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Spin-polarized transport through bistable magnetic adatoms or single-molecule magnets (SMMs), which exhibit both uniaxial and transverse magnetic anisotropy, is considered theoretically. The main focus is on the impact of transverse…

Mesoscale and Nanoscale Physics · Physics 2014-07-22 Maciej Misiorny , Józef Barnaś

We study the full counting statistics (FCS) in a single-molecule magnet (SMM) with finite Coulomb interaction $U$. For finite $U$ the FCS, differing from $U\rightarrow \infty $, shows a symmetric gate-voltage-dependence when the coupling…

Mesoscale and Nanoscale Physics · Physics 2011-01-05 Hai-Bin Xue , Y. -H. Nie , Z. -J. Li , J. -Q. Liang

By means of electronic transport, we study the transverse magnetic anisotropy of an individual Fe$_4$ single-molecule magnet (SMM) embedded in a three-terminal junction. In particular, we determine in situ the transverse anisotropy of the…

Mesoscale and Nanoscale Physics · Physics 2016-08-10 M. Misiorny , E. Burzurí , R. Gaudenzi , K. Park , M. Leijnse , M. R. Wegewijs , J. Paaske , A. Cornia , H. S. J. van der Zant

We present a method for precisely measuring the tunnel splitting in single-molecule magnets using electron-spin resonance, and use these measurements to precisely and independently determine the underlying transverse anisotropy parameter,…

Mesoscale and Nanoscale Physics · Physics 2016-12-13 Charles A. Collett , Rafael A. Allão Cassaro , Jonathan R. Friedman

Anisotropic magnetic molecules can be employed to manipulate charge transport in molecular nanojunctions. Charge transport through a molecular orbital connected to two leads and exchange-coupled with a precessing anisotropic molecular spin…

Mesoscale and Nanoscale Physics · Physics 2025-09-09 Milena Filipovic

We demonstrate that in a single molecule magnet (SMM) strongly coupled to electrodes the Kondo effect involves all magnetic excitations. This Kondo effect is induced by the quantum tunneling of the magnetic moment (QTM). Importantly, the…

Strongly Correlated Electrons · Physics 2009-11-11 C. Romeike , M. R. Wegewijs , W. Hofstetter , H. Schoeller

We investigate theoretically shot noise in an artificial Single Molecule Magnet based upon a CdTe quantum dot doped with a single S=5/2 Mn spin and gated in the hole sector. Mn-hole exchange anisotropy is shown to lead to profound…

Mesoscale and Nanoscale Physics · Physics 2011-03-31 L. D. Contreras-Pulido , R. Aguado

We review different electron transport methods to probe the magnetic properties, such as the magnetic anisotropy, of an individual Fe4 SMM. The different approaches comprise first and higher order transport through the molecule. Gate…

Mesoscale and Nanoscale Physics · Physics 2016-06-09 E. Burzurí , R. Gaudenzi , H. S. J. van der Zant

We demonstrate that transport spectroscopy of single molecular magnets shows signatures of quantum tunneling at low temperatures. We find current and noise oscillations as function of bias voltage due to a weak violation of spin selection…

Strongly Correlated Electrons · Physics 2009-11-11 C. Romeike , M. R. Wegewijs , H. Schoeller

Molecular spintroinic device based on a single-molecule magnet is one of the ultimate goals of semiconductor nanofabrication technologies. It is thus necessary to understand the electron transport properties of a single-molecule magnet…

Mesoscale and Nanoscale Physics · Physics 2014-10-15 Hai-Bin Xue , Jiu-Qing Liang , Wu-Ming Liu

To understand the effect of molecular environment on the electronic and magnetic properties of the single-molecule magnet (SMM) Mn$_{12}$, we explore two possible means for adding extra electrons to molecule. We explore both substitution of…

Materials Science · Physics 2009-11-10 Kyungwha Park , Mark R. Pederson

W-band ({\nu} ca. 94 GHz) electron paramagnetic resonance (EPR) spectroscopy was used for a single-crystal study of a star-shaped Fe3Cr single-molecule magnet (SMM) with crystallographically imposed trigonal symmetry. The high resolution…

Mesoscale and Nanoscale Physics · Physics 2013-09-13 L. Sorace , M. -E. Boulon , P. Totaro , A. Cornia , J. Fernandes-Soares , R. Sessoli

Spin-dependent transport through a multilevel quantum dot weakly coupled to ferromagnetic leads is analyzed theoretically by means of the real-time diagrammatic technique. Both the sequential and cotunneling processes are taken into…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 I. Weymann , J. Barnas

The transport properties of a large-spin molecule strongly coupled to ferromagnetic leads in the presence of transverse magnetic anisotropy are studied theoretically. The relevant spectral functions, linear-response conductance and the…

Mesoscale and Nanoscale Physics · Physics 2015-11-13 Maciej Misiorny , Ireneusz Weymann

We determine the shot noise asymmetry of a quantum dot under reversal of an external magnetic field. The dot is coupled to edge states which invert their chirality when the field is reversed, leading to a magnetoasymmetric electrochemical…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 David Sanchez

We have measured quantum transport through an individual Fe$_4$ single-molecule magnet embedded in a three-terminal device geometry. The characteristic zero-field splittings of adjacent charge states and their magnetic field evolution are…

We theoretically investigate the effect of transverse magnetic anisotropy on spin-flip assisted tunneling through atomic spin chains. Using a phenomenological approach and first-order perturbation theory, we analytically calculate the…

Mesoscale and Nanoscale Physics · Physics 2017-05-17 J. Hageman , M. Blaauboer

Transport properties in the Kondo regime of a nanosystem displaying uniaxial magnetic anisotropy (such as a magnetic molecule, magnetic adatom or quantum dot coupled to a localized magnetic moment) are analyzed theoretically. In particular,…

Mesoscale and Nanoscale Physics · Physics 2012-06-06 Maciej Misiorny , Ireneusz Weymann , Jozef Barnas

We study single-electron transport in a three-ion molecule with strong uniaxial anisotropy and in the presence of a transverse magnetic field. Two magnetic ions are connected to each other through a third, nonmagnetic ion. The magnetic ions…

Mesoscale and Nanoscale Physics · Physics 2014-05-12 Javier I. Romero , Eduardo R. Mucciolo

We analyze shot noise in a magnetic tunnel junction with a two-level quantum dot attached to the magnetic electrodes. The considerations are limited to the case when some transport channels are suppressed at low temperatures. Coupling of…

Mesoscale and Nanoscale Physics · Physics 2017-01-10 T. Szczepanski , V. K. Dugaev , J. Barnas , I. Martinez , J. P. Cascales , J. -Y. Hong , M. -T. Lin , F. G. Aliev
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