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By using first-principles methods based on density functional theory we revisited the zero-temperature phase diagram of stoichiometric SrCoO3, a ferromagnetic metallic perovskite that undergoes significant structural, electronic, and…

Materials Science · Physics 2016-12-21 Pablo Rivero , Claudio Cazorla

Iridium oxides (iridates) provide a good platform to study the delicate interplay between spin-orbit coupling (SOC) interactions, electron correlation effects, Hund's coupling and lattice degree of freedom. However, overwhelming…

Strongly Correlated Electrons · Physics 2024-01-09 Xujia Gong , Carmine Autieri , Huanfu Zhou , Jiafeng Ma , Xin Tang , Xiaojun Zheng , Xing Ming

We have synthesized and characterized laser-deposited film samples of perovskite BaCrO_{3}, a missing member of the perovskite-chromate family. The BaCrO_{3} films have a substantially larger lattice constant than other chromates, are…

Materials Science · Physics 2016-04-14 Z. H. Zhu , F. J. Rueckert , J. I. Budnick , W. A. Hines , M. Jain , H. Zhang , B. O. Wells

A new layered perovskite-type oxide Ba$_2$RhO$_4$ was synthesized by a high-pressure technique with the support of convex-hull calculations. The crystal and electronic structure were studied by both experimental and computational tools.…

Strongly Correlated Electrons · Physics 2021-02-03 I. Kurata , José A. Flores-Livas , H. Sugimoto , H. Takahashi , H. Sagayama , Y. Yamasaki , T. Nomoto , R. Arita , S. Ishiwata

Using an extension of a first-principles method developed by King-Smith and Vanderbilt [Phys. Rev. B {\bf 49}, 5828 (1994)], we investigate the effects of in-plane epitaxial strain on the ground-state structure and polarization of eight…

Materials Science · Physics 2009-12-22 Oswaldo Dieguez , Karin M. Rabe , David Vanderbilt

The short-range organization around Ni atoms in orthorhombic $R$NiO$_{3}$ ($R$=Pr,Nd,Eu) perovskites has been studied over a wide temperature range by Ni K-edge x-ray absorption spectroscopy. Our results demonstrate that two different Ni…

A monoclinic phase was recently discovered near the morphotropic phase boundary in several high-performance piezoelectric perovskite solid solutions, but its properties have not been reported. In this paper the dielectric, piezo- and…

Materials Science · Physics 2016-08-31 A. A. Bokov , Z. -G. Ye

5d transition-metal-based oxides display emergent phenomena due to the competition between the relevant energy scales of the correlation, bandwidth, and most importantly, the strong spin-orbit coupling (SOC). Starting from the prediction of…

Strongly Correlated Electrons · Physics 2017-04-04 Abhijit Biswas , Yoon Hee Jeong

The novel 4d perovskite compound SrRhO3 was investigated by isovalent doping studies. The solubility limits of Ca and Ba onto Sr-site were below 80% and 20%, respectively. Although SrRhO3 was chemically compressed, approximately 5.7% by the…

Strongly Correlated Electrons · Physics 2009-11-07 K. Yamaura , Q. Huang , D. P. Young , M. Arai , E. Takayama-Muromachi

Variable resistors were constructed from epitaxial SrRuO3 (SRO), La0.67Sr0.33MnO3 (LSMO) and SrTiO3 layers with perovskite crystal structure. Each layer was patterned separately by lithographic methods. Optimized wet chemical etchants and…

Materials Science · Physics 2013-01-22 Dieter Weber , Róza Vöfély , Yuehua Chen , Yulia Mourzina , Ulrich Poppe

Using the full-potential linearized-augmented-plane-wave (FLAPW) method, we have analyzed systematically the trends in the structural and electronic properties of the 3d and 4d transition-metal oxides SrMO_3 (M = Ti, V, Zr and Nb). The…

Materials Science · Physics 2016-08-31 I. R. Shein , V. L. Kozhevnikov , A. L. Ivanovskii

Organic or inorganic (A) metal (M) halide (X) perovskites (AMX3) are semiconductor materials setting the basis for the development of highly efficient, low-cost and multijunction solar energy conversion devices. The best efficiencies…

Materials Science · Physics 2018-10-17 Frederike Lehmann , Silvia Binet , Alexandra Franz , Andreas Taubert , Susan Schorr

The competition between kinematic, relativistic and Coulombic interactions in iridium-based oxides has spurred intense experimental and theoretical investigations regarding the electronic structure and magnetism. We argue here that the…

Strongly Correlated Electrons · Physics 2025-02-25 Kuldeep Kargeti , Bidyut Mallick , Vladislav Borisov , Sk. Soyeb Ali , Johan Hellsvik , Olle Eriksson , S. K. Panda

We report the time dependent response of electrical resistivity in the non-magnetic perovskite oxide NdNiO$_3$ in its phase separated state and provide a physical explanation of the observations. We also model the system and do an accurate…

Other Condensed Matter · Physics 2012-10-26 Devendra Kumar , K. P. Rajeev , J. A. Alonso , M. J. Martinez-Lope

Recent discovery of HfO2-based and nitride-based ferroelectrics that are compatible to the semiconductor manufacturing process have revitalized the field of ferroelectric-based nanoelectronics. Guided by a simple design principle of charge…

Materials Science · Physics 2023-04-19 Qisheng Yu , Jiawei Huang , Changming Ke , Zhuang Qian , Liyang Ma , Shi Liu

Silver niobate is a conventional perovskite oxide compound, known to exhibit a rich polymorphism. Although often classified as antiferroelectric, its low-temperature structure remains unclear. Here, first-principles calculations reveal a…

Materials Science · Physics 2026-04-13 Safari Amisi , Fernando Gómez-Ortiz , Eric Bousquet , Philippe Ghosez

The recent reports of superconductivity in Nd1-xSrxNiO2/SrTiO3 heterostructures have reinvigorated interest in potential superconductivity of low-valence nickelates. Synthesis of Ni1+-containing compounds is notoriously difficult. In the…

SrIrO$_3$ crystallizes in a monoclinic structure of distorted hexagonal perovskite at ambient pressure. The transport measurements show that the monoclinic SrIrO$_3$ is a low-carrier density semimetal, as in the orthorhombic perovskite…

Strongly Correlated Electrons · Physics 2019-01-30 T. Takayama , A. N. Yaresko , H. Takagi

We have investigated the electronic structure of meta-stable perovskite Ca1-xSrxIrO3 (x = 0, 0.5, and 1) thin films using transport measurements, optical spectroscopy, and first-principles calculations. We artificially fabricated the…

Strongly Correlated Electrons · Physics 2015-05-14 S. Y. Jang , H. S. Kim , S. J. Moon , W. S. Choi , B. C. Jeon , J. Yu , T. W. Noh

While nature provides a plethora of perovskite materials, only a few exhibits large ferroelectricity and possibly multiferroicity. The majority of perovskite materials have the non-polar CaTiO$_3$(CTO)structure, limiting the scope of their…

Materials Science · Physics 2022-05-25 Hongwei Wang , Fujie Tang , Massimiliano Stengel , Hongjun Xiang , Qi An , Tony Low , Xifan Wu