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The present paper gives an elaborate theoretical description of a new molecular charge transport mechanism applying to a single molecule trapped between two macroscopic electrodes in a solid state device. It is shown by a Hubbard type model…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Per Hedegard , Thomas Bjornholm

It was recently suggested that molecular junctions would be excellent elements for efficient and high-power thermoelectric energy conversion devices. However, experimental measurements of thermoelectric conversion in molecular junctions…

Mesoscale and Nanoscale Physics · Physics 2015-06-09 Elinor Zerah-Harush , Yonatan Dubi

We demonstrate theoretically that it is possible to use Rabi oscillations to coherently control the electron tunneling in an asymmetric double quantum dot system, a quantum dot molecule. By applying an optical pump pulse we can excite an…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 J. M. Villas-Boas , A. O. Govorov , Sergio E. Ulloa

Graphene electrodes are promising candidates to improve reproducibility and stability in molecular electronics through new electrode-molecule anchoring strategies. Here we report sequential electron transport in few-layer graphene…

We propose a mechanism which allows one to control the transmission of single electrons through a molecular junction. The principle utilizes the emergence of transmission sidebands when molecular vibrational modes are coupled to the…

Mesoscale and Nanoscale Physics · Physics 2010-03-26 Thomas Olsen , Jakob Schiøtz

We present experimental studies of the current pumped through a dynamic quantum dot over a wide range of magnetic fields. At low fields we observe repeatable structure indicating increased confinement of the electrons in the dynamic dot. At…

We investigate on the same footing the time-dependent electronic transport properties and vibrational dynamics of a molecular junction. We show that fluctuations of both the molecular vibron displacement and the electronic current across…

Mesoscale and Nanoscale Physics · Physics 2019-03-27 Rémi Avriller , R Souto , A. Martin-Rodero , A Yeyati

We investigate the thermopower of a metal-molecule-metal junction taking into account thermal effects on the junction. Based on analytical expressions and numerical simulations we show that the thermoelectric potential reveals valuable…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Dvira Segal

The possibility to exploit quantum coherence to strongly enhance the efficiency of charge transport in solid state devices working at ambient conditions would pave the way to disruptive technological applications. In this work, we tackle…

It was once purported that biological systems were far too warm and wet to support quantum phenomena mainly due to thermal effects disrupting quantum coherence. However recent experimental results and theoretical analyses have shown that…

We study a symmetric exclusion process in which the hopping rates at two chosen adjacent sites vary periodically in time and have a relative phase difference. This mimics a colloidal suspension subjected to external space and time dependent…

Statistical Mechanics · Physics 2009-11-13 Kavita Jain , Rahul Marathe , Abhishek Chaudhuri , Abhishek Dhar

The influence of multiple vibrational modes on current fluctuations in electron transport through single-molecule junctions is investigated. Our analysis is based on a generic model of a molecular junction, which comprises a single…

Mesoscale and Nanoscale Physics · Physics 2014-09-26 C. Schinabeck , R. Härtle , H. B. Weber , M. Thoss

Coherent electron transfer from a localized state trapped in a quantum dot into a ballistic conductor, taking place in on-demand electron sources, in general may result in excitation of particle-hole pairs. We consider a simple model for…

Mesoscale and Nanoscale Physics · Physics 2008-11-07 J. Keeling , A. V. Shytov , L. S. Levitov

Low-temperature transport spectroscopy measurements on a suspended few-hole carbon nanotube quantum dot are presented, showing a gate-dependent harmonic excitation spectrum which, strikingly, occurs in the Coulomb blockade regime. The…

Mesoscale and Nanoscale Physics · Physics 2009-06-02 A. K. Huettel , B. Witkamp , M. Leijnse , M. R. Wegewijs , H. S. J. van der Zant

We investigate the photon statistics, entanglement and squeezing of a pn-junction sandwiched between two superconducting leads, and show that such an electrically-driven photon pump generates correlated and entangled pairs of photons. In…

Mesoscale and Nanoscale Physics · Physics 2014-03-14 Paul Baireuther , Peter P. Orth , Ilya Vekhter , Jörg Schmalian

We investigate the dynamics of two interacting electrons confined to a pair of coupled quantum dots driven by an external AC field. By numerically integrating the two-electron Schroedinger equation in time, we find that for certain values…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 C. E. Creffield , G. Platero

We consider a molecular junction immersed in a solvent where the electron transfer is dominated by Marcus-type steps. However, the successive nature of the charge transfer through the junction does not imply that the solvent reach thermal…

Statistical Mechanics · Physics 2022-03-23 Henning Kirchberg , Abraham Nitzan

We propose a novel molecular device that pumps heat against a thermal gradient. The system consists of a molecular element connecting two thermal reservoirs that are characterized by different spectral properties. The pumping action is…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Dvira Segal , Abraham Nitzan

Charge transfer is a fundamental process that underlies a multitude of phenomena in chemistry and biology. Recent advances in observing and manipulating charge and heat transport at the nanoscale, and recently developed techniques for…

Mesoscale and Nanoscale Physics · Physics 2016-07-26 Galen T. Craven , Abraham Nitzan

Single-electron circuits of the future, consisting of a network of quantum dots, will require a mechanism to transport electrons from one functional part to another. For example, in a quantum computer[1] decoherence and circuit complexity…

Mesoscale and Nanoscale Physics · Physics 2011-11-02 R. P. G. McNeil , M. Kataoka , C. J. B. Ford , C. H. W. Barnes , D. Anderson , G. A. C. Jones , I. Farrer , D. A. Ritchie
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