Related papers: Excited electron-bubble states in superfluid heliu…
We have studied the evolution of an excited electron bubble in superfluid 4He for several tens of picoseconds combining the dynamics of the liquid with an adiabatic evolution for the electron. The path followed by the excited bubble in its…
Within Density Functional Theory, we have calculated the energy of the transitions from the ground state to the first two excited states in the electron bubbles in liquid helium at pressures from zero to about the solidification pressure.…
Discharge and electron-impact excitation lead to the production of metastable helium atoms in two metastable states, 2$^1$S$_0$ and 2$^3$S$_1$. However, many applications require pure beams of one of these species or at least a detailed…
A novel density functional, which accounts correctly for the equation of state, the static response function and the phonon-roton dispersion in bulk liquid helium, is used to predict static and dynamic properties of helium droplets. The…
A recent proposal by Maris[1], that single electron bubbles in helium might fission into separate, particle-like entities, does not properly take into account the failure of the adiabatic approximation when, due to tunneling, there is a…
We present a novel joint time-dependent density-functional theory for the description of solute-solvent systems in time-dependent external potentials. Starting with the exact quantum-mechanical action functional for both electrons and…
Quantum calculations are performed for an anion water cluster representing the first hydration shell of the solvated electron in solution. The absorption spectra from the ground state, the instant excited states and the relaxed excited…
We present a novel density functional for liquid 4He, properly accounting for the static response function and the phonon-roton dispersion in the uniform liquid. The functional is used to study both structural and dynamical properties of…
The $1s^2->1s2p(^1P)$ excitation in confined and compressed helium atoms in either the bulk material or encapsulated in a bubble is shifted to energies higher than that in the free atom. For bulk helium, the energy shifts predicted from…
The quantum entanglement for the two electrons in the excited states of the helium-like atom/ions is investigated using the two-electron wave functions constructed by the B-spline basis. As a measure of the spatial (electron-electron…
We study the entire energy spectrum of an electron droplet in the lowest Landau level. By exact diagonalization calculations, we find highly excited states in the middle of the spectrum that display unexpected density distribution and pair…
Superfluid helium nanodroplets are often considered as transparent and chemically inert nanometer-sized cryo-matrices for high-resolution or time-resolved spectroscopy of embedded molecules and clusters. On the other hand, when the helium…
The total energies and various bound state properties of the excited $2^1S(L = 0)-$states in two-electron helium atoms, including the ${}^{\infty}$He, ${}^4$He and ${}^3$He atoms, are determined to very high numerical accuracy. The…
We study dissipation effects for electrons on the surface of liquid helium, which may serve as qubits of a quantum computer. Each electron is localized in a 3D potential well formed by the image potential in helium and the potential from a…
We present measurements of the resonant microwave absorption by the Rydberg energy levels of surface state electrons on the surface of superfluid liquid helium, in the frequency range 165 - 220 GHz. The resonant frequency was strongly…
Guided by the analogy to the Bose-Einstein condensation of the ideal Bose gas (IBG) we propose a new model for the lambda transition of liquid helium. Deviating from the IBG our model uses phase ordered and localized single-particle…
We investigate an extension of excited state mean-field theory in which the energy expression is augmented with density functional components in an effort to include the effects of weak electron correlations. The approach remains…
We use the density functional method to examine the properties of the nonuniform (two-phase) fluid of two-level atoms, a part of which is excited. Basing on the analysis of the equation of state of a gas of two-level atoms, a part of which…
We construct an efficient zero-temperature semi-local density functional to dynamically simulate an electron bubble passing through superfluid 4He under various pressures and electric fields up to nanosecond timescale. Our simulated drift…
A set of density functionals coming from different rungs on Jacob's ladder are employed to evaluate the electronic excited states of three Ru(II) complexes. While most studies on the performance of density functionals compare the vertical…