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We derive and implement a new way of solving coupled cluster equations with lower computational scaling. Our method is based on decomposition of both amplitudes and two electron integrals, using a combination of tensor hypercontraction and…

Chemical Physics · Physics 2020-05-14 Roman Schutski , Jinmo Zhao , Thomas M. Henderson , Gustavo E. Scuseria

Unitary coupled cluster (UCC) theory offers a promising Hermitian alternative to conventional coupled cluster (CC) theory, but its practical implementation is hindered by the non-truncating nature of the Baker-Campbell-Hausdorff (BCH)…

Chemical Physics · Physics 2025-05-05 Justin T. Phillips , Lauren N. Koulias , Stephen H. Yuwono , A. Eugene DePrince

A parallel splitting method is proposed for solving systems of coupled monotone inclusions in Hilbert spaces. Convergence is established for a wide class of coupling schemes. Unlike classical alternating algorithms, which are limited to two…

Optimization and Control · Mathematics 2009-02-26 H. Attouch , L. M. Briceno-Arias , P. L. Combettes

A modified version of the Moller-Plesset approach for obtaining the correlation energy associated to a Hartree-Fock ground state is proposed. The method is tested in a model of interacting fermions that allows for an exact solution. Using…

Materials Science · Physics 2016-10-12 Alejandro Cabo , Francisco Claro , Eduardo Menendez-Proupin

The Hartree-Fock-Bogoliubov approximation is very useful for treating both long- and short-range correlations in finite quantum fermion systems, but it must be extended in order to describe detailed spectroscopic properties. One problem is…

Nuclear Theory · Physics 2017-08-23 L. M. Robledo , G. F. Bertsch

A coupled-cluster approach for systems of $N$ bosons in external traps is developed. In the coupled-cluster approach the exact many-body wavefunction is obtained by applying an exponential operator $\exp{T}$ to the ground configuration…

Other Condensed Matter · Physics 2009-11-11 Lorenz S. Cederbaum , Ofir E. Alon , Alexej I. Streltsov

Coupled cluster methods are widely regarded as the gold standard of computational quantum chemistry as they are perceived to offer the best compromise between computational cost and a high-accuracy resolution of the ground state eigenvalue…

Numerical Analysis · Mathematics 2025-12-03 Muhammad Hassan , Yvon Maday

We propose to improve the convergence properties of the single-reference coupled cluster (CC) method through an augmented Lagrangian formalism. The conventional CC method changes a linear high-dimensional eigenvalue problem with exponential…

Computational Physics · Physics 2024-03-26 Fabian M. Faulstich , Yuehaw Khoo , Kangbo Li

Tailored coupled cluster theory represents a computationally inexpensive way to describe static and dynamical electron correlation effects. In this work, we scrutinize the performance of various tailored coupled cluster methods externally…

Chemical Physics · Physics 2021-03-24 Aleksandra Leszczyk , Mihály Máté , Örs Legeza , Katharina Boguslawski

Over the past decade, a combinatorial framework for discrete, finite, and irreversibly aggregating systems has emerged. This work reviews its progress, practical applications, and limitations. We outline the approach's assumptions and…

Statistical Mechanics · Physics 2026-01-06 Michał Łepek , Agata Fronczak , Piotr Fronczak

A simple ``brute-force'' parallelisation procedure for the computational implementation of high-order coupled cluster method (CCM) calculations is presented here. This approach is investigated and illustrated by an application of high-order…

Strongly Correlated Electrons · Physics 2007-05-23 D. J. J. Farnell , R. F. Bishop

In the context of clustering, we consider a generative model in a Euclidean ambient space with clusters of different shapes, dimensions, sizes and densities. In an asymptotic setting where the number of points becomes large, we obtain…

Machine Learning · Statistics 2009-09-15 Ery Arias-Castro

We develop coupled-cluster theory for systems of electrons strongly coupled to photons, providing a promising theoretical tool in polaritonic chemistry with a perspective of application to all types of fermion-boson coupled systems. We show…

We have studied electron correlations in the doped two-dimensional (2D) Hubbard model by using the coupled-cluster method (CCM) to investigate whether or not the method can be applied to correct the independent particle approximations…

Strongly Correlated Electrons · Physics 2009-10-31 Yoshihiro Asai , Hideki Katagiri

The ground state correlations induced by a general pairing Hamiltonian in a finite system of like fermions are described in terms of four-body correlated structures (quartets). These are real superpositions of products of two pairs of…

Nuclear Theory · Physics 2015-06-15 M. Sambataro , N. Sandulescu

In this article, we investigate partially truncated correlation functions (PTCF) of infinite continuous systems of classical point particles with pair interaction. We derive Kirkwood-Salsburg-type equations for the PTCF and write the…

Mathematical Physics · Physics 2020-12-22 Tony C. Dorlas , Alexei L. Rebenko , Baptiste Savoie

Making and using polaritonic states (i.e., hybrid electron-photon states) for chemical applications have recently become one of the most prominent and active fields that connects the communities of chemistry and quantum optics. Modeling of…

Chemical Physics · Physics 2023-09-06 Braden M. Weight , Sergei Tretiak , Yu Zhang

In this paper, we propose a general model for plane-based clustering. The general model contains many existing plane-based clustering methods, e.g., k-plane clustering (kPC), proximal plane clustering (PPC), twin support vector clustering…

Machine Learning · Computer Science 2020-09-24 Zhen Wang , Yuan-Hai Shao , Lan Bai , Chun-Na Li , Li-Ming Liu

We consider a new formulation of the stochastic coupled cluster method in terms of the similarity transformed Hamiltonian. We show that improvement in the granularity with which the wavefunction is represented results in a reduction in the…

Chemical Physics · Physics 2016-02-02 Ruth S. T. Franklin , James S. Spencer , Alberto Zoccante , Alex J. W. Thom

Convergence problems in coupled-cluster iterations are discussed, and a new iteration scheme is proposed. Whereas the Jacobi method inverts only the diagonal part of the large matrix of equation coefficients, we invert a matrix which also…

Chemical Physics · Physics 2009-11-06 N. Mosyagin , E. Eliav , U. Kaldor