · Physics 2012-06-12 Julian Bialké , Thomas Speck , Hartmut Löwen

We extend the conventional mode-coupling theory of supercooled liquids to systems under stationary shear flow. Starting from generalized fluctuating hydrodynamics, a nonlinear equation for the intermediate scattering function is…

Statistical Mechanics · Physics 2009-11-10 Kunimasa Miyazaki , David R. Reichman

We perform Dynamic Monte Carlo simulations to investigate the equilibrium dynamics of hard colloidal cuboids in oblate and prolate nematic liquid crystals. In particular, we characterise the particles' diffusion along the nematic director…

Soft Condensed Matter · Physics 2020-05-27 Alejandro Cuetos , Alessandro Patti

Modeling the couplings between active particles often neglects the possible many-body effects that control the propulsion mechanism. Accounting for such effects requires the explicit modeling of the molecular details at the origin of…

Soft Condensed Matter · Physics 2023-09-18 Jeanne Decayeux , Jacques Fries , Vincent Dahirel , Marie Jardat , Pierre Illien

We use the dynamic length and time scale separation in suspensions to formulate a general description of colloidal thermophoresis. Our approach allows an unambiguous definition of separate contributions to the colloidal flux and clarifies…

Soft Condensed Matter · Physics 2017-12-19 Jerome Burelbach , Daan Frenkel , Ignacio Pagonabarraga , Erika Eiser

We present a plane-wave basis set implementation of charge constrained density functional molecular dynamics (CDFT-MD) for simulation of electron transfer reactions in condensed phase systems. Following earlier work of Wu et al. Phys. Rev.…

Chemical Physics · Physics 2015-05-13 H. Oberhofer , J. Blumberger

Proton transport property is studied by modelling the intermolecular pair correlation functions of the proton ion with the electrode and the electrolyte of a polymer electrolyte fuel cell (PEMFC) by using Materials-Studio and then applying…

Materials Science · Physics 2023-05-05 S. S. Awulachew , K. N. Nigussa

Extreme deformation of soft matter is central to our understanding of the effects of shock, fracture, and phase change in a variety of systems. Yet, despite, the increasing interest in this area, far-from-equilibrium behaviours of soft…

Soft Condensed Matter · Physics 2020-07-07 Axel Huerre , Marco De Corato , Valeria Garbin

We study compressible fluid flow in narrow two-dimensional channels using a novel molecular dynamics simulation method. In the simulation area, an upstream source is maintained at constant density and temperature while a downstream…

Condensed Matter · Physics 2009-10-22 M. Sun , C. Ebner

We study the role of active coupling on the transport properties of homogeneously charged macromolecules in an infinitely dilute solution. An enzyme becomes actively bound to a segment of the macromolecule, exerting an electrostatic force…

Soft Condensed Matter · Physics 2024-05-24 Tapas Singha , Siao-Fong Li , Murugappan Muthukumar

Sedimentation-diffusion equilibrium density profiles of suspensions of charge-stabilized colloids are calculated theoretically and by Monte Carlo simulation, both for a one-component model of colloidal particles interacting through pairwise…

Soft Condensed Matter · Physics 2013-05-29 Aldemar Torres , Alejandro Cuetos , Marjolein Dijkstra , Rene van Roij

The effects of the finite size of the simulation box in equilibrium molecular dynamics simulations are investigated for prototypical superionic conductors of different types, namely the fluorite-structure materials PbF2, CaF2, and UO2…

Materials Science · Physics 2022-04-20 Federico Grasselli

Biomolecular motors use free energy to drive a variety of cellular tasks, including the transport of cargo, such as vesicles and organelles. We find that the widely-used `constant-force' approximation for the effect of cargo on motor…

Statistical Mechanics · Physics 2023-04-11 Aidan I Brown , David A Sivak

The organization of water molecules and ions between charged mineral surfaces determines the stability of colloidal suspensions and the strength of phase-separated particulate gels. In this article we assemble a density functional that…

Soft Condensed Matter · Physics 2024-05-15 Thomas Petersen

Solid-state electrolytes with argyrodite structures, such as $\mathrm{Li_6PS_5Cl}$, have attracted considerable attention due to their superior safety compared to liquid electrolytes and higher ionic conductivity than other solid…

Materials Science · Physics 2023-10-31 Jiho Lee , Suyeon Ju , Seungwoo Hwang , Jinmu You , Jisu Jung , Youngho Kang , Seungwu Han

Molecular dynamics simulations are used to study the local dynamics of counterion-charged polymer association at charge densities above and below the counterion condensation threshold. Surprisingly, the counterions form weakly-interacting…

Soft Condensed Matter · Physics 2009-11-13 Tak Shing Lo , Boris Khusid , Joel Koplik

Using simulation and theory we study the dynamics of a colloidal suspension in two dimensions subject to a time-delayed repulsive feedback that depends on the positions of the colloidal particles. The colloidal particles experience an…

Soft Condensed Matter · Physics 2019-09-06 Sonja Tarama , Stefan U. Egelhaaf , Hartmut Löwen

We investigate stresses and particle motion during the start up of flow in a colloidal dispersion close to arrest into a glassy state. A combination of molecular dynamics simulation, mode coupling theory and confocal microscopy experiment…

Soft Condensed Matter · Physics 2009-11-13 J. Zausch , J. Horbach , M Laurati , S. U. Egelhaaf , J. M. Brader , Th. Voigtmann , M. Fuchs

We study the dynamics of colloidal suspensions of hard spheres that are subject to Brownian motion in the overdamped limit. We obtain the time evolution of the self and distinct parts of the van Hove function by means of dynamical density…

Soft Condensed Matter · Physics 2018-01-16 Daniel Stopper , Kevin Marolt , Hendrik Hansen-Goos , Roland Roth

Molecular dynamics (MD) is a widely-used tool for simulating the molecular and materials properties. It is a common wisdom that molecular dynamics simulations should obey physical laws and, hence, lots of effort is put into ensuring that…

Chemical Physics · Physics 2023-08-23 Lina Zhang , Yi-Fan Hou , Fuchun Ge , Pavlo O. Dral
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