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Relaxometry schemes employing nitrogen-vacancy (NV) centers in diamonds are essential in biology and physics to detect a reduction of the color centers' characteristic spin relaxation ($T_1$) time caused by, e.g., paramagnetic molecules in…

Quantum Physics · Physics 2024-11-05 Isabel Cardoso Barbosa , Jonas Gutsche , Artur Widera

Formation and excitation energies as well charge transition levels, are determined forthe substitutional nitrogen (Ns),the vacancy (V) and related point defects (NV, NVH, N2, N2V and V2) by screened non-local hybrid density functional…

Materials Science · Physics 2013-11-27 Peter Deák , Bálint Aradi , Moloud Kaviani , Thomas Frauenheim , Adam Gali

The negatively charged nitrogen-vacancy (NV-) center in diamond has realized new frontiers in quantum technology. Here, the center's optical and spin resonances are observed under hydrostatic pressures up to 60 GPa. Our observations…

Nitrogen-vacancy (NV) centers in diamond are extensively utilized as quantum sensors for imaging fields at the nanoscale. The ultra-high sensitivity of NV magnetometers has enabled the detection and spectroscopy of individual electron…

The interaction of solid-state electronic spins with deformations of their host crystal is an important ingredient in many experiments realizing quantum information processing schemes. Here, we theoretically characterize that interaction…

Mesoscale and Nanoscale Physics · Physics 2018-08-08 Péter Udvarhelyi , Vladyslav O. Shkolnikov , Adam Gali , Guido Burkard , András Pályi

Nitrogen vacancy (NV) centers in diamond are atom-scale defects with long spin coherence times that can be used to sense magnetic fields with high sensitivity and spatial resolution. Typically, the magnetic field projection at a single…

We introduce an alternate route to dynamically polarize the nuclear spin host of nitrogen-vacancy (NV) centers in diamond. Our approach articulates optical, microwave and radio-frequency pulses to recursively transfer spin polarization from…

Quantum Physics · Physics 2014-12-18 Daniela Pagliero , Abdelghani Laraoui , Jacob D. Henshaw , Carlos A. Meriles

Here we report the increase of the coherence time T$_2$ of a single electron spin at room temperature by using dynamical decoupling. We show that the Carr-Purcell-Meiboom-Gill (CPMG) pulse sequence can prolong the T$_2$ of a single…

We demonstrate precise control over the zero-phonon optical transition energies of individual nitrogen-vacancy (NV) centers in diamond by applying multiaxis electric fields, via the dc Stark effect. The Stark shifts display surprising…

Mesoscale and Nanoscale Physics · Physics 2015-03-19 L. C. Bassett , F. J. Heremans , C. G. Yale , B. B. Buckley , D. D. Awschalom

Substitutional nitrogen atoms in a diamond crystal (P1 centers) are, on one hand, a resource for creation of nitrogen-vacancy (NV) centers, that have been widely employed as nanoscale quantum sensors. On the other hand, P1's electron spin…

The room temperature compatibility of the negatively-charged nitrogen-vacancy (NV-) in diamond makes it the ideal quantum system for a university teaching lab. Here, we describe a low-cost experimental setup for coherent control experiments…

By efficient nanoscale plasma etching, the nitrogen-vacancy (NV) centers in diamond were brought to the sample surface step by step successfully. At each depth, we used the relative ratios of spin coherence times before and after applying…

Mesoscale and Nanoscale Physics · Physics 2018-01-03 Wenlong Zhang , Jian Zhang , Junfeng Wang , Fupan Feng , Shengran Lin , Liren Lou , Wei Zhu , Guanzhong Wang

We studied the parameters to optimize the production of negatively-charged nitrogen-vacancy color centers (NV-) in type~1b single crystal diamond using proton irradiation followed by thermal annealing under vacuum. Several samples were…

Materials Science · Physics 2015-05-28 J. Botsoa , T. Sauvage , M. -P. Adam , P. Desgardin , E. Leoni , B. Courtois , F. Treussart , M. -F. Barthe

Single defect centers in diamond have been generated via nitrogen implantation. The defects have been investigated by single defect center fluorescence microscopy. Optical and EPR spectra unambiguously show that the produced defect is the…

Materials Science · Physics 2009-11-11 J. Meijer , B. Burchard , M. Domhan , C. Wittmann , T. Gaebel , I. Popa , F. Jelezko , J. Wrachtrup

We show that electric field noise from surface charge fluctuations can be a significant source of spin decoherence for near-surface nitrogen-vacancy (NV) centers in diamond. This conclusion is based on the increase in spin coherence…

Mesoscale and Nanoscale Physics · Physics 2015-08-26 M. Kim , H. J. Mamin , M. H. Sherwood , K. Ohno , D. D. Awschalom , D. Rugar

We investigate the electron spin resonance of an ensemble of Nitrogen-Vacancy (NV) color centers in a bulk diamond crystal. The four possible orientations of the NV-center in the lattice lead to different dependences on the magnitude and…

Materials Science · Physics 2009-09-08 Ngoc Diep Lai , Dingwei Zheng , Fedor Jelezko , François Treussart , Jean-François Roch

We present a scheme of positioning a single electron spin with sub-nanometer resolution through multiple nitrogen-vacancy centers in diamond. With unwanted noise suppressed by dynamical decoupling, the spin coherence of each center develops…

Quantum Physics · Physics 2016-04-27 Wen-Long Ma , Shu-Shen Li , Geng-Yu Cao , Ren-Bao Liu

The nitrogen-vacancy (NV) centre in diamond has emerged as a candidate to non-invasively hyperpolarise nuclear spins in molecular systems to improve the sensitivity of nuclear magnetic resonance (NMR) experiments. Several promising proof of…

Mesoscale and Nanoscale Physics · Physics 2021-05-26 A. J. Healey , L. T. Hall , G. A. L. White , T. Teraji , M. -A. Sani , F. Separovic , J. -P. Tetienne , L. C. L. Hollenberg

Scalable realizations of quantum network technologies utilizing the nitrogen vacancy center in diamond require creation of optically coherent NV centers in close proximity to a surface for coupling to optical structures. We create single NV…

Mesoscale and Nanoscale Physics · Physics 2021-09-01 Srivatsa Chakravarthi , Christian Pederson , Zeeshawn Kazi , Andrew Ivanov , Kai-Mei C. Fu

Although a nuclear spin is weakly coupled to its environment, due to its small gyromagnetic ratio, its coherence time is limited by the hyperfine coupling to a nearby noisy electron. Here, we propose to utilize continuous dynamical…

Quantum Physics · Physics 2017-03-07 Itsik Cohen , Thomas Unden , Fedor Jelezko , Alex Retzker