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We performed electron energy-loss spectroscopy studies in order to get a deeper insight into the electronic properties of potassium intercalated picene, a recently discovered superconductor. A comparison of the loss function of the undoped…

Superconductivity · Physics 2011-04-05 Friedrich Roth , Benjamin Mahns , Bernd Büchner , Martin Knupfer

We study superconductivity in doped solid picene (C22H14) with linear response calculations of the phonon spectrum and electron-phonon (ep) interaction. We show that the coupling of the high-energy C bond-stretching phonons to the {\pi}…

Superconductivity · Physics 2011-07-26 Alaska Subedi , Lilia Boeri

Potassium-doped picene (K$_x$picene) has recently been reported to be a superconductor at $x=3$ with critical temperatures up to 18 K. Here we study the electronic structure of K-doped picene films by photoelectron spectroscopy and {\it ab…

Strongly Correlated Electrons · Physics 2015-06-11 Andreas Ruff , Michael Sing , Ralph Claessen , Hunpyo Lee , Milan Tomić , Harald O. Jeschke , Roser Valentí

K$_3$-picene is a superconducting molecular crystal with critical temperature T$_c=7$K or 18K, depending on preparation conditions. Using density functional theory we show that electron-phonon interaction accounts for T$_c ~ 3-8$ K. The…

Superconductivity · Physics 2015-05-28 Michele Casula , Matteo Calandra , Gianni Profeta , Francesco Mauri

The electronic structure of the unoccupied and occupied states of potassium (K)-doped and undoped picene crystalline films has been investigated by using the element-selective and bulk-sensitive photon-detection methods of X-ray absorption…

Materials Science · Physics 2012-10-16 Hiroyuki Yamane , Nobuhiro Kosugi

By the first principles calculations and X-ray diffraction simulations, we perform a systematic study of multiple superconducting phases of potassium-doped picene [Nature {\bf464} 76, 2010]. The combination of optimized lattice parameters,…

Superconductivity · Physics 2014-07-04 Xun-Wang Yan , Zhongbing Huang , Hai-Qing Lin

Recently, Mitsuhashi et al., have observed superconductivity with transition temperature up to 18 K in potassium doped picene (C22H14), a polycyclic aromatic hydrocarbon compound [Nature 464 (2010) 76]. Theoretical analysis indicate the…

We performed electron energy-loss spectroscopy studies in transmission in order to obtain insight into the electronic properties of potassium intercalated coronene, a recently discovered superconductor with a rather high transition…

Superconductivity · Physics 2012-01-20 Friedrich Roth , Johannes Bauer , Benjamin Mahns , Bernd Büchner , Martin Knupfer

Recently, a new organic superconductor, K-intercalated Picene with high transition temperatures $T_c$ (up to 18\,K) has been discovered. We have investigated the electronic properties of the undoped relative, solid picene, using a…

Based on the first-principles density functional theory electronic structure calculation, we investigate the possible phonon-mediated superconductivity in arsenene, a two-dimensional buckled arsenic atomic sheet, under electron doping. We…

Superconductivity · Physics 2018-03-28 Xin Kong , Miao Gao , Xun-Wang Yan , Zhong-Yi Lu , Tao Xiang

We have obtained the first-principles electronic structure of solid coronene, which has been recently discovered to exhibit superconductivity with potassium doping. Since coronene, along with picene, the first aromatic superconductor, now…

Superconductivity · Physics 2015-05-28 Taichi Kosugi , Takashi Miyake , Shoji Ishibashi , Ryotaro Arita , Hideo Aoki

We propose that electron doped nontransition metal-phthalocyanines (MPc) like ZnPc and MgPc, similar to those very recently reported, should constitute novel strongly correlated metals. Due to orbital degeneracy, Jahn-Teller coupling and…

Strongly Correlated Electrons · Physics 2009-11-10 Erio Tosatti , Michele Fabrizio , Jaroslav Tobik , Giuseppe E. Santoro

We propose an electron-phonon parameterization which reliably reproduces the geometry and harmonic frequencies of a real system. With respect to standard electron-phonon models, it adds a "double-counting" correction, which takes into…

Strongly Correlated Electrons · Physics 2015-03-19 Gianluca Giovannetti , Michele Casula , Philipp Werner , Francesco Mauri , Massimo Capone

High-transition-temperature (high-Tc) superconductivity develops near antiferromagnetic phases, and it is possible that magnetic excitations contribute to the superconducting pairing mechanism. To assess the role of antiferromagnetism, it…

Superconductivity · Physics 2007-05-23 E. M. Motoyama , G. Yu , I. M. Vishik , O. P. Vajk , P. K. Mang , M. Greven

The effects of electron-electron correlations on the low-energy electronic structure and their relationship with unconventional superconductivity are central aspects in the research on the iron-based pnictide superconductors. Here we use…

To explore the electronic structure of the first aromatic superconductor, potassium-doped solid picene which has been recently discovered by Mitsuhashi et al with the transition temperatures $T_c=7 - 20$ K, we have obtained a…

Superconductivity · Physics 2015-05-14 Taichi Kosugi , Takashi Miyake , Shoji Ishibashi , Ryotaro Arita , Hideo Aoki

We present a systematical study on the roles of electron correlation and spin-orbit coupling in the isovalent Pd-doped superconductor SrPt$_3$P. By using solid state reaction method, we fabricated the strong spin-orbit coupling…

Strong electron correlation effects in the photophysics of quasi-one-dimensional $\pi$-conjugated organic systems such as polyenes, polyacetylenes, polydiacetylenes, etc., have been extensively studied. Far less is known on correlation…

Strongly Correlated Electrons · Physics 2014-02-18 K. Aryanpour , A. Roberts , A. Sandhu , R. Rathore , A. Shukla , S. Mazumdar

Antimonene is a recently discovered two-dimensional semiconductor with exceptional environmental stability, high carrier mobility, and strong spin-orbit interactions. In combination with electric field, the latter provides an additional…

Superconductivity · Physics 2019-03-06 A. V. Lugovskoi , M. I. Katsnelson , A. N. Rudenko

Electron-boson coupling plays a key role in superconductivity for many systems. However, in copper-based high-temperature ($T_c$) superconductors, its relation to superconductivity remains controversial despite strong spectroscopic…

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