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Using a combination of ultraviolet-vacuum ultraviolet reflectivity and spectroscopic ellipsometry, we observe a resonant exciton at an unusually high energy of 6.3eV in epitaxial graphene. Surprisingly, the resonant exciton occurs at room…

We present ab initio many-body calculations of the optical absorption in bulk graphite, graphene and bilayer of graphene. Electron-hole interaction is included solving the Bethe-Salpeter equation on top of a GW quasiparticle electronic…

Materials Science · Physics 2015-05-14 Paolo E. Trevisanutto , Markus Holzmann , Michel Cote , Valerio Olevano

We study the effect of electron-electron interactions in the optical conductivity of graphene under applied bias and derive a generalization of Elliot's formula, commonly used for semiconductors, for the optical intensity. We show that {\it…

Mesoscale and Nanoscale Physics · Physics 2010-07-29 N. M. R. Peres , R. M. Ribeiro , A. H. Castro Neto

We develop an ab initio framework that captures the impact of electron-electron and electron-hole interactions on phonon properties. This enables the inclusion of excitonic effects in the optical phonon dispersions and lifetimes of…

Materials Science · Physics 2025-06-17 Alberto Guandalini , Francesco Macheda , Giovanni Caldarelli , Francesco Mauri

Using first principles many-body theory methods (GW+BSE) we demonstrate that optical properties of graphane are dominated by localized charge-transfer excitations governed by enhanced electron correlations in a two-dimensional dielectric…

Materials Science · Physics 2015-05-18 Pierluigi Cudazzo , Claudio Attacalite , Ilya V. Tokatly , Angel Rubio

The optical properties of graphene are strongly affected by electron-electron (e-e) and electron-hole (e-h) interactions. Here we tune these many-body interactions through varying the density of free charge carriers. Measurements from the…

We investigate the role of electron-hole correlations in the absorption of freestanding monolayer and bilayer graphene using optical transmission spectroscopy from 1.5 to 5.5 eV. Line shape analysis demonstrates that the ultraviolet region…

Mesoscale and Nanoscale Physics · Physics 2015-05-20 Dong-Hun Chae , Tobias Utikal , Siegfried Weisenburger , Harald Giessen , Klaus. v. Klitzing , Markus Lippitz , Jurgen H. Smet

The role of electron-phonon interactions is experimentally and theoretically investigated near the saddle point absorption peak of graphene. The differential optical transmission spectra of multiple, non-interacting layers of graphene…

We present a first-principles calculation of the optical properties of armchair-edged graphene nanoribbons (AGNRs) with many-electron effects included. The reduced dimensionality of the AGNRs gives rise to an enhanced electron-hole binding…

Mesoscale and Nanoscale Physics · Physics 2007-10-10 Li Yang , Marvin L. Cohen , Steven G. Louie

We present first-principles calculations of many-electron effects on the optical response of graphene, bilayer graphene, and graphite employing the GW-Bethe Salpeter equation approach. We find that resonant excitons are formed in these…

Materials Science · Physics 2009-10-31 Li Yang , Jack Deslippe , Cheol-Hwan Park , Marvin L. Cohen , Steven G. Louie

The disclosure of basic nonlinear optical properties of graphene-like nanostructures with correlated electron-hole nonlinear dynamics over a wide range of frequencies and pump field intensities is of great importance for both graphene…

Mesoscale and Nanoscale Physics · Physics 2022-06-15 H. K. Avetissian , S. S. Israelyan , H. H. Matevosyan , G. F. Mkrtchian

We have performed first-principles calculations to study optical absorption spectra of doped graphene with many-electron effects included. Both self-energy corrections and electron-hole interactions are reduced due to the enhanced screening…

Mesoscale and Nanoscale Physics · Physics 2011-09-09 Li Yang

In this work we perform electron energy-loss spectroscopy (EELS) of freestanding graphene with high energy and momentum resolution to disentangle the quasielastic scattering from the excitation gap of Dirac electrons close to the optical…

Magneto Raman scattering study of the E$_{2g}$ optical phonons in multi-layer epitaxial graphene grown on a carbon face of SiC are presented. At 4.2K in magnetic field up to 33 T, we observe a series of well pronounced avoided crossings…

Materials Science · Physics 2015-05-13 C. Faugeras , M. Amado , P. Kossacki , M. Orlita , M. Sprinkle , C. Berger , W. A. de Heer , M. Potemski

Linear and nonlinear optical properties of low dimensional nanostructures have attracted a large interest in the scientific community as tools to probe the strong confinement of the electrons and for possible applications in optoelectronic…

Materials Science · Physics 2017-03-08 C. Attaccalite , E. Cannuccia , M. Grüning

We report on resonance Raman spectroscopy measurements with excitation photon energy down to 1.16 eV on graphene, to study how low-energy carriers interact with lattice vibrations. Thanks to the excitation energy close to the Dirac point at…

Many-electron effects often dramatically modify the properties of reduced dimensional systems. We report calculations, based on an many-electron Green's function approach, of electron-hole interaction effects on the optical spectra of…

Materials Science · Physics 2009-11-10 Catalin D. Spataru , Sohrab Ismail-Beigi , Lorin X. Benedict , Steven G. Louie

The energy spectra and wavefunctions of bound excitons in important two-dimensional (2D) graphene derivatives, i.e., graphyne and graphane, are found to be strongly modified by quantum confinement, making them qualitatively different from…

Mesoscale and Nanoscale Physics · Physics 2015-06-16 Shouting Huang , Yufeng Liang , Li Yang

We report a theoretical study of the many-body effects of electron-electron interaction on the ground-state and spectral properties of double-layer graphene. Using a projector-based renormalization method we show that if a finite voltage…

Strongly Correlated Electrons · Physics 2015-06-04 Van-Nham Phan , Holger Fehske

We review the basic aspects of electrons in graphene (two-dimensional graphite) exposed to a strong perpendicular magnetic field. One of its most salient features is the relativistic quantum Hall effect the observation of which has been the…

Mesoscale and Nanoscale Physics · Physics 2011-11-24 M. O. Goerbig
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