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Coherent phonons (CP) generated by laser pulses on the femtosecond scale have been proposed as a means to achieve ultrafast, non-thermal switching in phase-change materials such as Ge$_{2}$Sb$_{2}$Te$_{5}$(GST). Here we use ultrafast…

We report on the generation of four spatially multiplexed picosecond 40-GHz pulse trains in a km-long 6-LP multimode optical fiber. The principle of operation is based on the parallel nonlinear compression of initial beat-signals into well…

Optics · Physics 2020-04-08 H. Zhang , M. Bigot-Astruc , P. Sillard , Julien Fatome

Time-resolved spectroscopies using intense THz pulses appear as a promising tool to address collective electronic excitations in condensed matter. In particular recent experiments showed the possibility to selectively excite collective…

Strongly Correlated Electrons · Physics 2019-11-18 Mattia Udina , Tommaso Cea , Lara Benfatto

We analyse the temporal properties of the optical pulse wave that is obtained by applying a set of spectral $\pi/2$ phase shifts to continuous-wave light that is phase-modulated by a temporal sinusoidal wave. We develop an analytical model…

Gallium selenide (GaSe) is an efficient nonlinear crystal for electro-optic (EO) sampling in the multi-terahertz (THz) frequency range. However, the lattice resonance at several THz frequencies hampers broadband EO sampling, resulting in…

Dynamical control of the nonlinear optical properties of solids -- with light itself -- will be essential for future ultrafast photonic technologies. Previously, methods to modulate nonlinear processes including second-harmonic generation…

There are implementations and proposals for using microwave or optical radiation for electron acceleration, undulation, deflection, and spatial as well as temporal focusing. Using terahertz (THz) radiation in such applications can be…

Accelerator Physics · Physics 2011-10-03 J. Hebling , J. A. Fülöp , M. I. Mechler , L. Pálfalvi , C. Tőke , G. Almási

We demonstrate the generation of coherent phonons in a quartz Bulk Acoustic Wave (BAW) resonator through the photoelastic properties of the crystal, via the coupling to a microwave cavity enhanced by a photonic lambda scheme. This is…

We theoretically and experimentally demonstrate a new electro-optic linear approach to generate high repetition-rate picosecond pulse trains. This simple cavity-free method is based on a temporal sinusoidal phase modulation combined with a…

Optics · Physics 2019-10-23 Ugo Andral , Julien Fatome , Bertrand Kibler , Christophe Finot

Coupling phase-stable single-cycle terahertz (THz) pulses to scanning tunneling microscope (STM) junctions enables spatio-temporal imaging with femtosecond temporal and \r{A}ngstrom spatial resolution. The time resolution achieved in such…

Applied Physics · Physics 2020-08-28 Melanie Müller , Natalia Martín Sabanés , Tobias Kampfrath , Martin Wolf

Optical rectification of ultrashort laser pulses in LiNbO3 by tilted-pulse-front excitation is a powerful way to generate near single-cycle terahertz (THz) pulses. Motivated by various applications, calculations were carried out to optimize…

We demonstrate a compact source of energetic and phase-locked multi-terahertz pulses at a repetition rate of 190 kHz. Difference frequency mixing of the fundamental output of an Yb:KGW amplifier with the idler of an optical parametric…

Many experiments in biological and medical sciences currently use multiphoton microscopy as a core imaging technique. To date, solid-state lasers are most commonly used as excitation beam sources. However, the most demanding applications…

Strong-field mid-infrared pump--terahertz (THz) probe spectroscopy has been proven as a powerful tool for light control of different orders in strongly correlated materials. We report the construction of an ultrafast broadband infrared…

Instrumentation and Detectors · Physics 2017-10-10 S. J. Zhang , Z. X. Wang , T. Dong , N. L. Wang

We propose an experimental technique to generate large amplitude coherent phonons with irradiation of THz-rate pump pulses and to study the dynamics of phase transition in GeTe ferroelectrics. When a single pump pulse irradiates the sample…

Materials Science · Physics 2011-02-01 Muneaki Hase , Masahiro Kitajima , Shin-ichi Nakashima , Kohji Mizoguchi

Coherent radiation with frequencies ranging from 0.3 to 30 THz has recently become accessible by femtosecond laser technology. Terahertz (THz) waves have already found many applications in spectroscopy and imaging, and they can be…

We discuss terahertz pump-probe experiments in hBN from the perspective of Floquet optical materials and photonic time crystals. Anisotropic nature of this material results in a large separation of frequencies of in-plane and out-of-plane…

The spectrum of a CW field whose phase experiences a periodic sawtooth modulation is analyzed. Two types of the sawtooth phase modulation are considered. One is created by combining many harmonics of the fundamental frequency. The second is…

Optics · Physics 2019-10-23 R. N. Shakhmuratov

Microscopic understanding of low-frequency molecular motions in liquids has been a longstanding goal in soft-matter science. So far, such low-frequency motions have mostly been accessed indirectly by off-resonant optical pulses. A more…

Soft Condensed Matter · Physics 2017-04-26 Mohsen Sajadi , Martin Wolf , Tobias Kampfrath

High-power multi-color terahertz (THz) radiation exhibits extraordinary scientific application prospects at various scientific frontiers, for its capacity to deliver THz excitation at multiple frequencies simultaneously. However, the…

Accelerator Physics · Physics 2025-10-15 Yin Kang , Weiyi Yin , Xianzhe Li , Yixuan Liu , Yue Wang , Yuan Ma , Kaiqing Zhang , Chao Feng