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We show that the antiferromagnetic state commonly observed in the phase diagrams of the iron-based superconductors necessarily triggers loop currents characterized by charge transfer between different Fe $ 3d $ orbitals. This effect is…

Strongly Correlated Electrons · Physics 2018-04-17 Markus Klug , Jian Kang , Rafael M. Fernandes , Jörg Schmalian

Magnetism and nematic order are the two non-superconducting orders observed in iron-based superconductors. To elucidate the interplay between them and ultimately unveil the pairing mechanism, several models have been investigated. In models…

Superconductivity · Physics 2016-12-07 Andrey V. Chubukov , Maxim Khodas , Rafael M. Fernandes

We study the electronic and magnetic properties of L1$_0$ phase of FeNi, a perspective rare-earth-free permanent magnet, by using a combination of density functional and dynamical mean-field theory. Although L1$_0$ FeNi has a slightly…

Strongly Correlated Electrons · Physics 2020-07-02 A. S. Belozerov , A. A. Katanin , V. I. Anisimov

Neutron diffraction studies of Ba(Fe[1-x]Co[x])2As2 reveal that commensurate antiferromagnetic order gives way to incommensurate magnetic order for Co compositions between 0.056 < x < 0.06. The incommensurability has the form of a small…

Ultra-thin FeAs is of interest both as the active component in the newly identified pnictide superconductors, and in spintronic applications at the interface between ferromagnetic Fe and semiconducting GaAs. Here we use first-principles…

Superconductivity · Physics 2013-05-30 Sinéad M. Griffin , Nicola A. Spaldin

The unconventional superconductivity in the newly discovered iron-based superconductors is intimately related to its multi-band/multi-orbital nature. Here we report the comprehensive orbital characters of the low-energy three-dimensional…

The magnetic properties of iron-arsenides are investigated using the LSDA+U approach. In addition to one high moment state, we find that a positive U also produces two low moment states with m~0.4 $\mu_{B}$ and m~1.0 $\mu_{B}$. The…

Superconductivity · Physics 2011-05-30 Guo-Qiang Liu

We argue that the newly discovered superconductivity in a nearly magnetic, Fe-based layered compound is unconventional and mediated by antiferromagnetic spin fluctuations, though different from the usual superexchange and specific to this…

Superconductivity · Physics 2015-05-13 I. I. Mazin , D. J. Singh , M. D. Johannes , M. H. Du

We examine the influence of the excess of interstitial Fe on the magnetic properties of Fe$_{1+y}$Te compounds. Because in iron chalcogenides the correlations are stronger than in the iron arsenides, we assume in our model that some of the…

Strongly Correlated Electrons · Physics 2015-06-22 Samuel Ducatman , Rafael M. Fernandes , Natalia B. Perkins

The presence of macroscopic phase separation into superconducting and magnetic phases in LaFeAsO$_{1-x}$F$_x$ (LFAOF) and CaFe$_{1-x}$Co$_x$AsF (CFCAF) is demonstrated by muon spin rotation (muSR) measurement across their phase boundaries…

Superconductivity · Physics 2009-04-01 S. Takeshita , R. Kadono

The lattice dynamics of the superconducting materials LaFeSiH and LaFeSiO as well as their intermetallic precursor LaFeSi are investigated by polarized Raman spectroscopy and first-principles calculations, together with X-ray and advanced…

Iron oxide is one of the most important components in Earth's mantle. Recent discovery of the stable presence of Fe5O6 at Earth's mantle environment stimulates significant interests in the understanding of this new category of iron oxides.…

Materials Science · Physics 2021-09-01 Qiao-Ying Qin , Ai-Qin Yang , Xiang-Ru Tao , Liu-Xiang Yang , Hui-Yang Gou , Peng Zhang

A density functional theory study of the BiS$_{2}$ superconductors containing rare-earths: \textit{Ln}O$_{1-x}$F$_{x}$BiS$_{2}$ (\textit{Ln} = La, Ce, Pr, and Nd) is presented. We find that CeO$_{0.5}$F$_{0.5}$BiS$_{2}$ has competing…

Superconductivity · Physics 2017-06-21 Corentin Morice , Emilio Artacho , Sian E. Dutton , Hyeong-Jin Kim , Siddharth S. Saxena

Unlike the ferropnictide superconductors, which crystallize in a tetragonal crystal structure, binary FeAs forms in an orthorhombic crystal structure, where the local atomic environment resembles a highly distorted variant of the FeAs4…

Other Condensed Matter · Physics 2015-03-17 J. R. Jeffries , N. P. Butch , H. Cynn , S. R. Saha , K. Kirshenbaum , S. T. Weir , Y. K. Vohra , J. Paglione

By using variational Monte Carlo method, we examine an effective low-energy model for LaFeAsO derived from an ab initio downfolding scheme. We show that quantum and many-body fluctuations near a quantum critical point largely reduce the…

Strongly Correlated Electrons · Physics 2011-01-26 Takahiro Misawa , Kazuma Nakamura , Masatoshi Imada

We have studied the interplay of magnetism and superconductivity in LaFeAsO$_{1-x}$F$_x$ and Ca(Fe$_{1-x}$Co$_x$)$_2$As$_2$. While antiferromagnetic spin density wave formation is suppressed and superconductivity evolves, all samples show a…

We have calculated the local magnetic susceptibility of one of the prototypical Fe-based superconductors (LaFeAsO) by means of the local density approximation + dynamical mean field theory as a function of both (imaginary) time and real…

Strongly Correlated Electrons · Physics 2012-08-28 A. Toschi , R. Arita , P. Hansmann , G. Sangiovanni , K. Held

The transition temperature Tc~26 K of the recently discovered superconductor LaFeAs(O,F) has been demonstrated to be extremely sensitive to the lanthanide ion, reaching 55 K for the Sm containing oxypnictides. Therefore, it is important to…

Superconductivity · Physics 2008-12-17 Y. Qiu , Wei Bao , Q. Huang , T. Yildirim , J. Simmons , J. W. Lynn , Y. C. Gasparovic , J. Li , M. Green , T. Wu , G. Wu , X. H. Chen

Disentangling orbital (OAM) and spin (SAM) angular momenta in the ultrafast spin dynamics of two-dimensional (2D) ferromagnets on subfemtoseconds is a challenge in the field of ultrafast magnetism. Herein, we employed non-collinear spin…

Materials Science · Physics 2024-01-09 Shuo Li , Ran Wang , Thomas Frauenheim , Junjie He

Motivated by the discovery of superconductivity in F-doped LaFeAsO, we investigated the magnetic fluctuations in a related compound Fe(Se1-xTex)0.92 (x = 0.75, 1) using neutron scattering techniques. Non-superconducting FeTe0.92 shows…

Strongly Correlated Electrons · Physics 2015-05-13 Satoshi Iikubo , Masaki Fujita , Seiji Niitaka , Hidenori Takagi