Related papers: Single-pulse stimulated Raman scattering spectrosc…
Micro-ring resonators (MRRs) "trap" incoming light, and therefore, have been shown to achieve extremely high local intensities of light. Thus, they can be used to facilitate highly non-linear optical signals. By embedding materials that…
The hybrid Stimulated Raman Scattering - Two Plasmon Decay instability had shown to play the dominant role for plasma waves excitation and energy absorption at interaction of very intense femtosecond obliquely incident $p$-polarized laser…
Single-shot ultrafast absorbance spectroscopy based on the frequency encoding of the kinetics is analyzed theoretically and implemented experimentally. The kinetics are sampled in the frequency domain using linearly chirped, amplified 33 fs…
We investigate the evolution of coherence property of noise-seeded Stokes wave in short (< 1 ps) and long pulse (> 1 ps) regimes. Nonlinear equations expressing the evolution of pump and Stokes wave are solved numerically for both the…
Stimulated Raman scattering of a laser pump pulse seeded by a Stokes pulse generically leaves a two-level medium initially at rest in an excited state constituted of static solitons and radiation. The soliton birth manifests as sudden very…
In a recent experiment (N. Wagner et al., PNAS v103, p13279) on SF$_{6}$, a high-harmonic generating laser pulse is preceded by a pump pulse which stimulates Raman-active modes in the molecule. Varying the time delay between the two pulses…
A coherent microwave radiation, concomitant with experiments of stimulated Raman scattering (SRS) in weakly compressed hydrogen, had been observed; qualitative and quantitative results had been obtained, and are given in this article. .An…
We present a novel approach to transient Raman spectroscopy, which combines stochastic probe pulses and a covariance-based detection to measure stimulated Raman signals in alpha-quartz. A coherent broadband pump is used to simultaneously…
In this work we extend low frequency impulsive stimulated Raman microspectroscopy to the pre-electronic resonance regime. We use a broadband two color collinear pump probe scheme which can be readily extended to imaging. We discuss the…
Raman spectroscopy is a powerful and non-invasive method for analysis of chemicals and detection of unknown substances. However, Raman signal is so weak that background noise can distort the actual Raman signal. These baseline shifts that…
The key challenge of time-resolved Raman spectroscopy is the identification of the constituent species and the analysis of the kinetics of the underlying reaction network. In this work we present an integral approach that allows for…
Quantum networks require flying qubits that transfer information between the nodes. This may be implemented by means of single atoms (the nodes) that emit and absorb single photons (the flying qubits) and requires full control of photon…
Linear off-resonant X-ray Raman techniques are capable of detecting the ultrafast electronic coherences generated when a photoexcited wave packet passes through a conical intersection. A hybrid femtosecond or attosecond probe pulse is…
In this work, we present a high pulse energy multi-wavelength Raman laser spanning from 1.53 um up to 2.4 um by employing the cascaded rotational stimulated Raman scattering (SRS) effect in a 5-m hydrogen (H2) -filled nested anti-resonant…
The bonding configuration of the crater walls formed in urethane dimethacrylate-based polymer doped with plasmonic gold nanorods upon irradiation with a single-shot high-energy femtosecond laser pulse has been studied by Raman spectroscopy.…
Lead sulfide is an important semiconductor that has found technological applications for over a century. Raman spectroscopy, a standard tool for the investigation and characterization of semiconductors, has limited application to this…
Stimulated Raman scattering (SRS) microscopy is a highly sensitive chemical imaging technique. However, the broader application of SRS has been limited by two key challenges: the reliance on low-noise but bulky solid-state laser sources and…
We present a simple and efficient method for refining maps or correspondences by iterative upsampling in the spectral domain that can be implemented in a few lines of code. Our main observation is that high quality maps can be obtained even…
A possibility to greatly enhance frequency-conversion efficiency of stimulated Raman scattering is shown by making use of extraordinary properties of three-wave mixing of ordinary and backward waves. Such processes are commonly attributed…
Raman scattering enables unforeseen uses for the laser guide-star system of the Very Large Telescope. Here, we present the observation of one up-link sodium laser beam acquired with the ESPRESSO spectrograph at a resolution…