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Because of new telescopes that will dramatically improve our knowledge of the interstellar medium, chemical models will have to be used to simulate the chemistry of many regions with diverse properties. To make these models more robust, it…

Astrophysics of Galaxies · Physics 2011-03-16 V. Wakelam , E. Herbst , J. Le Bourlot , F. Hersant , F. Selsis , S. Guilloteau

Gas-phase processes were long thought to be the key formation mechanisms for complex organic molecules in star-forming regions. However, recent experimental and theoretical evidence has cast doubt on the efficiency of such processes.…

Astrophysics · Physics 2009-11-13 Robin T. Garrod , Susanna L. Widicus Weaver , Eric Herbst

One of the stumbling blocks for studying the evolution of interstellar molecules is the lack of adequate knowledge of the rate co-efficients of various reactions which take place in the Interstellar medium and molecular clouds. Some of the…

Cosmology and Nongalactic Astrophysics · Physics 2015-03-20 Liton Majumdar , Ankan Das , Sandip K. Chakrabarti , Sonali Chakrabarti

Recent observations have revealed significant variations in the abundances of gas- and ice-phase molecules in galaxies with different luminosities and types. In order to discuss the physical origins of these variations, we incorporate gas-…

Astrophysics of Galaxies · Physics 2025-12-16 K. Bekki , K. Furuya , T. Shimonishi

The gas-phase chemistry of dark clouds has been studied with a treatment of uncertainties caused both by errors in individual rate coefficients and uncertainties in physical conditions. Moreover, a sensitivity analysis has been employed to…

Astrophysics · Physics 2009-11-11 Valentine Wakelam , Eric Herbst , Franck Selsis

AIM: We have recently developed a microscopic Monte Carlo approach to study surface chemistry on interstellar grains and the morphology of ice mantles. The method is designed to eliminate the problems inherent in the rate-equation formalism…

Astrophysics · Physics 2009-11-13 Q. Chang , H. M. Cuppen , E. Herbst

Astrochemical models are essential to bridge the gap between the timescales of reactions, experiments, and observations. Ice chemistry in these models experiences a large computational complexity as a result of the many parameters required…

Astrophysics of Galaxies · Physics 2026-02-18 Tobias M. Dijkhuis , Thanja Lamberts , Serena Viti , Herma M. Cuppen

The observed gas-phase molecular inventory of hot cores is believed to be significantly impacted by the products of chemistry in interstellar ices. In this study, we report the construction of a full macroscopic Monte Carlo model of both…

Astrophysics of Galaxies · Physics 2015-06-12 A. I. Vasyunin , E. Herbst

Chemical models used to study the chemical composition of the gas and the ices in the interstellar medium are based on a network of chemical reactions and associated rate coefficients. These reactions and rate coefficients are partially…

A new chemical model is presented for the carbon-rich circumstellar envelope of the AGB star IRC+10216. The model includes shells of matter with densities that are enhanced relative to the surrounding circumstellar medium. The chemical…

Astrophysics of Galaxies · Physics 2009-11-13 M. A. Cordiner T. J. Millar

Context: Diffusion of species on the dust surface is a key process for determining the chemical composition of interstellar ices. On the dust surface, adsorbed species diffuse from one potential well to another and react with other adsorbed…

Astrophysics of Galaxies · Physics 2018-12-12 Wasim Iqbal , Valentine Wakelam , Pierre Gratier

We discuss models that astrochemists have developed to study the chemical composition of the interstellar medium. These models aim at computing the evolution of the chemical composition of a mixture of gas and dust under as- trophysical…

Astrophysics of Galaxies · Physics 2013-10-01 Valentine Wakelam , Herma M. Cuppen , Eric Herbst

The physical conditions in a collapsing cloud can be traced by observations of molecular lines. To correctly interpret these observations the abundance distributions of the observed species need to be derived. The chemistry in a collapsing…

Solar and Stellar Astrophysics · Physics 2009-11-13 R. J. van Weeren , C. Brinch , M. R. Hogerheijde

The evolution of star-forming regions and their thermal balance are strongly influenced by their chemical composition, that, in turn, is determined by the physico-chemical processes that govern the transition between the gas phase and the…

HNC and HCN, typically used as dense gas tracers in molecular clouds, are a pair of isomers that have great potential as a temperature probe because of temperature dependent, isomer-specific formation and destruction pathways. Previous…

Astrophysics of Galaxies · Physics 2015-06-19 Dawn Graninger , Eric Herbst , Karin I. Oberg , Anton I. Vasyunin

Dust grains are an important component of the interstellar medium (ISM) of galaxies. We present the first direct measurement of the residence times of interstellar dust in the different ISM phases, and of the transition rates between these…

We review the reactions involving HCN and HNC in dark molecular clouds to elucidate new chemical sources and sinks of these isomers. We find that the most important reactions for the HCN-HNC system are Dissociative Recombination (DR)…

Astrophysics of Galaxies · Physics 2015-06-19 Jean-Christophe Loison , Valentine Wakelam , Kevin M. Hickson

Theoretical studies have revealed that dust grains are usually moving fast through the turbulent interstellar gas, which could have significant effects upon interstellar chemistry by modifying grain accretion. This effect is investigated in…

Astrophysics of Galaxies · Physics 2015-12-09 J. X. Ge , J. H. He , H. R. Yan

Ice is ubiquitous in the interstellar medium. We model the formation of the main constituents of interstellar ices, including H2O, CO2 , CO, and CH3 OH. We strive to understand what physical or chemical parameters influence the final…

Astrophysics of Galaxies · Physics 2023-07-26 A. Clément , A. Taillard , V. Wakelam , P. Gratier , J. -C. Loison , E. Dartois , F. Dulieu , J. A. Noble , M. Chabot

Chemical models have been developed over the years by astrophysicists to study the pro- cesses at play in the various environments of the interstellar medium (ISM) that define the chemical composition of the gas and the dust. These…

Astrophysics of Galaxies · Physics 2013-10-15 Marcelino Agundez , Valentine Wakelam