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The formation of donor-acceptor complexes (DACs) between the electron donor Dibenzotetrathiafulvalene (DBTTF) and the acceptor Hexaaza\-triphenylene\-hexacarbo\-nitrile (HATCN) results in a new phase with a distinctly different crystal…

The design of low-dimensional organic-inorganic interfaces for the next generation of opto-electronic applications requires an in-depth understanding of the microscopic mechanisms ruling electronic interactions in these systems. In this…

We present a study for a sample of galaxies with active nuclei to characterize the main type of PAH molecules present in these objects and the local physical conditions of their irradiating sources, as well as the characteristics of the…

While powerful techniques exist to accurately account for anharmonicity in vibrational molecular spectroscopy, they are computationally very expensive and cannot be routinely employed for large species and/or at non- zero vibrational…

Chemical Physics · Physics 2018-10-17 Giacomo Mulas , Cyril Falvo , Patrick Cassam-Chenaï , Christine Joblin

Polycyclic Aromatic Hydrocarbons (PAHs) are carbon-based molecules resulting from the union of aromatic rings and related species, which are likely responsible for strong infrared emission features (3.3, 6.2, 7.7, 8.6, 11.3 and 12.7…

Astrophysics of Galaxies · Physics 2021-11-05 I. García-Bernete , D. Rigopoulou , A. Alonso-Herrero , M. Pereira-Santaella , P. F. Roche , B. Kerkeni

Several examples of metallic electron doped polycyclic aromatic hydrocarbons (PAHs) molecular crystals have recently been experimentally proposed. Some of them have superconducting components, but most other details are still unknown…

Superconductivity · Physics 2013-09-06 S. Shahab Naghavi , Michele Fabrizio , Tao Qin , Erio Tosatti

We present an on-line database of computed molecular properties for a large sample of polycyclic aromatic hydrocarbons (PAHs) in four charge states: -1, 0, +1, and +2. At present our database includes 40 molecules ranging in size from…

Astrophysics · Physics 2009-11-13 G. Malloci , C. Joblin , G. Mulas

We extend the prediction of vibrational spectra to large sized polycyclic aromatic hydrocarbon (PAH) molecules comprising up to \sim 1500 carbon atoms by evaluating the efficiency of several computational chemistry methodologies. We employ…

Aims. We aim to elucidate the spectral changes in the 3 micron region that result from chemical changes in the molecular periphery of polycyclic aromatic hydrocarbons (PAHs) with extra hydrogens (H-PAHs) and methyl groups (Me-PAHs).…

Astrophysics of Galaxies · Physics 2018-04-04 E. Maltseva , C. J. Mackie , A. Candian , A. Petrignani , X. Huang , T. J. Lee , A. G. G. M. Tielens , J. Oomens , WJ Buma

In this paper we present a detailed computational study of the electronic structure and optical properties of triply-bonded hydrocarbons with linear, and graphyne substructures, with the aim of identifying their potential in opto-electronic…

Materials Science · Physics 2018-01-23 Deepak Kumar Rai , Himanshu Chakraborty , Alok Shukla

Polycyclic Aromatic Hydrocarbons (PAHs) are ubiquitous complex molecules in the interstellar medium and are used as an indirect indicator of star-formation. On the other hand the ultraviolet (UV) emission from the young massive stars…

Astrophysics of Galaxies · Physics 2024-01-09 K. Ujjwal , Sreeja S Kartha , Akhil Krishna R , Blesson Mathew , Smitha Subramanian , Sudheesh T P , Robin Thomas

Amino acids are essential to all life. However, our understanding of some aspects of their intrinsic structure, molecular chemistry, and electronic structure is still limited. In particular the nature of amino acids in their crystalline…

Materials Science · Physics 2020-11-02 Anna Regoutz , Marta S. Wolinska , Nathalie K. Fernando , Laura E. Ratcliff

A systemically theoretical study has been presented to explored the crystal structures and electronic characteristics of polycyclic aromatic hydrocarbons (PAHs), such as solid phenanthrene, picene, 1,2;8,9-dibenzopentacene, and…

Materials Science · Physics 2015-12-10 Guohua Zhong , Zhongbing Huang , Chao Zhang , Xunwang Yan , Xiaojia Chen , Haiqing Lin

We present a new method to decompose the emission features of polycyclic aromatic hydrocarbons (PAHs) from mid-infrared spectra using theoretical PAH templates in conjunction with modified blackbody components for the dust continuum and an…

Astrophysics of Galaxies · Physics 2018-06-26 Yanxia Xie , Luis C. Ho , Aigen Li , Jinyi Shangguan

The electronic spectra of gas-phase cationic polycyclic aromatic hydrocarbons (PAHs), trapped in the Fourier Transform Ion Cyclotron Resonance cell of the PIRENEA experiment, have been measured by multiphoton dissociation spectroscopy in…

Chemical Physics · Physics 2015-03-13 F. Useli-Bacchitta , A. Bonnamy , G. Mulas , G. Malloci , D. Toublanc , C. Joblin

We reanalyze the mid-infrared (5-40 $\mu$m) Spitzer spectra of 86 low-redshift ($z < 0.5$) Palomar-Green quasars to investigate the nature of polycyclic aromatic hydrocarbon (PAH) emission and its utility as a star formation rate (SFR)…

Astrophysics of Galaxies · Physics 2022-02-16 Yanxia Xie , Luis C. Ho

In this paper, we perform large-scale electron-correlated calculations of optoelectronic properties of rectangular graphene-like polycyclic aromatic hydrocarbon molecules. Theoretical methodology employed in this work is based upon…

Materials Science · Physics 2019-05-29 Deepak Kumar Rai , Alok Shukla

The PAH family of organic compounds (polycyclic aromatic hydrocarbons), involved in several fields of chemistry, has received particular attention in astrochemistry, where their vibrational spectroscopy, thermodynamic, dynamic, and…

Chemical Physics · Physics 2017-06-13 Georges Trinquier , Aude Simon , Mathias Rapacioli , Florent Xavier Gadéa

We present a charge distribution based model that computes the infrared spectrum of polycyclic aromatic hydrocarbon (PAH) molecules using recent measurements or quantum chemical calculations of specific PAHs. The model is applied to a…

Astrophysics of Galaxies · Physics 2022-06-15 Ameek Sidhu , A. G. G. M. Tielens , Els Peeters , Jan Cami

Fragmentation is an important decay mechanism for polycyclic aromatic hydrocarbons (PAHs) under harsh interstellar conditions and represents a possible formation pathway for small molecules such as H2, C2H2, C2H4. Our aim is to investigate…